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International Research Journal of Engineering and Technology (IRJET) e-ISSN: 2395-0056
Volume: 04 Issue: 07 | July -2017 www.irjet.net p-ISSN: 2395-0072
© 2017, IRJET | Impact Factor value: 5.181 | ISO 9001:2008 Certified Journal | Page 582
Taguchi method of optimization performed on 49 cm2 active area on
interdigitated flow channel of PEMFC
Dr V LAKSHMINARAYANAN
Department of Mechanical Engineering, B V Raju Institute of Technology, Narsapur, Telangana, India - 502313
---------------------------------------------------------------------***---------------------------------------------------------------------
Abstract - In this paper, optimization of operating and
design parameters on interdigitatedflowchannelwith49cm2
effective area of the Proton Exchange Membrane Fuel Cell
(PEMFC) was considered numerically using CFD and Minitab
17 software. The factors considered for the optimization was
landing to channel width ratios (L: C) -1:1, 1:2, 2:1 and 2:2,
operating pressure (1, 1.5, 2 and 2.5 bar), temperature (313,
323, 333 and 343 K), anode and cathode reactants as
stoichiometric ratios (S/F) of 3, 3.5, 4 and 4.5. Based on the
optimization study, the L:C-1:2 has maximum influence on
PEMFC performance and square of response factor (R2) was
achieved by Taguchi method as 99.9 %.
Key Words: Interdigitated flow channel;CFD;Optimization;
Design parameters; operating parameters.
1. INTRODUCTION
The Proton Exchange Membrane Fuel Cell (PEMFC) is an
electrochemical device, which is convertingchemical energy
of fuels (hydrogen and oxygen) directly into electricity
without any intermediate stage like classical combustion of
two and four stroke engine. The PEMFC performance
depends on the channel depth and width, flow channel
design, number of flow path, cross section of the flow
channel, operating pressure, temperature,relativehumidity,
mass flow rate of the reactant gases and stoichiometricratio
of the reactants. It is being developed for commercial
applications in the field of transportation and back-up
power. One of the main advantages of the fuel cells is the
negligible emission of pollutants, such as SOx, NOx,
particulates. It is Eco-friendlypowersourcewhichissuitable
for powering both portable devices and mobile application
due to their high energy density and lower operating
temperature range [1 & 2].The effect of the various
parameters like landing width to channel width of (L: C) 1:1,
1:2 and 2:2 Multi pass serpentine flow channel PEMFC with
36 cm2 (6cm x 6cm) active area was analyzednumericallyby
Lakshminarayanan et al [3].The results revealed that the
maximum power densities were obtained 0.658W/cm2 for
the L: C of 1:1. Guvelioglu & Stenger [4] studied a CFD model
to analyse the effects of channel size, electrode porosity and
reactant humidification on the performance of PEMFC. The
results revealed thatsmaller sizedchannelswererequiredto
obtain the higher current densities,althoughlargerchannels
were satisfactory to produce moderate current densities.
The effect of the relative humidity of the anode gas stream
was found to be the important factor for affecting the
performance of the PEMFC.
Ahmed & Sung [5] investigated the performance of PEMFCs
with different flow fields like a rectangular, trapezoidal and
parallelogram using CFD. The results showed that a
rectangular flow field gave higher cell voltages compared
with parallelogram and trapezoidal flowfields.However, the
trapezoidal flow field helped reactant diffusion, uniform
reactant flow and current density circulations over the
reacting area, results in lower cathode over potential of the
fuel cell. The performance enhancement of the combined
effect of design and operating parametersofbothserpentine
and interdigitated flow channel with 25 cm2 active area of
PEM fuel cell with four different parameters using
optimization technique and CFD carried out by
Lakshminarayanan and Karthikeyan [6]. The results
revealed that the peak power density of interdigitated flow
channel with landing to channel width (L:C)1:2 showed
better than the serpentineflowchannel withL:C-1:2.Grujicic
and Chittajallu [7] have studied the performance of PEMFC
by using a single-phase two-dimensional electrochemical
model. The model was coupled with a nonlinearconstrained
optimization algorithm to define an optimum design of the
fuel cell with respect to the operation and the geometrical
parameters of the cathode. The results of the optimization
analysis showed that higher current densities at a constant
cell voltage were obtained as the inlet air pressure. On the
other hand, the statistical sensitivityanalysisresultsshowed
that the equilibriumcathode/membranepotential difference
has the largest effect on the predicted polarization curve of
the PEMFC. Karthikeyan et al. [8] studiedtheperformance of
single channel PEMFC using Taguchi method for various
operating and design parameters like cell temperature,back
pressure, anode and cathode inlet velocities, porosity and
thickness of the gas diffusion layer, cathode water mass
fraction, flow channel dimensions, rib width and porous
electrode thickness. The results revealed that the back
pressure showed maximum effect and rib width had less
effect on the PEMFC performance in the first stage. Further,
enhancement of power density by 3% when selected factors
in the second stage of fine-tuned optimization has been
carried out.
