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High Precision, Not High Energy 
Using Atomic Physics to Look Beyond the Standard Model 
Part 1: Impossible Things
Image credit: Fermilab
Source: Harvard/ Chandra Source: CERN Bulletin 
Source: J-PARC
Particle 
Physics?
Beyond the Standard Model 
Ways to look for new physics: 
1) Direct creation 
Accelerate particles to near 
light-speed, convert that energy 
to matter
Images: CERN 
ATLAS 
CMS
Beyond the Standard Model 
Ways to look for new physics: 
1) Direct creation 
2) Passive detection 
Build large detector sensitive 
to particles of interest, hope 
one happens by 
Image: Super-Kamiokande
Beyond the Standard Model 
Ways to look for new physics: 
1) Direct creation 
2) Passive detection 
Image: Mike Tarbutt/ Physics World 
3) Precision measurement 
Look for exotic physics in 
relatively mundane systems 
using precision spectroscopy to 
measure extremely tiny effects
LHC vs AMO 
Particle Physics 
Energy scale: ~1TeV 
Length scale: ~ 10-19 m 
Atomic Physics 
Photo by Matt Milless 
Energy scale: ~1eV 
Length scale: ~ 10-10 m 
Vast scale mismatch: How do AMO systems detect new physics? 
Measuring tiny effects is what we do...
Historical Precedent 
~1930, Dirac: Relativistic equation for electron 
Predicts energy levels of hydrogen 
Willis Lamb Image: National 
Archives and Records 
Administration, via AIP Emilio 
Segre Visual Archives 
1947, Willis Lamb, Robert Retherford: 
Measure shift between two energy 
levels that Dirac equation predicts 
should have same energy 
“Lamb Shift” energy: 4.372×10-6 eV 
(out of ~10 eV) 
 Kick-starts development of QED
QED 
Energy of electron depends on interaction with nucleus 
Feynman picture: exchange photons 
Electron 
Photon 
N 
U 
C 
L 
E 
U 
S 
Time 
Space 
Story in pictures: 
Once upon a time, there was 
an electron moving along 
through space, and it 
exchanged a photon with the 
nucleus, which changed its 
momentum. 
The End … Or Is It?
Virtual Particles 
Quantum Physics: Everything not forbidden is mandatory 
 QED story has to include additional effects 
Electron 
Photon 
Virtual 
Photon 
N 
U 
C 
L 
E 
U 
S 
Virtual 
Positron 
Virtual 
Electron 
N 
U 
C 
L 
E 
U 
S 
Electron Self-Energy Vacuum Polarization
Lamb Shift 
What difference does this make? 
QED effects “smear out” 
electron position over a small 
range 
“Pushes” electron farther from 
nucleus  reduces energy 
Probability 
(not to scale) 
Distance 
Distance scale: ~10-16 m 
(1/10th size of nucleus) 
 Extremely small shift, but detectable 
Nobels for Lamb, Kusch, Feynman, Schwinger, Tomonaga…
Atomic Structure 
Diagram from http://raptor.physics.wisc.edu/download2.htm 
States defined by: 
Electronic energy 
Angular momentum 
Spin 
Nuclear Spin 
Selection rules: 
Only certain types of 
transitions allowed 
Control transitions by 
choosing light 
properties: frequency, 
intensity, polarization
Atomic Structure 
 Frequency 
Diagram from http://raptor.physics.wisc.edu/download2.htm 
Selection rules: 
Only certain types of 
transitions allowed 
… WHY? 
Symmetry, conservation laws 
Light carries: 
Energy 
Momentum 
Angular 
momentum 
 Forces 
 Polarization
CPT 
Fundamental symmetry transformations: 
+ 
+ 
- 
- 
+ 
+ 
+ 
+ 
Charge Parity Time 
Physics looks the same under these 
…except when it doesn’t
Parity Symmetry 
NORDITA
Parity Violation
CPT 
Fundamental symmetry transformations: 
+ 
+ 
- 
- 
+ 
+ 
+ 
+ 
Charge Parity Time 
Physics looks the same under these 
…except when it doesn’t
Parity Violation 
Chien-ShiungWu, 1963 
http://commons.wikimedia.org/wiki/File:Chien-shiung_Wu_(1912-1997).jpg 
http://commons.wikimedia.org/wiki/File:Wu_experiment.jpg
CPT 
Fundamental symmetry transformations: 
+ 
+ 
- 
- 
+ 
+ 
+ 
+ 
Charge Parity Time 
Individual symmetries violated 
Product of all three– “CPT” symmetry– preserved
CPT 
Fundamental symmetry transformations: 
+ 
+ 
- 
- 
+ 
+ 
+ 
+ 
Charge Parity Time 
Many atomic selection 
rules are parity-based
Parity Violation in Atoms 
Simplest search for exotic physics: 
Look for transitions that 
shouldn’t happen 
Example: 6S7S in Cs 
First measured (in Cs): 
