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International Journal of Research in Engineering and Science (IJRES)
ISSN (Online): 2320-9364, ISSN (Print): 2320-9356
www.ijres.org Volume 2 Issue 1 ǁ Jan 2014 ǁ PP.19-25
www.ijres.org 19 | Page
Spray Angle Expansion Method of a Twin-Fluid Atomizer for the
Application to CO2absorption
Jiafeng Yao1
, Michio Sadatomi1
, Akimaro Kawahara1
, Shinji Furusawa2
1
(Department of Advanced Mechanical Systems, Kumamoto University, Japan)
2
(Japan Marine United Corporation, Japan)
ABSTRACT :This paper presents the results of an experimental study for a new type twin-fluid atomizer,
which is based on a multi fluids mixer patented by Sadatomi & Kawahara (2012). This atomizer has a simple
structure and can suck water by itself without a pump by introducing pressurized air alone into an internal
mixing chamber with less energy consumption. The present study focuses on the improved design of the atomizer
for spray angle expansion and its application to CO2 absorption. Experiments relating to two angle expansion
methods (Coanda effect and propellers) were conducted, also six sizes of PET (Polyethylene Terephthalate)
propellers were tested. We found that, the atomizer with a PET propeller of 4 blades and 25 mm in diameter
showed the best spray angle expansion effect and presented a good spray quality, especially reduced the Sauter
mean diameter (d32) significantly. Finally, the mist sprayed by the optimized atomizer was applied to CO2
absorption, and experimental results showed that the mist sprayed by the optimized atomizer can significantly
decrease the CO2 concentration in a closed room.
Keywords -Atomizer, spray-angle, Coanda effect, propeller, CO2absorption
I. INTRODUCTION
Liquid atomizer has been applied extensively in our daily life, such as fire suppression, paint spraying,
humidity control, etc. In this context, several types of atomizers have been developed by Lal et al. [1], and some
makers such as HYPRO EU Ltd. [2]. Till now, all forms of pressure nozzles accomplish this by discharging the
liquid at high velocity into quiescent or relatively slow-moving air. Rotary atomizers employ a similar principle,
the liquid being ejected at high velocity from the rim of a rotating cup or disc. An alternative method of
achieving a high relative velocity between liquid and air is to expose slow-moving liquid into a high-velocity
stream of air. Devices based on this approach are usually termed air-assist, air-blast or, more generally, twin-
fluid atomizers.
There are also plenty of experimental and numerical researches that address the atomization methods of
the twin-fluid atomizers. Some employ the pressure principle, where the liquid is supplied from a pressurized
source; others use the gravity principle, where the liquid supply is located above the nozzle, invoking gravity for
the liquid flow; the siphon principle is also used in some twin-fluid atomizers, where the liquid source is self-
aspirating. Applications for this family of atomizers includes humidification, dust control, gas cooling, precision
coating and spray drying.
The purpose of the present study is to expand the spray angle of Sadatomi & Kawahara’s new type
twin-fluid atomizer [3], which had the characteristic of less energy consumption and simple structure but narrow
spray angle. In order to expand the spray angel, two methods (Coanda effect and propellers with different
material, different blade number and diameter) are tested, and the best specifications are determined.
In addition, Carbon dioxide (CO2) is the primary greenhouse gas emitted through human activities. In
2011, CO2 accounted for about 84% of all U.S. greenhouse gas emissions from human activities. Carbon
dioxide is naturally present in the atmosphere as part of the Earth's carbon cycle (the natural circulation of
carbon among the atmosphere, oceans, soil, plants, and animals). Human activities are altering the carbon
cycle—both by adding more CO2 to the atmosphere and by influencing the ability of natural sinks, like forests,
to remove CO2 from the atmosphere. While CO2 emissions come from a variety of natural sources, human-
related emissions are responsible for the increase that has occurred in the atmosphere since the industrial
revolution. In consequence, the growing awareness on the risks associated with the green-house effect caused by
CO2 motivates the researchers to develop various methods for eliminating CO2 since 1989 [4]. So, we tried to
utilize Sadatomi & Kawahara's atomizer for the absorption of CO2.
II. EXPERIMENTS AND METHODS
2.1 Principle of Sadatomi & Kawahara's atomizer
The proto type of the atomizer is shown in Fig. 1, in which pressurized air is supplied into a pipe with
an orifice in the core. From the conservation equations of mass and energy, (1) and (2).