Wu et al. [9] integrated the neural network and Taguchi
technique for parametric analysis with various parameters
like operating temperatures, cathode and anode
humidification temperature, operating pressure, and
reactant flow rate for the enhancement of PEMFC
International Research Journal of Engineering and Technology (IRJET) e-ISSN: 2395-0056
Volume: 04 Issue: 07 | July -2017 www.irjet.net p-ISSN: 2395-0072
© 2017, IRJET | Impact Factor value: 5.181 | ISO 9001:2008 Certified Journal | Page 583
performance. The results indicated that among the various
parameters, temperature and pressure were the major
factors to influence the PEMFC performance. The effects of
interdigitated flow channel withtraditional flowchannel,the
effects of the flow area ratio and the baffle-blocked position
of the interdigitated flow field on the performanceofPEMFC
were examined experimentally by Yan et al [10]. The results
concluded that, the cell performance can be enhanced with
an increased inlet flow rate of reactant and cathode
humidification temperature. The interdigitated flow fields
have better performancethanconventional flowfielddesign.
Also the results showed that the interdigitated flow fieldhas
larger limiting current density, and the power output was
about 1.4 times than the conventional flow field. It is clearly
indicated that immediateattentionisrequiredforoptimizing
the simultaneous influence of operating and design
parameters for the performance of the PEMFC. Hence this
paper has a detailed study about the optimization of
operating parameters like operating pressure, temperature,
stoichiometric ratio of inlet reactant mass flow rate and
design parameter like various rib width to channel width
(L:C)-1:1, 1:2, 2:1& 2:2 on interdigitated flow channel of 49
cm2 active area of PEMFC are to be studied and compared
the influence of individual parameters contribution on the
total performance of PEMFC.
2. MODEL DEVELOPMENT
The modeling was done by creating all individual partsofthe
PEMFC and the dimensions of individual parts such as the
anodeandcathodeGDL,solidpolymerelectrolytemembrane,
the anode and cathode catalyst layers as shown in the Table
1. Three dimensional (3-D) PEMFC modelwithinterdigitated
flow channel of various landing width to channel width ratio
(L: C) -1:1, 1:2, 2:1 and 2:2 was created by Creo Parametric
2.0 and meshed by using ICEM 14.5 (a module of Ansys 14.5)
as shown in Fig.1.
Table -1: Dimensions and Zone type of parts assigning of
fuel cell
(a)
(b)
(c)
(d)
Fig -1: Various landing to channel width (L: C) (a) 1:1 (b)
1:2 (c) 2:1 and (d) 2:2 of interdigitated flow channel of 49
cm2 active area of PEMFC
S.
No
Part Name
Wid
th
(mm
)
Len
gth
(mm
)
Thickn
ess
(mm)
Zone
type
1
Anode & Cathode
Flow channel
70 70
10 Solid
2
Anode & Cathode
catalyst 0.08
Fluid
3 Membrane
0.127
Fluid
4
GDL anode &
cathode
0.3 Fluid
International Research Journal of Engineering and Technology (IRJET) e-ISSN: 2395-0056
Volume: 04 Issue: 07 | July -2017 www.irjet.net p-ISSN: 2395-0072
© 2017, IRJET | Impact Factor value: 5.181 | ISO 9001:2008 Certified Journal | Page 584
After geometry modeling, thenextstepwasdiscretization
of PEMFC donebyICEMsoftware.TheCartesiangridmeshing
method was used, which is used in the formation of
hexahedral mesh to attain accurate results. Split block
method was used forblocking and bodyfittedmeshwasused
for meshing. The projection factor was set to 1and the
projection factor decides how closely the edges of the mesh
match up with the grid.
The simulation of PEMFC was solved by simultaneous
equations like conservation of mass, momentum, energy,
species concentration, butler–Volmerequation,Jouleheating
reaction and the Nernst equation to obtain reaction kinetics.
The model used to consider the system as 3-D, steady state
and inlet gases as ideal condition, system as an isothermal
and flow aslaminar, fluid as incompressible,thermophysical
properties as constant and the porous GDL, two catalyst
layers and the membrane as an isotropic.
A control volume approach based on commercial solver
FLUENT 14.5 was used to solve the various governing
equations. Three-dimensional, double precision and serial
processing were used for this model. The species
concentration on anode side of H2, O2, and H2O were set to
0.8, 0, and 0.2 respectively. Similarly, on the cathode side
were set as 0, 0.2 and 0.1 respectively. The porosity at anode
and cathodesidewas 0.5. Open circuit voltage wassetat0.95
V on the cathode and the anode was grounded. The cathode
voltage has been varied from 0.05 V to 0.95Vusedforsolving
kinetics reaction in order to get the current flux density H2,
O2, and H2O fractions along with the flow field design.
Multigrid settings were modified as F-Cycle for all the
equations and entered termination restriction value was set
as 0.001 for H2, O2, H2O and water saturation. The Anode and
Cathode reference currentdensitywassettobe10000A/cm2
and 20 A/cm2 respectively 0.1 kmol/m3 wasset to anodeand
cathode reference concentration, Anode and cathode
exchange coefficient was settobe2.TheReferencediffusivity
of H2, O2 and H2O was set to as 3E-5. The electric and proton
potential values were set at 0.0001. Stabilization method
BCGSTAB was selected for H2, O2, H2O, water saturation,
electric and proton potential.