1982 Bouchiat et al.
Parity Violation in Cesium 
Principle of measurement: 
Use green laser to excite forbidden 
transition 
Look at fluorescence from allowed 
transition 
539.4 nm 
1360 nm 
Technical details: 
Apply electric field to define 
preferred direction 
Field mixes states, allowing 
some transition 
Parity violation rotates 
polarization of light
Parity Violation in Atoms 
Simplest search for exotic physics: 
Look for transitions that 
shouldn’t happen 
Example: 6S7S in Cs 
First measured (in Cs): 
1982 Bouchiat et al. 
Current most precise (Cs): 
1.5935±0.0056 mV/cm 
(Boulder 1997) 
 10-11 times allowed transition
Atomic Parity Violation and New Physics 
Parity violating transitions test electroweak physics 
Weak interactions allow parity violation (as in Wu experiment) 
 compare measured values to SM predictions 
 Very theory-dependent 
Catch-22: Parity violation enhanced in heavy atoms (~Z3)… 
…but necessary theory much harder in heavy atoms 
Cesium: current best, because it’s a “one-electron” atom
Francium 
Atomic theory simpler in “one-electron” atoms alkali metals 
 Do APV measurements in francium 
PROBLEM: No stable isotopes of Fr 
Fr
Francium Trapping 
Produce Fr isootpes in accelerator at TRIUMF 
Laser cool, trap, do spectroscopy 
Image source: L. Orozco 
http://www.physics.umd.edu/rgroups/amo/orozco/results/2012/CAARI12.pdf
Francium Trapping 
100,000 209Fr atoms 
Trapped for ~20s 
From Tandecki et al., arXiv:1312.3562 (2013)
Atomic Parity Violation and New Physics 
Parity violating transitions test electroweak physics 
Weak interactions allow parity violation (as in Wu experiment) 
 compare measured values to SM predictions 
 Very theory-dependent 
Catch-22: Parity violation enhanced in heavy atoms (~Z3)… 
…but necessary theory much harder in heavy atoms 
Cesium: current best, because it’s a “one-electron” atom 
Other elements have larger APV effects: 
Thallium, Bismuth, Ytterbium,…
Parity Violation in Yb 
Budker group at UC-Berkeley, 2009 
100x bigger 
APV than Cs 
From Tsigutkin et al., PRL 103, 071601 (2009)
Parity Violation Prospects 
No signs of new physics …yet 
Incremental improvements: 
Better measurements 
 steady technical improvements 
Better theory 
 dominant source of uncertainty 
Closely linked 
More drastic changes: 
Different atomic systems 
Bigger effects in Tl, Yb, Fr, Ra+… 
Multiple isotopes allow investigation of nuclear effects 
Change to measuring frequency shift, rather than probability 
…about which more later…
Other Things That Shouldn’t Happen 
http://arxiv.org/abs/1001.1771
Other Things That Shouldn’t Happen
Location, Location, Location 
Factor of 26,000 
improvement
New Physics from Forbidden Events 
Parity-Violating Transitions 
 Observed, levels consistent with Standard Model 
Photon Statistics, other departures from normal 
 No sign, consistent with Standard Model 
Lorentz/ CPT symmetry violation 
 No sign, consistent with Standard Model 
 Standard Model holding strong… 
… but more stringent tests possible 
 frequency shift measurements
Names to Conjure With 
Experiment Theory 
Andrei Derevianko 
http://www.dereviankogroup.com/ 
Marianna Safranova 
http://www.physics.udel.edu/~msafrono/ 
Michael Romalis 
http://physics.princeton.edu/romalis/ 
Dmitry Budker 
http://budker.berkeley.edu/ 
Luis Orozco 
http://www.physics.umd.edu/rgroups/amo/orozco/ 
Larry Hunter 
https://www.amherst.edu/people/facstaff/lrhunter/ 
Alan Kostelecky 
http://www.physics.indiana.edu/~kostelec/faq.html 
DISCLAIMER: This is a highly biased selection from a larger 
community, and not a complete list by any means
Old Physics 
1913: Bohr model 
Electrons restricted to special orbits 
Absorb/emit light when 
moving between allowed 
states 
Energy of nth state: 퐸푛 = − 
퐸1 
푛2 
Energy of light: ℎ푓 = |퐸푓푖푛푎푙 − 퐸푖푛푖푡푖푎푙 | 
Scale: E1 ~ 10 – 1 eV 
f ~ 1015 – 1014 Hz 
l ~ 100 – 1000 nm
Old Physics 
~1930: Fine structure 
Additional effects shift energy states 
 Relativity 
 “Spin-orbit” interaction 
Fine structure constant 