Spray angle expansion method of a twin-fluid atomizer for the application to CO2 absorption
www.ijres.org 20 | Page
𝑃1
𝜌𝑔
+
𝑣 𝐺1
2
2𝑔
=
𝑃2
𝜌𝑔
+
𝑣 𝐺2
2
2𝑔
(1)
𝑃2 − 𝑃1 = 𝑃1 −
𝜌
2
(𝑣 𝐺2
2
− 𝑣 𝐺1
2
) (2)
Fig. 1 Principle of new-type twin-fluid atomizer patented by Sadatomi & Kawahara (2012).
The velocity of the air after passing through the orifice, vG2, becomes much higher than before vG1, so,
vG2>vG1, and the pressure there becomes much lower, P2<P1. If the pressure becomes negative, then the water
can be automatically sucked into air stream through a porous pipe. Since the air flow there is highly-turbulent
and shear flow, air and water interact each other in the internal mixing chamber of the atomizer, and a huge
number of tiny water droplet, i.e. mist is formed and discharged through the outlet port.
Based on previous studies in this series [5, 6], we can conclude the main special advantages of
Sadatomi & Kawahara’s atomizer as follows: (a) lower energy consumption. The energy is supplied only by a
compressor or blower although it is a twin-fluid atomizer, and the gas pressure needed is less than 70 kPa., quite
lower than those for other atomizers [7, 8]; (b) simple structure, which means easy to manufacture. The mixing
chamber and the orifice are easy to manufacture, and the porous pipe is a kind of common fiber material which
can be readily available; (c) mist diameters are quite small, 90% of them are less than 30 µm. That means the
atomizer can jet fine mists, which is qualified to be applied to air cooling, CO2 absorption, smoke absorption,
etc.
However, the spray angle of Sadatomi & Kawahara’s atomizer is limited by the inherent structure of
the atomizer and is not wide enough for many applications, this disadvantagewill be solved in the present study.
2.2Experimental Apparatus
The experimental apparatus for studying the sprayangle expansion is revealed in Fig. 2. In the
experiment, the volume flow rate of air and water are QG = 300 l/min, QL = 0.2 l/min. At 500 mm downward
from the atomizer nozzle, 22 test tubes each 13 mm apart in center to center distance were set in line in four
radial directions, so as to collect mist and get the radial distribution of the mist. Meanwhile, to eliminate the
introduction of water due to level difference, the water in the tank and the water suction part of the atomizer
should be on the same level. The output signals from the flow rate and pressure sensors were acquired by
computer via an A/D converter.
Fig. 2 Experimental apparatus for the test of spray performance of twin-fluid atomizer.
Spray angle expansion method of a twin-fluid atomizer for the application to CO2 absorption
www.ijres.org 21 | Page
For the droplet measurement, a digital camera (in Fig. 3) with a microscope is used, and more than a
thousand droplet diameters are tested with an image processing system. Fig. 4 shows a typical picture of water
droplets in an oil pond, which are about unity in sphericity, even in the largest 150 µm droplet [9].
Fig. 3 Drop size testing facility
Fig. 4 A typical picture of water droplets.
Drop-size distributions are often described by characteristic diameters (3) [10]:
1
a a b
i ii
ab b
i ii
n d
d
n d
 
  
  


(3)
Here,i denotes the number of droplet size range, ni is the number of droplets in the size rangei, and diis
the diameter of the size range i. Thus, for example, d10 is the arithmeticmeandiameter of all the drops in the
spray; and d32, Sauter mean diameter, is the diameter of the droplet whose ratio of volume to surface area is the
same as that of the entire spray, which is often of use in applications where the active surface or surface area is
important (e.g. air cooling, gas absorption) [11]. In the present experiments, d10 and d32 are used to identify the
spray effect of droplets.
2.3Spray-Angle Expansion Methods
Spray angle (injection angle) is an apex angle of the spray, which characteristics the shape of the drop
jet. In many cases it is necessary to predict the spray shape because it guarantees proper utilization of the jet
[12]. It is important mostly in cases in which atomizers are applied in gas absorption (e.g. CO2 capture in this
study). For Sadatomi & Kawahara’s atomizer, it is an atomizer with internal mixing chamber and a cylindroid
outlet, so spray angle is too narrow, and need to be expanded as large as possible.We developed two methods to
expand the spray angle: Coanda effect and propeller.
The Coanda effect states that a fluid or gas stream will hug a convex contour when directed at a tangent
to that surface. This was discovered in the 1930s by a Romanian named Henri-Marie Coanda [13]. What is
unusual about the Coanda effect is the fact that the fluid or gas flow is pulled so strongly by a curved surface. A
concave curve will naturally push the flow, but the fact that a convex one would react so strongly to fluid or gas
is unusual. This property is particularly relevant to aircraft design. This paper designed an outlet for the atomizer
described in Fig. 5.