Taguchi method of optimization has been usedtofindout
the most optimum combination among the various input
parameters which would result in getting the maximum
possible output whichcausesthe performanceenhancement
of PEMFC. The factorsconsidered for the analysis were rib to
channel ratios on interdigitated flow field design (L: C-1:1,
1:2, 2:1 and 2:2), pressure(1,1.5, 2 and2.5bar),temperature
(313, 323, 333 and 343 K), anode and cathode reactants as
stoichiometric ratios (S/F) of 3, 3.5, 4 and 4.5. The standard
L16 orthogonal array with 4-level and 4factorswasusedand
the parameters were considered as low, high and medium
range values. When this orthogonal array was used,
significance of factors and optimum combination can be
found in 16 runs itself. The theoretical value of hydrogen in
the anode side was 4.33E-07 kg/s and oxygen in the cathode
side was 3.33E-06 kg/s.
3. RESULTS AND DISCUSSION
As per L16 orthogonal array,theinputsof16combination
of various parameters were given to the Ansys CFD Fluent
analysis software and having all other parameters constant.
The obtained power densities from analysis software for all
16 runs were fed in to the Minitab 17 software. The
corresponding Signal/Noise (S/N) ratios for all 16
combinations were found from Minitab 17 software itself as
shown in the Table 2.
The landing to channel width ratio of 1:1 for interdigitated
flow field has shown maximum power densities of 0.195
W/cm2 and minimum power densities of 0.142
W/cm2respectively. Similarly for L:C of 1:2 and 2:1 having
maximum power density of 0.203W/cm2 and 0.161 W/cm2
respectively. The minimum power densities for the sameL:C
ratios have 0.157W/cm2 and 0.127 W/cm2 respectively. For
the landing to channel width ratio of 2:2 has shown
maximum power density of 0.189 W/cm2andpowerdensity
of 0.159 W/cm2. The optimizationwasperformedfor“Larger
the Better” type of Taguchi method since power output of
PEMFC must be maximized. The S/N ratio plot for the same
were obtained using Minitab 17 software and the
corresponding maximum S/N ratio givesbetterperformance
as analyzed based on larger the better as shown in the Fig.2.
Table -2: Factors, levels, power density and S/N ratio for
16 runs of optimization
Ru
n
R:C
Pr
ess
ure
Tempe
rature
Stoi.
Rati
o
Power
Density
(W/cm2)
S/N Ratio
1
1x
1
1 313 3
0.141 -16.9838
2 1.5 323 3.5 0.159 -15.9262
3 2 333 4 0.179 -14.9638
4 2.5 343 4.5 0.195 -14.1839
5
1x
2
1 323 4 0.169 -15.4043
6 1.5 313 4.5 0.157 -16.0978
7 2 343 3 0.203 -13.8341
8 2.5 333 3.5 0.197 -14.1025
9
2x
1
1 333 4.5 0.144 -16.8392
10 1.5 343 4 0.161 -15.8525
11 2 313 3.5 0.127 -17.8901
12 2.5 323 3 0.143 -16.8818
13
2x
2
1 343 3.5 0.189 -14.4271
14 1.5 333 3 0.187 -14.5604
15 2 323 4.5 0.175 -15.1536
16 2.5 313 4 0.159 -15.9489
Average S/N Ratio -15.566
International Research Journal of Engineering and Technology (IRJET) e-ISSN: 2395-0056
Volume: 04 Issue: 07 | July -2017 www.irjet.net p-ISSN: 2395-0072
© 2017, IRJET | Impact Factor value: 5.181 | ISO 9001:2008 Certified Journal | Page 585
Fig.2. Mean S/N ratio plot for Pressure (U1-U4),
Temperature (V1-V4), L:C (X1-X4), Stoi.Ratio (Y1-Y4)
Based on the result available from the Table 3, It was
concluded that the design parameter such as, landing to
channel width ratio of interdigitatedflowchannelhaving-1:2
as X2,and the operating parameters like pressure -2.5baras
U4, temperature - 343 K as V4, Stoichiometric ratio of inlet
mass flow rate - 4 as Y3 were the optimum parameters to
show the better PEMFC performance. The optimization
results of various parameters were based on S/N ratios and
the significance of each factor by ranking them according to
their performance. Delta value of each factoravailable onthe
Minitab 17 software itself was shown in Table 3.