Scale: DEfs ~ Z2a2 E ~ 10-5 – 10-2 eV 
Df fs~ 1010 – 1013 Hz 
Dlfs ~ 0.01 – 10 nm 
훼 = 
1 
4휋휖0 
푒2 
ℏ푐 
~ 
1 
137
Old Physics 
~1920’s: Hyperfine structure 
Electron, nucleus act like magnets 
Spin-spin interaction 
Split “spin up” and “spin down” 
Important technologies: 
“21-cm line” in H: Radio astronomy, NMR 
Cs ground state: Atomic clocks, GPS 
Scale: DEhfs ~ Za2 푚푒푙푒푐푡푟표푛 
푚푝푟표푡표푛 
E ~ 10-5 – 10-8 eV 
Dfhfs ~ 107 – 1010 Hz 
Dlhfs ~ 0.01 – 10 cm
Atoms and Light 
Everything we know about atoms and molecules comes from 
studying how they interact with light 
Simplest picture: Fully Quantum 
Atoms have discrete energy states 
Light is stream of photons with 
discrete energy 
Photon energy = Difference between states 
|퐸푓푖푛푎푙 − 퐸푖푛푖푡푖푎푙 | = ℎ푓
Atoms and Light II 
Second-simplest picture: Einstein 1917 
Three processes: 
1) Spontaneous emission 
Atoms in higher-energy 
states emit light, drop down 
2) Resonant absorption 
Atoms in lower-energy states 
absorb light, move up 
3) Stimulated emission 
Atoms in higher-energy 
interact with light, emit 
more, drop down 
A21 B21 B12 
A and B coefficients 
 probability of each 
 relationship between
Atoms and Light III 
Most complicated picture: Rabi Oscillations 
“Semi-classical” treatment: 
Atoms have discrete states 
Light treated as wave 
(Must work when Nphotons >> 1 ) 
Qualitative features: 
1) Atoms oscillate between ground & excited states 
2) Oscillation at “Rabi Frequency” W 
Ω~ 퐼푛푡푒푛푠푖푡푦 
3) Atoms in coherent superposition of states
Time 
Probability of Excitation 
1.0 
0.8 
0.6 
0.4 
0.2 
0.0 
Rabi Oscillations 
Fast oscillations 
 Driving 
Slow decay 
 decoherence
Atoms and Light III 
Most complicated picture: Rabi Oscillations 
Ω~ 퐼푛푡푒푛푠푖푡푦 
Rabi oscillations allow complete control 
of atomic state 
 Know laser power, know time needed to prepare any 
arbitrary superposition of states 
Key terms: “p-pulse”  drive all atoms from one state to other 
“p/2-pulse”  drive all atoms into equal 
superposition of two states
Anapole Moment

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High Precision, Not High Energy: Using Atomic Physics to Look Beyond the Standard Model (Part I)

  • 1. High Precision, Not High Energy Using Atomic Physics to Look Beyond the Standard Model Part 1: Impossible Things
  • 3. Source: Harvard/ Chandra Source: CERN Bulletin Source: J-PARC
  • 5. Beyond the Standard Model Ways to look for new physics: 1) Direct creation Accelerate particles to near light-speed, convert that energy to matter
  • 7. Beyond the Standard Model Ways to look for new physics: 1) Direct creation 2) Passive detection Build large detector sensitive to particles of interest, hope one happens by Image: Super-Kamiokande
  • 8.
  • 9. Beyond the Standard Model Ways to look for new physics: 1) Direct creation 2) Passive detection Image: Mike Tarbutt/ Physics World 3) Precision measurement Look for exotic physics in relatively mundane systems using precision spectroscopy to measure extremely tiny effects
  • 10. LHC vs AMO Particle Physics Energy scale: ~1TeV Length scale: ~ 10-19 m Atomic Physics Photo by Matt Milless Energy scale: ~1eV Length scale: ~ 10-10 m Vast scale mismatch: How do AMO systems detect new physics? Measuring tiny effects is what we do...
  • 11. Historical Precedent ~1930, Dirac: Relativistic equation for electron Predicts energy levels of hydrogen Willis Lamb Image: National Archives and Records Administration, via AIP Emilio Segre Visual Archives 1947, Willis Lamb, Robert Retherford: Measure shift between two energy levels that Dirac equation predicts should have same energy “Lamb Shift” energy: 4.372×10-6 eV (out of ~10 eV)  Kick-starts development of QED
  • 12. QED Energy of electron depends on interaction with nucleus Feynman picture: exchange photons Electron Photon N U C L E U S Time Space Story in pictures: Once upon a time, there was an electron moving along through space, and it exchanged a photon with the nucleus, which changed its momentum. The End … Or Is It?