Spray angle expansion method of a twin-fluid atomizer for the application to CO2 absorption
www.ijres.org 22 | Page
Fig. 5 Coanda effects of spreader utilizing.
Fig. 6 Propellers with different materials.
Table 1 Specifications of PET propellers.
PET
Propeller
Blade No. Outer Dia. Mass
- mm g
b3d15 3
15
0.113
b4d15 4 0.112
b3d25 3
25
0.321
b4d25 4 0.320
b3d35 3
35
0.636
b4d35 4 0.634
Fig. 7 Installed position of the propeller is 40 mm downward from the exit of the atomizer nozzle
Fig. 8 Six sizes of PET propellers with different outer diameters.
 16.5
 7
 87
Spray angle expansion method of a twin-fluid atomizer for the application to CO2 absorption
www.ijres.org 23 | Page
For another method, two kinds of propellers were developed like Fig. 6, which is made of PET and
brass with outer diameter of 25 mm.
Furthermore, propellers made of PET with different specifications are listed in in Table I, the name of
propeller such as b3d15 for example, stands for a PET propeller with 3 blades, and 15 mm in outer diameter.
These propellers could rotate automatically by an action of the air stream with mist.
The position of the propeller was about 40 mm downward from the exit of the atomizer nozzle as
shown in Fig. 7. Six types of PET propellers were tested as listed in Table 1 and shown in Fig. 8.
2.4CO2 absorption
As for the application of CO2 absorption, we developed a facility like a vinyl greenhouse as shown in
Fig. 9. Inside the house (2000mm high ×1200mm wide ×1200mm deep), the atomizer was set at 1800 mm in
height in the middle of the house. In the bottom space, the carbon dioxide concentration meter and a balloon
filled with CO2 gas were placed near the side walls.
In the experiment, at first, the house was filled with mist at QG = 300 l/min, QL = 0.2 l/min, and with
the propeller of PP-b4d25. After breaking the balloon with a needle, we collected the data of CO2 concentration
every 4 seconds, for 150 times.
Fig. 9 CO2 absorption method and facility.
III. RESULTS AND DISCUSSION
3.1Results of Spray-Angle Expansion
Fig. 10 shows the spay angle expansion effect with different methods, the abscissa gives out the radial
distance from the center of spray area, and the ordinate describes the mist flow rate sprayed by the atomizer. For
all cases, the flow rate decreased from center to rim, but only for the method with PET propeller, we can get a
relative uniform flow rate comparing other methods. This effect comes from the less momentum of the PET
propeller than that of brass propeller.
Fig. 10 Radial mist flow rate distribution with different spay angle expansion methods.
Fig. 11 demonstrates the experimental results of the atomizer's spray angle expansion with six sizes of
PET propellers, and the condition without a propeller. Abscissa and ordinate directions stand for the radial
distance from the center and the flow rate of the mist, respectively. We can notice that, under different
conditions, the flow rate also decreased from center to rim. When we used 15 mm diameter propeller or without
a propeller, most of the mists were distributed around the center, so the effect of expansion was not visible. For
0.0
0.1
0.2
0.3
0.4
0.5
0.6
0.7
0 10 20 30
QLCcm3
/min
r cm
Without spreader
Coanda spreader
Propeller (PET)
Propeller (brass)
Spray angle expansion method of a twin-fluid atomizer for the application to CO2 absorption
www.ijres.org 24 | Page
the 25 mm and 35 mm diameter propeller, the flow rate around the center can be reduced under 0.1 cm3
/min,
and displayed good expansion effect.
Fig. 11 Results of spray-angle expansion
Fig. 12 shows mist size distribution classified into 11 diameter ranges for different propellers and no
propeller. We find that the atomizer with b4d25 propeller shows the best atomization performance, and about
95% of the mist diameter is smaller than 30 µm.
Fig. 12 Mist diameter distribution for the atomizer with six propellers and no propeller.
Fig. 13 illustrates the Sauter mean diameter (d32) of mist for different propellers. The abscissa is the
cutting frequency (cutting times for the mist flow per second), fc, by the propeller blades determined from the
number of blades, the blade diameter and the number of rotation. Of these propellers, b4d25 propeller shows the
highest cutting frequency and the lowest d32 of about 18 µm.
Fig. 13 Comparison of Sauter mean diameter for the atomizer with different propellers.
It is worthwhile to note that, comparing to other types of propellers, b4d25 propeller can provide the
lowest flow rate as 0.08 cm3
/min within 5 mm radius, and sustained this value until about 15 cm away from the
center. That is to say, b4d25 propeller showed the best expansion effect and good spray quality.