Table 3. Mean S/N ratios, Delta and Rank for each level of
factors
Factors
Leve
l 1
Leve
l 2
Leve
l 3
Leve
l 4
Delt
a
Ran
k
Landing to
Channel
width (L:C)
-
15.5
1
-
14.8
6
-
16.8
7
-
15.0
2
2.01 2
Pressure
(bar)
-
15.9
1
-
15.6
1
-
15.4
6
-
15.2
8
0.63 3
Temperatur
e (K)
-
16.7
3
-
15.8
4
-
15.1
2
-
14.5
7
2.16 1
Stoi.Ratio
-
15.5
7
-
15.5
9
-
15.5
4
-
15.5
7
0.04 4
The factor with highest delta value indicates higher
significance factor. It was found that the operating pressure
was the predominant factor affecting the performance and it
has been contributed as 45.24 % of overall performance of
PEMFC. The other parameters were also influencing the
performance to a considerable extent such as, landing to
channel width ratio (L:C) of interdigitated flow channel was
to be 19.02%, stoichiometricratio of inlet massflowratewas
10.54% and operating temperature was to be 0.97%
respectively. The combined effect of combinationofpressure
with temperature and pressure with L:C has shown 0.11 %
and 16.95 % respectively contributing to peak power
performance of the PEMFC. Also the percentagecontribution
of individual parameters, P-test and F-test on the
interdigitated flow fields for the performance of PEMFC has
been shown in the Table 4.
Table 4.The percentage contribution of individual
parameters of interdigitated flow channel
Factors
D
O
F
Sum of
square
s
Varian
ce
F-test
P-
Tes
t
Contri
bution
(%)
Pressure
2 0.0003
64
0.0001
8
910.0
8
0.0
76
45.24
Tempera
ture
2 0.0008
08
0.0004
0
2020.
96
0.0
18
0.97
Stoichio
metric
ratio
2 0.0000
14
0.0000
1
35.55 0.1
1
10.54
L:C
3 0.0031
89
0.0010
6
2659.
64
0 19.02
Pressure
&
Tempera
ture
1 0.0000
23
0.0000
2
58.26 0.0
17
0.11
Pressure
& L:C
3 0.0000
08
0 6.28 0.1
4
16.95
Error
2 0.0000
01
0 7.17
Total
15 0.0077
08
0.0016
82167
5684.
63
0.3
61
100
4. CONCLUSIONS
The maximum power density for optimizing the four
different parameters on 49 cm2 active area of interdigitated
flow channel of PEMFC usingCFD Fluent software was found
to be 0.203 W/cm2 from L:C-1:2 with 2 bar operating
pressure, 343 K temperature and 3 stoichiometric ratio of
inlet reactant gases and R2 value was arrived 99.9 %. The
maximum to minimum percentage of power deviation in 49
cm2 interdigitated flow channel has found to be 59.8. The
performance of PEMFC with various design and operating
parameters has been affected considerably.
REFERENCES
[1] Nicholas, S.;Siefert.; Shawn Litster.(2011).Voltage loss
and fluctuation in proton exchangemembranefuel cells:
The role of cathode channel plurality and air
stoichiometric ratio, Journalof Power Sources, 196,
1948–1954.
International Research Journal of Engineering and Technology (IRJET) e-ISSN: 2395-0056
Volume: 04 Issue: 07 | July -2017 www.irjet.net p-ISSN: 2395-0072
© 2017, IRJET | Impact Factor value: 5.181 | ISO 9001:2008 Certified Journal | Page 586
[2] Manso, A. P.;Garikano, X.;GarmendiaMujika, M.(2012).
Influence of geometric parameters of the flow fields on
the performance of a PEM fuel cell, A review
International Journal of Hydrogen Energy, 37,15256-
15287.
[3] Lakshminarayanan V, Karthikeyan P, Kiran Kumar DS
and Dhilip Kumar SM K. Numerical analysis on 36cm2
PEM fuel cell for performance enhancement, ARPN
Journal of Engineering and Applied Sciences, 2016, 11,
no. 2.
[4] Guvelioglu, GH & Stenger, HG 2005, 'Computational
fluid dynamics modeling of polymer electrolyte
membrane fuel cells', Journal ofPowerSources,vol.147,
no. 1, pp. 95-106.
[5] Ahmed, DH & Sung, HJ 2006, 'Effects of channel
geometrical configurationandshoulderwidthonPEMFC
performance at high current density', Journal of Power
Sources, vol. 162, no. 1, pp. 327-339.
[6] Lakshminarayanan V & Karthikeyan P. Optimization of
Flow Channel Design and Operating Parameters on
Proton Exchange Membrane Fuel Cell Using Mat lab.
Periodica Polytechnica Chemical Engineering.Budapest
Univ Technology Economics. 2016, 60, 3; 173-180.
[7] Grujicic, M & Chittajallu, K 2004, 'Design and
optimization of polymer electrolyte membrane (PEM)
fuel cells', Applied surface science, vol.227,no.1,pp.56-
72.
[8] Karthikeyan, P, Muthukumar, M, Shanmugam, SV,
Kumar, PP, Murali, S & Kumar, AS 2013, 'Optimizationof
Operating and Design Parameters on Proton Exchange
Membrane Fuel Cell by using Taguchi method',Procedia
Engineering, vol. 64, pp. 409-418.
[9] Wu, S-J, Shiah, S-W & Yu, W-L 2009, 'Parametric analysis
of proton exchange membrane fuel cell performance by
using the Taguchi method and a neural network',
Renewable Energy, vol. 34, no. 1, pp. 135-144.