  • 13. Virtual Particles Quantum Physics: Everything not forbidden is mandatory  QED story has to include additional effects Electron Photon Virtual Photon N U C L E U S Virtual Positron Virtual Electron N U C L E U S Electron Self-Energy Vacuum Polarization
  • 14. Lamb Shift What difference does this make? QED effects “smear out” electron position over a small range “Pushes” electron farther from nucleus  reduces energy Probability (not to scale) Distance Distance scale: ~10-16 m (1/10th size of nucleus)  Extremely small shift, but detectable Nobels for Lamb, Kusch, Feynman, Schwinger, Tomonaga…
  • 15. Atomic Structure Diagram from http://raptor.physics.wisc.edu/download2.htm States defined by: Electronic energy Angular momentum Spin Nuclear Spin Selection rules: Only certain types of transitions allowed Control transitions by choosing light properties: frequency, intensity, polarization
  • 16. Atomic Structure  Frequency Diagram from http://raptor.physics.wisc.edu/download2.htm Selection rules: Only certain types of transitions allowed … WHY? Symmetry, conservation laws Light carries: Energy Momentum Angular momentum  Forces  Polarization
  • 17. CPT Fundamental symmetry transformations: + + - - + + + + Charge Parity Time Physics looks the same under these …except when it doesn’t
  • 20. CPT Fundamental symmetry transformations: + + - - + + + + Charge Parity Time Physics looks the same under these …except when it doesn’t
  • 21. Parity Violation Chien-ShiungWu, 1963 http://commons.wikimedia.org/wiki/File:Chien-shiung_Wu_(1912-1997).jpg http://commons.wikimedia.org/wiki/File:Wu_experiment.jpg
  • 22. CPT Fundamental symmetry transformations: + + - - + + + + Charge Parity Time Individual symmetries violated Product of all three– “CPT” symmetry– preserved
  • 23. CPT Fundamental symmetry transformations: + + - - + + + + Charge Parity Time Many atomic selection rules are parity-based
  • 24. Parity Violation in Atoms Simplest search for exotic physics: Look for transitions that shouldn’t happen Example: 6S7S in Cs First measured (in Cs): 1982 Bouchiat et al.
  • 25. Parity Violation in Cesium Principle of measurement: Use green laser to excite forbidden transition Look at fluorescence from allowed transition 539.4 nm 1360 nm Technical details: Apply electric field to define preferred direction Field mixes states, allowing some transition Parity violation rotates polarization of light
  • 26. Parity Violation in Atoms Simplest search for exotic physics: Look for transitions that shouldn’t happen Example: 6S7S in Cs First measured (in Cs): 1982 Bouchiat et al. Current most precise (Cs): 1.5935±0.0056 mV/cm (Boulder 1997)  10-11 times allowed transition
  • 27. Atomic Parity Violation and New Physics Parity violating transitions test electroweak physics Weak interactions allow parity violation (as in Wu experiment)  compare measured values to SM predictions  Very theory-dependent Catch-22: Parity violation enhanced in heavy atoms (~Z3)… …but necessary theory much harder in heavy atoms Cesium: current best, because it’s a “one-electron” atom
  • 28. Francium Atomic theory simpler in “one-electron” atoms alkali metals  Do APV measurements in francium PROBLEM: No stable isotopes of Fr Fr
  • 29. Francium Trapping Produce Fr isootpes in accelerator at TRIUMF Laser cool, trap, do spectroscopy Image source: L. Orozco http://www.physics.umd.edu/rgroups/amo/orozco/results/2012/CAARI12.pdf
  • 30. Francium Trapping 100,000 209Fr atoms Trapped for ~20s From Tandecki et al., arXiv:1312.3562 (2013)
  • 31. Atomic Parity Violation and New Physics Parity violating transitions test electroweak physics Weak interactions allow parity violation (as in Wu experiment)  compare measured values to SM predictions  Very theory-dependent Catch-22: Parity violation enhanced in heavy atoms (~Z3)… …but necessary theory much harder in heavy atoms Cesium: current best, because it’s a “one-electron” atom Other elements have larger APV effects: Thallium, Bismuth, Ytterbium,…
  • 32. Parity Violation in Yb Budker group at UC-Berkeley, 2009 100x bigger APV than Cs From Tsigutkin et al., PRL 103, 071601 (2009)
  • 33. Parity Violation Prospects No signs of new physics …yet Incremental improvements: Better measurements  steady technical improvements Better theory  dominant source of uncertainty Closely linked More drastic changes: Different atomic systems Bigger effects in Tl, Yb, Fr, Ra+… Multiple isotopes allow investigation of nuclear effects Change to measuring frequency shift, rather than probability …about which more later…
  • 34. Other Things That Shouldn’t Happen http://arxiv.org/abs/1001.1771
  • 35. Other Things That Shouldn’t Happen
  • 36. Location, Location, Location Factor of 26,000 improvement
  • 37. New Physics from Forbidden Events Parity-Violating Transitions  Observed, levels consistent with Standard Model Photon Statistics, other departures from normal  No sign, consistent with Standard Model Lorentz/ CPT symmetry violation  No sign, consistent with Standard Model  Standard Model holding strong… … but more stringent tests possible  frequency shift measurements
  • 38.