3.2CO2 absorption effect
The experimental results of CO2 absorption effect are denoted in Fig. 14 under three conditions: air
with mist (condition 1), air with mist using b4d25 propeller (condition 2), and air alone (condition 3). X
direction expresses the time after the rupture of CO2 balloon, while Y direction is the concentration of CO2.
Spray angle expansion method of a twin-fluid atomizer for the application to CO2 absorption
www.ijres.org 25 | Page
Fig. 14 CO2 absorption effect.
It can be concluded that, the mist at conditions 1 and 2 can control the CO2 concentration
under 2400 ppm, much lower than 4200 ppm of condition 3. Though the absorption effect was similar
between conditions 2 and 1, condition 2 can spray mist with much larger angle, this is an important
advantage for absorbing CO2 if the house is wide.
IV. CONCLUSIONS
In the present study we could expand the spray-angle withtwo methods, by using Coanda effect or
inserting a propeller into the air flow with mist discharged from a new type twin-fluid atomizer invented by
Sadatomi & Kawahara. The experimental results are concluded as follows:
(1) Compared with Coanda effect, an atomizer with a propeller can jet a spray with much larger angle.
(2) Propellers made of PET material possess lower momentum, so they can expand a much larger spray angle
than that of brass.
(3) Among six PET propellers with different outer diameter, the propeller with 4 blades and 25 mm in outer
diameter (b4d25) can providesthe largest spray angle and the most uniform mist flow rate from spray center
to rim, and also, 95% of the mist diametersare smaller than 30 µm, Sauter mean diameter is only 18µm. That
means high quality of spray is generated by the atomizer with b4d25 propeller of PET material.
(4) A new application in CO2 absorption was developed. The mist sprayed by the optimizedatomizer with a large
spray angle can effectively absorb the CO2 in a closed room and reduce the CO2 concentration significantly.
V. Acknowledgements
The authors would like to express their sincerely appreciation to Mr. S. Miyagawa and S. Nakakido,
students at Kumamoto University, and Mr. E. Sakurai, working in Kawasaki Heavy Industries, for their
experimental cooperation. Financial support from Nohmi Bosai LTD. is also appreciated.
REFERENCES
[1] S. Lal, A. Kushari, M. Gupta, J.C. Kapoor and S.Maji, Experimental study of an air assisted mist generator, Experimental Thermal
and Fluid Science,34,2010, 1029-1035.
[2] HYPRO EU Ltd., http://www.hypro-eu.com/en-gb/.
[3] M. Sadatomi and A. Kawahara, Fluids mixer and fluids mixing method, Japanese Patent, 2012, No. 5103625.
[4] Y. F.Diao and X. Y.Zheng, Experimental study on capturing CO2 greenhouse gas by ammonia scrubbing, Energy Convers.
Manag., 45, 2004, 2283-2296.
[5] M. Sadatomi, F. Matsuyama, A. Kawahara and T. Fukamachi, “Development of a large-flow-rate mist generator-Prediction of
hydraulic performance”, Proc. of FEDSM2007, 5th Joint ASME/JSME Fluids Engineering, Conf. San Diego, CA, FEDSM2007-
37143, 8 pages in CD-ROM, 2007.
[6] M. Sadatomi, A. Kawahara, K. Fukamachi and S. Shikatani, Micro-bubble generation rate and bubble dissolution rate into water
by a simple multi-fluid mixer with orifice and porous tube, Experimental Thermal and Fluid Science,41, 2012, 23-30.
[7] P. Watanawanyoo, H. Mochida, T. Furukawa, M. Nakamura and H. Hirahara, Experimental study on the spray characteristics of an
air assisted atomizer with internal mixing chamber, European Journal of Scientific Research,84,2012, 507-521.
[8] PNR UK Ltd., http://www.pnr.co.uk/.
[9] M. Sadatomi, A. Kawahara, K. Fukamachi, F. Matsuyama and N. Tanaka, Development of a new large-flow-rate and efficient mist
generator, and its application to air cooling in greenhouses, Multiphase Science and Technology,22(1), 2010, 79-93.
[10] N. Ashgriz, Handbook of Atomization and Sprays-Theory and Applications (Springer New York Dordrecht Heidelberg London,
2011).
[11] A. Rawle, The basic principles of particle size analysis, An internal document in Malvern Instruments Limited, 2008.
[12] L. Bayvel and Z. Orzechowski, Liquid Atomization (Washington DC: Taylor and Francis, 1993).