[10] Yan WM, Chen CY, Mei SC, Soong CY & Chen F. 'Effects
of operating conditions on cell performance of PEM fuel
cells with conventional or interdigitated flow field,
Journal of Power Sources,2006, 162, no. 2; 1157-1164.

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Taguchi Method of Optimization Performed on 49 cm2 Active Area on Interdigitated Flow Channel of PEMFC

  • 1. International Research Journal of Engineering and Technology (IRJET) e-ISSN: 2395-0056 Volume: 04 Issue: 07 | July -2017 www.irjet.net p-ISSN: 2395-0072 © 2017, IRJET | Impact Factor value: 5.181 | ISO 9001:2008 Certified Journal | Page 582 Taguchi method of optimization performed on 49 cm2 active area on interdigitated flow channel of PEMFC Dr V LAKSHMINARAYANAN Department of Mechanical Engineering, B V Raju Institute of Technology, Narsapur, Telangana, India - 502313 ---------------------------------------------------------------------***--------------------------------------------------------------------- Abstract - In this paper, optimization of operating and design parameters on interdigitatedflowchannelwith49cm2 effective area of the Proton Exchange Membrane Fuel Cell (PEMFC) was considered numerically using CFD and Minitab 17 software. The factors considered for the optimization was landing to channel width ratios (L: C) -1:1, 1:2, 2:1 and 2:2, operating pressure (1, 1.5, 2 and 2.5 bar), temperature (313, 323, 333 and 343 K), anode and cathode reactants as stoichiometric ratios (S/F) of 3, 3.5, 4 and 4.5. Based on the optimization study, the L:C-1:2 has maximum influence on PEMFC performance and square of response factor (R2) was achieved by Taguchi method as 99.9 %. Key Words: Interdigitated flow channel;CFD;Optimization; Design parameters; operating parameters. 1. INTRODUCTION The Proton Exchange Membrane Fuel Cell (PEMFC) is an electrochemical device, which is convertingchemical energy of fuels (hydrogen and oxygen) directly into electricity without any intermediate stage like classical combustion of two and four stroke engine. The PEMFC performance depends on the channel depth and width, flow channel design, number of flow path, cross section of the flow channel, operating pressure, temperature,relativehumidity, mass flow rate of the reactant gases and stoichiometricratio of the reactants. It is being developed for commercial applications in the field of transportation and back-up power. One of the main advantages of the fuel cells is the negligible emission of pollutants, such as SOx, NOx, particulates. It is Eco-friendlypowersourcewhichissuitable for powering both portable devices and mobile application due to their high energy density and lower operating temperature range [1 & 2].The effect of the various parameters like landing width to channel width of (L: C) 1:1, 1:2 and 2:2 Multi pass serpentine flow channel PEMFC with 36 cm2 (6cm x 6cm) active area was analyzednumericallyby Lakshminarayanan et al [3].The results revealed that the maximum power densities were obtained 0.658W/cm2 for the L: C of 1:1. Guvelioglu & Stenger [4] studied a CFD model to analyse the effects of channel size, electrode porosity and reactant humidification on the performance of PEMFC. The results revealed thatsmaller sizedchannelswererequiredto obtain the higher current densities,althoughlargerchannels were satisfactory to produce moderate current densities. The effect of the relative humidity of the anode gas stream was found to be the important factor for affecting the performance of the PEMFC. Ahmed & Sung [5] investigated the performance of PEMFCs with different flow fields like a rectangular, trapezoidal and parallelogram using CFD. The results showed that a rectangular flow field gave higher cell voltages compared with parallelogram and trapezoidal flowfields.However, the trapezoidal flow field helped reactant diffusion, uniform reactant flow and current density circulations over the reacting area, results in lower cathode over potential of the fuel cell. The performance enhancement of the combined effect of design and operating parametersofbothserpentine and interdigitated flow channel with 25 cm2 active area of PEM fuel cell with four different parameters using optimization technique and CFD carried out by Lakshminarayanan and Karthikeyan [6]. The results revealed that the peak power density of interdigitated flow channel with landing to channel width (L:C)1:2 showed better than the serpentineflowchannel withL:C-1:2.Grujicic and Chittajallu [7] have studied the performance of PEMFC by using a single-phase two-dimensional electrochemical model. The model was coupled with a nonlinearconstrained optimization algorithm to define an optimum design of the fuel cell with respect to the operation and the geometrical parameters of the cathode. The results of the optimization analysis showed that higher current densities at a constant cell