  • 39. Names to Conjure With Experiment Theory Andrei Derevianko http://www.dereviankogroup.com/ Marianna Safranova http://www.physics.udel.edu/~msafrono/ Michael Romalis http://physics.princeton.edu/romalis/ Dmitry Budker http://budker.berkeley.edu/ Luis Orozco http://www.physics.umd.edu/rgroups/amo/orozco/ Larry Hunter https://www.amherst.edu/people/facstaff/lrhunter/ Alan Kostelecky http://www.physics.indiana.edu/~kostelec/faq.html DISCLAIMER: This is a highly biased selection from a larger community, and not a complete list by any means
  • 40. Old Physics 1913: Bohr model Electrons restricted to special orbits Absorb/emit light when moving between allowed states Energy of nth state: 퐸푛 = − 퐸1 푛2 Energy of light: ℎ푓 = |퐸푓푖푛푎푙 − 퐸푖푛푖푡푖푎푙 | Scale: E1 ~ 10 – 1 eV f ~ 1015 – 1014 Hz l ~ 100 – 1000 nm
  • 41. Old Physics ~1930: Fine structure Additional effects shift energy states  Relativity  “Spin-orbit” interaction Fine structure constant Scale: DEfs ~ Z2a2 E ~ 10-5 – 10-2 eV Df fs~ 1010 – 1013 Hz Dlfs ~ 0.01 – 10 nm 훼 = 1 4휋휖0 푒2 ℏ푐 ~ 1 137
  • 42. Old Physics ~1920’s: Hyperfine structure Electron, nucleus act like magnets Spin-spin interaction Split “spin up” and “spin down” Important technologies: “21-cm line” in H: Radio astronomy, NMR Cs ground state: Atomic clocks, GPS Scale: DEhfs ~ Za2 푚푒푙푒푐푡푟표푛 푚푝푟표푡표푛 E ~ 10-5 – 10-8 eV Dfhfs ~ 107 – 1010 Hz Dlhfs ~ 0.01 – 10 cm
  • 43. Atoms and Light Everything we know about atoms and molecules comes from studying how they interact with light Simplest picture: Fully Quantum Atoms have discrete energy states Light is stream of photons with discrete energy Photon energy = Difference between states |퐸푓푖푛푎푙 − 퐸푖푛푖푡푖푎푙 | = ℎ푓
  • 44. Atoms and Light II Second-simplest picture: Einstein 1917 Three processes: 1) Spontaneous emission Atoms in higher-energy states emit light, drop down 2) Resonant absorption Atoms in lower-energy states absorb light, move up 3) Stimulated emission Atoms in higher-energy interact with light, emit more, drop down A21 B21 B12 A and B coefficients  probability of each  relationship between
  • 45. Atoms and Light III Most complicated picture: Rabi Oscillations “Semi-classical” treatment: Atoms have discrete states Light treated as wave (Must work when Nphotons >> 1 ) Qualitative features: 1) Atoms oscillate between ground & excited states 2) Oscillation at “Rabi Frequency” W Ω~ 퐼푛푡푒푛푠푖푡푦 3) Atoms in coherent superposition of states
  • 46. Time Probability of Excitation 1.0 0.8 0.6 0.4 0.2 0.0 Rabi Oscillations Fast oscillations  Driving Slow decay  decoherence
  • 47. Atoms and Light III Most complicated picture: Rabi Oscillations Ω~ 퐼푛푡푒푛푠푖푡푦 Rabi oscillations allow complete control of atomic state  Know laser power, know time needed to prepare any arbitrary superposition of states Key terms: “p-pulse”  drive all atoms from one state to other “p/2-pulse”  drive all atoms into equal superposition of two states