[13] C.C. Hong, J.W. Choi and C.H. Ahn, A Novel In-Plane Passive Micromixer Using Coanda Effect, Micro Total Analysis Systems,
2001, 31-33.

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Spray Angle Expansion Method of a Twin-Fluid Atomizer for the Application to CO2absorption

  • 1. International Journal of Research in Engineering and Science (IJRES) ISSN (Online): 2320-9364, ISSN (Print): 2320-9356 www.ijres.org Volume 2 Issue 1 ǁ Jan 2014 ǁ PP.19-25 www.ijres.org 19 | Page Spray Angle Expansion Method of a Twin-Fluid Atomizer for the Application to CO2absorption Jiafeng Yao1 , Michio Sadatomi1 , Akimaro Kawahara1 , Shinji Furusawa2 1 (Department of Advanced Mechanical Systems, Kumamoto University, Japan) 2 (Japan Marine United Corporation, Japan) ABSTRACT :This paper presents the results of an experimental study for a new type twin-fluid atomizer, which is based on a multi fluids mixer patented by Sadatomi & Kawahara (2012). This atomizer has a simple structure and can suck water by itself without a pump by introducing pressurized air alone into an internal mixing chamber with less energy consumption. The present study focuses on the improved design of the atomizer for spray angle expansion and its application to CO2 absorption. Experiments relating to two angle expansion methods (Coanda effect and propellers) were conducted, also six sizes of PET (Polyethylene Terephthalate) propellers were tested. We found that, the atomizer with a PET propeller of 4 blades and 25 mm in diameter showed the best spray angle expansion effect and presented a good spray quality, especially reduced the Sauter mean diameter (d32) significantly. Finally, the mist sprayed by the optimized atomizer was applied to CO2 absorption, and experimental results showed that the mist sprayed by the optimized atomizer can significantly decrease the CO2 concentration in a closed room. Keywords -Atomizer, spray-angle, Coanda effect, propeller, CO2absorption I. INTRODUCTION Liquid atomizer has been applied extensively in our daily life, such as fire suppression, paint spraying, humidity control, etc. In this context, several types of atomizers have been developed by Lal et al. [1], and some makers such as HYPRO EU Ltd. [2]. Till now, all forms of pressure nozzles accomplish this by discharging the liquid at high velocity into quiescent or relatively slow-moving air. Rotary atomizers employ a similar principle, the liquid being ejected at high velocity from the rim of a rotating cup or disc. An alternative method of achieving a high relative velocity between liquid and air is to expose slow-moving liquid into a high-velocity stream of air. Devices based on this approach are usually termed air-assist, air-blast or, more generally, twin- fluid atomizers. There are also plenty of experimental and numerical researches that address the atomization methods of the twin-fluid atomizers. Some employ the pressure principle, where the liquid is supplied from a pressurized source; others use the gravity principle, where the liquid supply is located above the nozzle, invoking gravity for the liquid flow; the siphon principle is also used in some twin-fluid atomizers, where the liquid source is self- aspirating. Applications for this family of atomizers includes humidification, dust control, gas cooling, precision coating and spray drying. The purpose of the present study is to expand the spray angle of Sadatomi & Kawahara’s new type twin-fluid atomizer [3], which had the characteristic of less energy consumption and simple structure but narrow spray angle. In order to expand the spray angel, two methods (Coanda effect and propellers with different material, different blade number and diameter) are tested, and the best specifications are determined. In addition, Carbon dioxide (CO2) is the primary greenhouse gas emitted through human activities. In 2011, CO2 accounted for about 84% of all U.S. greenhouse gas emissions from human activities. Carbon dioxide is naturally present in the atmosphere as part of the Earth's carbon cycle (the natural circulation of carbon among the atmosphere, oceans, soil, plants, and animals). Human activities are altering the carbon cycle—both by adding more CO2 to the atmosphere and by influencing the ability of natural sinks, like forests, to remove CO2 from the atmosphere. While CO2 emissions come from a variety of natural sources, human- related emissions are responsible for the increase that has occurred in the atmosphere since the industrial revolution. In consequence, the growing awareness on the risks associated with the green-house effect caused by CO2 motivates the researchers to develop various methods for eliminating CO2 since 1989 [4]. So, we tried to utilize Sadatomi & Kawahara's atomizer for the absorption of CO2. II. EXPERIMENTS AND METHODS 2.1 Principle of Sadatomi & Kawahara's atomizer The proto type of the atomizer is shown in Fig. 1, in which pressurized air is supplied into a pipe with an orifice in the core. From the conservation equations of mass and energy, (1) and (2).