voltage were obtained as the inlet air pressure. On the other hand, the statistical sensitivityanalysisresultsshowed that the equilibriumcathode/membranepotential difference has the largest effect on the predicted polarization curve of the PEMFC. Karthikeyan et al. [8] studiedtheperformance of single channel PEMFC using Taguchi method for various operating and design parameters like cell temperature,back pressure, anode and cathode inlet velocities, porosity and thickness of the gas diffusion layer, cathode water mass fraction, flow channel dimensions, rib width and porous electrode thickness. The results revealed that the back pressure showed maximum effect and rib width had less effect on the PEMFC performance in the first stage. Further, enhancement of power density by 3% when selected factors in the second stage of fine-tuned optimization has been carried out. Wu et al. [9] integrated the neural network and Taguchi technique for parametric analysis with various parameters like operating temperatures, cathode and anode humidification temperature, operating pressure, and reactant flow rate for the enhancement of PEMFC
  • 2. International Research Journal of Engineering and Technology (IRJET) e-ISSN: 2395-0056 Volume: 04 Issue: 07 | July -2017 www.irjet.net p-ISSN: 2395-0072 © 2017, IRJET | Impact Factor value: 5.181 | ISO 9001:2008 Certified Journal | Page 583 performance. The results indicated that among the various parameters, temperature and pressure were the major factors to influence the PEMFC performance. The effects of interdigitated flow channel withtraditional flowchannel,the effects of the flow area ratio and the baffle-blocked position of the interdigitated flow field on the performanceofPEMFC were examined experimentally by Yan et al [10]. The results concluded that, the cell performance can be enhanced with an increased inlet flow rate of reactant and cathode humidification temperature. The interdigitated flow fields have better performancethanconventional flowfielddesign. Also the results showed that the interdigitated flow fieldhas larger limiting current density, and the power output was about 1.4 times than the conventional flow field. It is clearly indicated that immediateattentionisrequiredforoptimizing the simultaneous influence of operating and design parameters for the performance of the PEMFC. Hence this paper has a detailed study about the optimization of operating parameters like operating pressure, temperature, stoichiometric ratio of inlet reactant mass flow rate and design parameter like various rib width to channel width (L:C)-1:1, 1:2, 2:1& 2:2 on interdigitated flow channel of 49 cm2 active area of PEMFC are to be studied and compared the influence of individual parameters contribution on the total performance of PEMFC. 2. MODEL DEVELOPMENT The modeling was done by creating all individual partsofthe PEMFC and the dimensions of individual parts such as the anodeandcathodeGDL,solidpolymerelectrolytemembrane, the anode and cathode catalyst layers as shown in the Table 1. Three dimensional (3-D) PEMFC modelwithinterdigitated flow channel of various landing width to channel width ratio (L: C) -1:1, 1:2, 2:1 and 2:2 was created by Creo Parametric 2.0 and meshed by using ICEM 14.5 (a module of Ansys 14.5) as shown in Fig.1. Table -1: Dimensions and Zone type of parts assigning of fuel cell (a) (b) (c) (d) Fig -1: Various landing to channel width (L: C) (a) 1:1 (b) 1:2 (c) 2:1 and (d) 2:2 of interdigitated flow channel of 49 cm2 active area of PEMFC S. No Part Name Wid th (mm ) Len gth (mm ) Thickn ess (mm) Zone type 1 Anode & Cathode Flow channel 70 70 10 Solid 2 Anode & Cathode catalyst 0.08 Fluid 3 Membrane 0.127 Fluid 4 GDL anode & cathode 0.3 Fluid
  • 3. International Research Journal of Engineering and Technology (IRJET) e-ISSN: 2395-0056 Volume: 04 Issue: 07 | July -2017 www.irjet.net p-ISSN: 2395-0072 © 2017, IRJET | Impact Factor value: 5.181 | ISO 9001:2008 Certified Journal | Page 584 After geometry modeling, thenextstepwasdiscretization of PEMFC donebyICEMsoftware.TheCartesiangridmeshing method was used, which is used in the formation of hexahedral mesh to attain accurate results. Split block method was used forblocking and bodyfittedmeshwasused for meshing. The projection factor was set to 1and the projection factor decides how closely the edges of the mesh match up with the grid. The simulation of PEMFC was solved by simultaneous equations like conservation of mass, momentum, energy, species concentration, butler–Volmerequation,Jouleheating reaction and the Nernst equation to obtain reaction kinetics. The model used to consider the system as 3-D, steady state and inlet gases as ideal condition, system as an isothermal and flow aslaminar, fluid as incompressible,thermophysical properties as constant and the porous GDL, two catalyst layers and the membrane as an isotropic. A