  • 2. Spray angle expansion method of a twin-fluid atomizer for the application to CO2 absorption www.ijres.org 20 | Page 𝑃1 𝜌𝑔 + 𝑣 𝐺1 2 2𝑔 = 𝑃2 𝜌𝑔 + 𝑣 𝐺2 2 2𝑔 (1) 𝑃2 − 𝑃1 = 𝑃1 − 𝜌 2 (𝑣 𝐺2 2 − 𝑣 𝐺1 2 ) (2) Fig. 1 Principle of new-type twin-fluid atomizer patented by Sadatomi & Kawahara (2012). The velocity of the air after passing through the orifice, vG2, becomes much higher than before vG1, so, vG2>vG1, and the pressure there becomes much lower, P2<P1. If the pressure becomes negative, then the water can be automatically sucked into air stream through a porous pipe. Since the air flow there is highly-turbulent and shear flow, air and water interact each other in the internal mixing chamber of the atomizer, and a huge number of tiny water droplet, i.e. mist is formed and discharged through the outlet port. Based on previous studies in this series [5, 6], we can conclude the main special advantages of Sadatomi & Kawahara’s atomizer as follows: (a) lower energy consumption. The energy is supplied only by a compressor or blower although it is a twin-fluid atomizer, and the gas pressure needed is less than 70 kPa., quite lower than those for other atomizers [7, 8]; (b) simple structure, which means easy to manufacture. The mixing chamber and the orifice are easy to manufacture, and the porous pipe is a kind of common fiber material which can be readily available; (c) mist diameters are quite small, 90% of them are less than 30 µm. That means the atomizer can jet fine mists, which is qualified to be applied to air cooling, CO2 absorption, smoke absorption, etc. However, the spray angle of Sadatomi & Kawahara’s atomizer is limited by the inherent structure of the atomizer and is not wide enough for many applications, this disadvantagewill be solved in the present study. 2.2Experimental Apparatus The experimental apparatus for studying the sprayangle expansion is revealed in Fig. 2. In the experiment, the volume flow rate of air and water are QG = 300 l/min, QL = 0.2 l/min. At 500 mm downward from the atomizer nozzle, 22 test tubes each 13 mm apart in center to center distance were set in line in four radial directions, so as to collect mist and get the radial distribution of the mist. Meanwhile, to eliminate the introduction of water due to level difference, the water in the tank and the water suction part of the atomizer should be on the same level. The output signals from the flow rate and pressure sensors were acquired by computer via an A/D converter. Fig. 2 Experimental apparatus for the test of spray performance of twin-fluid atomizer.
  • 3. Spray angle expansion method of a twin-fluid atomizer for the application to CO2 absorption www.ijres.org 21 | Page For the droplet measurement, a digital camera (in Fig. 3) with a microscope is used, and more than a thousand droplet diameters are tested with an image processing system. Fig. 4 shows a typical picture of water droplets in an oil pond, which are about unity in sphericity, even in the largest 150 µm droplet [9]. Fig. 3 Drop size testing facility Fig. 4 A typical picture of water droplets. Drop-size distributions are often described by characteristic diameters (3) [10]: 1 a a b i ii ab b i ii n d d n d           (3) Here,i denotes the number of droplet size range, ni is the number of droplets in the size rangei, and diis the diameter of the size range i. Thus, for example, d10 is the arithmeticmeandiameter of all the drops in the spray; and d32, Sauter mean diameter, is the diameter of the droplet whose ratio of volume to surface area is the same as that of the entire spray, which is often of use in applications where the active surface or surface area is important (e.g. air cooling, gas absorption) [11]. In the present experiments, d10 and d32 are used to identify the spray effect of droplets. 2.3Spray-Angle Expansion Methods Spray angle (injection angle) is an apex angle of the spray, which characteristics the shape of the drop jet. In many cases it is necessary to predict the spray shape because it guarantees proper utilization of the jet [12]. It is important mostly in cases in which atomizers are applied in gas absorption (e.g. CO2 capture in this study). For Sadatomi & Kawahara’s atomizer, it is an atomizer with internal mixing chamber and a cylindroid outlet, so spray angle is too narrow, and need to be expanded as large as possible.We developed two methods to expand the spray angle: Coanda effect and propeller. The Coanda effect states that a fluid or gas stream will hug a convex contour when directed at a tangent to that surface. This was discovered in the 1930s by a Romanian named Henri-Marie Coanda [13]. What is unusual about the Coanda effect is the fact that the fluid or gas flow is pulled so strongly by a curved surface. A concave curve will naturally push the flow, but the fact that a convex one would react so strongly to fluid or gas is unusual. This property is particularly relevant to aircraft design. This paper designed an outlet for the atomizer described in Fig. 5.
  • 4. Spray angle expansion method of a twin-fluid atomizer for the application to CO2 absorption www.ijres.org 22 | Page Fig. 5 Coanda effects of spreader utilizing. Fig. 6 Propellers with different materials. Table 1 Specifications of PET propellers. PET Propeller Blade No. Outer Dia. Mass - mm g b3d15 3 15 0.113 b4d15 4 0.112 b3d25 3 25 0.321 b4d25 4 0.320 b3d35 3 35 0.636 b4d35 4 0.634 Fig. 7 Installed position of the propeller is 40 mm downward from the exit of the atomizer nozzle Fig. 8 Six sizes of PET propellers with different outer diameters.  16.5  7  87
  • 5. Spray angle expansion method of a twin-fluid atomizer for the application to CO2 absorption www.ijres.org 23 | Page For another method, two kinds of propellers were developed like Fig. 6, which is made of PET and brass with outer diameter of 25 mm. Furthermore, propellers made of PET with different specifications are listed in in Table I, the name of propeller such as b3d15 for example, stands for a PET propeller with 3 blades, and 15 mm in outer diameter. These propellers could rotate automatically by an action of the air stream with mist. The position of the propeller was about 40 mm downward from the exit of the atomizer nozzle as shown in Fig. 7. Six types of PET propellers were tested as listed in Table 1 and shown in Fig. 8. 2.4CO2 absorption As for the application of CO2 absorption, we developed a facility like a vinyl greenhouse as shown in Fig. 9. Inside the house (2000mm high ×1200mm wide ×1200mm deep), the atomizer was set at 1800 mm in height in the middle of the house. In the bottom space, the carbon dioxide concentration meter and a balloon filled with CO2 gas were placed near the side walls. In the experiment, at first, the house was filled with mist at QG = 300 l/min, QL = 0.2 l/min, and with the propeller of PP-b4d25. After breaking the balloon with a needle, we collected the data of CO2 concentration every 4 seconds, for 150 times. Fig. 9 CO2 absorption method and facility. III. RESULTS AND DISCUSSION 3.1Results of Spray-Angle Expansion Fig. 10 shows the spay angle expansion effect with different methods, the abscissa gives out the radial distance from the center of spray area, and the ordinate describes the mist flow rate sprayed by the atomizer. For all cases, the flow rate decreased from center to rim, but only for the method with PET propeller, we can get a relative uniform flow rate comparing other methods. This effect comes from the less momentum of the PET propeller than that of brass propeller. Fig. 10 Radial mist flow rate distribution with different spay angle expansion methods. Fig. 11 demonstrates the experimental results of the atomizer's spray angle expansion with six sizes of PET propellers, and the condition without a propeller. Abscissa and ordinate directions stand for the radial distance from the center and the flow rate of the mist, respectively. We can notice that, under different conditions, the flow rate also decreased from center to rim. When we used 15 mm diameter propeller or without a propeller, most of the mists were distributed around the center, so the effect of expansion was not visible. For 0.0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0 10 20 30 QLCcm3 /min r cm Without spreader Coanda spreader Propeller (PET) Propeller (brass)
  • 6. Spray angle expansion method of a twin-fluid atomizer for the application to CO2 absorption www.ijres.org 24 | Page the 25 mm and 35 mm diameter propeller, the flow rate around the center can be reduced under 0.1 cm3 /min, and displayed good expansion effect. Fig. 11 Results of spray-angle expansion Fig. 12 shows mist size distribution classified into 11 diameter ranges for different propellers and no propeller. We find that the atomizer with b4d25 propeller shows the best atomization performance, and about 95% of the mist diameter is smaller than 30 µm. Fig. 12 Mist diameter distribution for the atomizer with six propellers and no propeller. Fig. 13 illustrates the Sauter mean diameter (d32) of mist for different propellers. The abscissa is the cutting frequency (cutting times for the mist flow per second), fc, by the propeller blades determined from the number of blades, the blade diameter and the number of rotation. Of these propellers, b4d25 propeller shows the highest cutting frequency and the lowest d32 of about 18 µm. Fig. 13 Comparison of Sauter mean diameter for the atomizer with different propellers. It is worthwhile to note that, comparing to other types of propellers, b4d25 propeller can provide the lowest flow rate as 0.08 cm3 /min within 5 mm radius, and sustained this value until about 15 cm away from the center. That is to say, b4d25 propeller showed the best expansion effect and good spray quality. 3.2CO2 absorption effect The experimental results of CO2 absorption effect are denoted in Fig. 14 under three conditions: air with mist (condition 1), air with mist using b4d25 propeller (condition 2), and air alone (condition 3). X direction expresses the time after the rupture of CO2 balloon, while Y direction is the concentration of CO2.