control volume approach based on commercial solver FLUENT 14.5 was used to solve the various governing equations. Three-dimensional, double precision and serial processing were used for this model. The species concentration on anode side of H2, O2, and H2O were set to 0.8, 0, and 0.2 respectively. Similarly, on the cathode side were set as 0, 0.2 and 0.1 respectively. The porosity at anode and cathodesidewas 0.5. Open circuit voltage wassetat0.95 V on the cathode and the anode was grounded. The cathode voltage has been varied from 0.05 V to 0.95Vusedforsolving kinetics reaction in order to get the current flux density H2, O2, and H2O fractions along with the flow field design. Multigrid settings were modified as F-Cycle for all the equations and entered termination restriction value was set as 0.001 for H2, O2, H2O and water saturation. The Anode and Cathode reference currentdensitywassettobe10000A/cm2 and 20 A/cm2 respectively 0.1 kmol/m3 wasset to anodeand cathode reference concentration, Anode and cathode exchange coefficient was settobe2.TheReferencediffusivity of H2, O2 and H2O was set to as 3E-5. The electric and proton potential values were set at 0.0001. Stabilization method BCGSTAB was selected for H2, O2, H2O, water saturation, electric and proton potential. Taguchi method of optimization has been usedtofindout the most optimum combination among the various input parameters which would result in getting the maximum possible output whichcausesthe performanceenhancement of PEMFC. The factorsconsidered for the analysis were rib to channel ratios on interdigitated flow field design (L: C-1:1, 1:2, 2:1 and 2:2), pressure(1,1.5, 2 and2.5bar),temperature (313, 323, 333 and 343 K), anode and cathode reactants as stoichiometric ratios (S/F) of 3, 3.5, 4 and 4.5. The standard L16 orthogonal array with 4-level and 4factorswasusedand the parameters were considered as low, high and medium range values. When this orthogonal array was used, significance of factors and optimum combination can be found in 16 runs itself. The theoretical value of hydrogen in the anode side was 4.33E-07 kg/s and oxygen in the cathode side was 3.33E-06 kg/s. 3. RESULTS AND DISCUSSION As per L16 orthogonal array,theinputsof16combination of various parameters were given to the Ansys CFD Fluent analysis software and having all other parameters constant. The obtained power densities from analysis software for all 16 runs were fed in to the Minitab 17 software. The corresponding Signal/Noise (S/N) ratios for all 16 combinations were found from Minitab 17 software itself as shown in the Table 2. The landing to channel width ratio of 1:1 for interdigitated flow field has shown maximum power densities of 0.195 W/cm2 and minimum power densities of 0.142 W/cm2respectively. Similarly for L:C of 1:2 and 2:1 having maximum power density of 0.203W/cm2 and 0.161 W/cm2 respectively. The minimum power densities for the sameL:C ratios have 0.157W/cm2 and 0.127 W/cm2 respectively. For the landing to channel width ratio of 2:2 has shown maximum power density of 0.189 W/cm2andpowerdensity of 0.159 W/cm2. The optimizationwasperformedfor“Larger the Better” type of Taguchi method since power output of PEMFC must be maximized. The S/N ratio plot for the same were obtained using Minitab 17 software and the corresponding maximum S/N ratio givesbetterperformance as analyzed based on larger the better as shown in the Fig.2. Table -2: Factors, levels, power density and S/N ratio for 16 runs of optimization Ru n R:C Pr ess ure Tempe rature Stoi. Rati o Power Density (W/cm2) S/N Ratio 1 1x 1 1 313 3 0.141 -16.9838 2 1.5 323 3.5 0.159 -15.9262 3 2 333 4 0.179 -14.9638 4 2.5 343 4.5 0.195 -14.1839 5 1x 2 1 323 4 0.169 -15.4043 6 1.5 313 4.5 0.157 -16.0978 7 2 343 3 0.203 -13.8341 8 2.5 333 3.5 0.197 -14.1025 9 2x 1 1 333 4.5 0.144 -16.8392 10 1.5 343 4 0.161 -15.8525 11 2 313 3.5 0.127 -17.8901 12 2.5 323 3 0.143 -16.8818 13 2x 2 1 343 3.5 0.189 -14.4271 14 1.5 333 3 0.187 -14.5604 15 2 323 4.5 0.175 -15.1536 16 2.5 313 4 0.159 -15.9489 Average S/N Ratio -15.566
  • 4. International Research Journal of Engineering and Technology (IRJET) e-ISSN: 2395-0056 Volume: 04 Issue: 07 | July -2017 www.irjet.net p-ISSN: 2395-0072 © 2017, IRJET | Impact Factor value: 5.181 | ISO 9001:2008 Certified Journal | Page 585 Fig.2. Mean S/N ratio plot for Pressure (U1-U4), Temperature (V1-V4), L:C (X1-X4), Stoi.Ratio (Y1-Y4) Based on the result available from the Table 3, It was concluded that the design parameter such as, landing to channel width ratio of interdigitatedflowchannelhaving-1:2 as X2,and the operating parameters like pressure -2.5baras U4, temperature - 343 K as V4, Stoichiometric ratio of inlet mass flow rate - 4 as Y3 were the optimum parameters to show the better PEMFC performance. The optimization results of various parameters were based on S/N ratios and the significance