  • 7. Spray angle expansion method of a twin-fluid atomizer for the application to CO2 absorption www.ijres.org 25 | Page Fig. 14 CO2 absorption effect. It can be concluded that, the mist at conditions 1 and 2 can control the CO2 concentration under 2400 ppm, much lower than 4200 ppm of condition 3. Though the absorption effect was similar between conditions 2 and 1, condition 2 can spray mist with much larger angle, this is an important advantage for absorbing CO2 if the house is wide. IV. CONCLUSIONS In the present study we could expand the spray-angle withtwo methods, by using Coanda effect or inserting a propeller into the air flow with mist discharged from a new type twin-fluid atomizer invented by Sadatomi & Kawahara. The experimental results are concluded as follows: (1) Compared with Coanda effect, an atomizer with a propeller can jet a spray with much larger angle. (2) Propellers made of PET material possess lower momentum, so they can expand a much larger spray angle than that of brass. (3) Among six PET propellers with different outer diameter, the propeller with 4 blades and 25 mm in outer diameter (b4d25) can providesthe largest spray angle and the most uniform mist flow rate from spray center to rim, and also, 95% of the mist diametersare smaller than 30 µm, Sauter mean diameter is only 18µm. That means high quality of spray is generated by the atomizer with b4d25 propeller of PET material. (4) A new application in CO2 absorption was developed. The mist sprayed by the optimizedatomizer with a large spray angle can effectively absorb the CO2 in a closed room and reduce the CO2 concentration significantly. V. Acknowledgements The authors would like to express their sincerely appreciation to Mr. S. Miyagawa and S. Nakakido, students at Kumamoto University, and Mr. E. Sakurai, working in Kawasaki Heavy Industries, for their experimental cooperation. Financial support from Nohmi Bosai LTD. is also appreciated. REFERENCES [1] S. Lal, A. Kushari, M. Gupta, J.C. Kapoor and S.Maji, Experimental study of an air assisted mist generator, Experimental Thermal and Fluid Science,34,2010, 1029-1035. [2] HYPRO EU Ltd., http://www.hypro-eu.com/en-gb/. [3] M. Sadatomi and A. Kawahara, Fluids mixer and fluids mixing method, Japanese Patent, 2012, No. 5103625. [4] Y. F.Diao and X. Y.Zheng, Experimental study on capturing CO2 greenhouse gas by ammonia scrubbing, Energy Convers. Manag., 45, 2004, 2283-2296. [5] M. Sadatomi, F. Matsuyama, A. Kawahara and T. Fukamachi, “Development of a large-flow-rate mist generator-Prediction of hydraulic performance”, Proc. of FEDSM2007, 5th Joint ASME/JSME Fluids Engineering, Conf. San Diego, CA, FEDSM2007- 37143, 8 pages in CD-ROM, 2007. [6] M. Sadatomi, A. Kawahara, K. Fukamachi and S. Shikatani, Micro-bubble generation rate and bubble dissolution rate into water by a simple multi-fluid mixer with orifice and porous tube, Experimental Thermal and Fluid Science,41, 2012, 23-30. [7] P. Watanawanyoo, H. Mochida, T. Furukawa, M. Nakamura and H. Hirahara, Experimental study on the spray characteristics of an air assisted atomizer with internal mixing chamber, European Journal of Scientific Research,84,2012, 507-521. [8] PNR UK Ltd., http://www.pnr.co.uk/. [9] M. Sadatomi, A. Kawahara, K. Fukamachi, F. Matsuyama and N. Tanaka, Development of a new large-flow-rate and efficient mist generator, and its application to air cooling in greenhouses, Multiphase Science and Technology,22(1), 2010, 79-93. [10] N. Ashgriz, Handbook of Atomization and Sprays-Theory and Applications (Springer New York Dordrecht Heidelberg London, 2011). [11] A. Rawle, The basic principles of particle size analysis, An internal document in Malvern Instruments Limited, 2008. [12] L. Bayvel and Z. Orzechowski, Liquid Atomization (Washington DC: Taylor and Francis, 1993). [13] C.C. Hong, J.W. Choi and C.H. Ahn, A Novel In-Plane Passive Micromixer Using Coanda Effect, Micro Total Analysis Systems, 2001, 31-33.