of each factor by ranking them according to their performance. Delta value of each factoravailable onthe Minitab 17 software itself was shown in Table 3. Table 3. Mean S/N ratios, Delta and Rank for each level of factors Factors Leve l 1 Leve l 2 Leve l 3 Leve l 4 Delt a Ran k Landing to Channel width (L:C) - 15.5 1 - 14.8 6 - 16.8 7 - 15.0 2 2.01 2 Pressure (bar) - 15.9 1 - 15.6 1 - 15.4 6 - 15.2 8 0.63 3 Temperatur e (K) - 16.7 3 - 15.8 4 - 15.1 2 - 14.5 7 2.16 1 Stoi.Ratio - 15.5 7 - 15.5 9 - 15.5 4 - 15.5 7 0.04 4 The factor with highest delta value indicates higher significance factor. It was found that the operating pressure was the predominant factor affecting the performance and it has been contributed as 45.24 % of overall performance of PEMFC. The other parameters were also influencing the performance to a considerable extent such as, landing to channel width ratio (L:C) of interdigitated flow channel was to be 19.02%, stoichiometricratio of inlet massflowratewas 10.54% and operating temperature was to be 0.97% respectively. The combined effect of combinationofpressure with temperature and pressure with L:C has shown 0.11 % and 16.95 % respectively contributing to peak power performance of the PEMFC. Also the percentagecontribution of individual parameters, P-test and F-test on the interdigitated flow fields for the performance of PEMFC has been shown in the Table 4. Table 4.The percentage contribution of individual parameters of interdigitated flow channel Factors D O F Sum of square s Varian ce F-test P- Tes t Contri bution (%) Pressure 2 0.0003 64 0.0001 8 910.0 8 0.0 76 45.24 Tempera ture 2 0.0008 08 0.0004 0 2020. 96 0.0 18 0.97 Stoichio metric ratio 2 0.0000 14 0.0000 1 35.55 0.1 1 10.54 L:C 3 0.0031 89 0.0010 6 2659. 64 0 19.02 Pressure & Tempera ture 1 0.0000 23 0.0000 2 58.26 0.0 17 0.11 Pressure & L:C 3 0.0000 08 0 6.28 0.1 4 16.95 Error 2 0.0000 01 0 7.17 Total 15 0.0077 08 0.0016 82167 5684. 63 0.3 61 100 4. CONCLUSIONS The maximum power density for optimizing the four different parameters on 49 cm2 active area of interdigitated flow channel of PEMFC usingCFD Fluent software was found to be 0.203 W/cm2 from L:C-1:2 with 2 bar operating pressure, 343 K temperature and 3 stoichiometric ratio of inlet reactant gases and R2 value was arrived 99.9 %. The maximum to minimum percentage of power deviation in 49 cm2 interdigitated flow channel has found to be 59.8. The performance of PEMFC with various design and operating parameters has been affected considerably. REFERENCES [1] Nicholas, S.;Siefert.; Shawn Litster.(2011).Voltage loss and fluctuation in proton exchangemembranefuel cells: The role of cathode channel plurality and air stoichiometric ratio, Journalof Power Sources, 196, 1948–1954.
  • 5. International Research Journal of Engineering and Technology (IRJET) e-ISSN: 2395-0056 Volume: 04 Issue: 07 | July -2017 www.irjet.net p-ISSN: 2395-0072 © 2017, IRJET | Impact Factor value: 5.181 | ISO 9001:2008 Certified Journal | Page 586 [2] Manso, A. P.;Garikano, X.;GarmendiaMujika, M.(2012). Influence of geometric parameters of the flow fields on the performance of a PEM fuel cell, A review International Journal of Hydrogen Energy, 37,15256- 15287. [3] Lakshminarayanan V, Karthikeyan P, Kiran Kumar DS and Dhilip Kumar SM K. Numerical analysis on 36cm2 PEM fuel cell for performance enhancement, ARPN Journal of Engineering and Applied Sciences, 2016, 11, no. 2. [4] Guvelioglu, GH & Stenger, HG 2005, 'Computational fluid dynamics modeling of polymer electrolyte membrane fuel cells', Journal ofPowerSources,vol.147, no. 1, pp. 95-106. [5] Ahmed, DH & Sung, HJ 2006, 'Effects of channel geometrical configurationandshoulderwidthonPEMFC performance at high current density', Journal of Power Sources, vol. 162, no. 1, pp. 327-339. [6] Lakshminarayanan V & Karthikeyan P. Optimization of Flow Channel Design and Operating Parameters on Proton Exchange Membrane Fuel Cell Using Mat lab. Periodica Polytechnica Chemical Engineering.Budapest Univ Technology Economics. 2016, 60, 3; 173-180. [7] Grujicic, M & Chittajallu, K 2004, 'Design and optimization of polymer electrolyte membrane (PEM) fuel cells', Applied surface science, vol.227,no.1,pp.56- 72. [8] Karthikeyan, P, Muthukumar, M, Shanmugam, SV, Kumar, PP, Murali, S & Kumar, AS 2013, 'Optimizationof Operating and Design Parameters on Proton Exchange Membrane Fuel Cell by using Taguchi method',Procedia Engineering, vol. 64, pp. 409-418. [9] Wu, S-J, Shiah, S-W & Yu, W-L 2009, 'Parametric analysis of proton exchange membrane fuel cell performance by using the Taguchi method and a neural network', Renewable Energy, vol. 34, no. 1, pp. 135-144. [10] Yan WM, Chen CY, Mei SC, Soong CY & Chen F. 'Effects of operating conditions on cell performance of PEM fuel cells with conventional or interdigitated flow field, Journal of Power Sources,2006, 162, no. 2; 1157-1164.