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Evaluation of a turbulence-based description of
the air-water gas transfer velocity
Leonie Esters, Erik Sahl´ee, Erik Nilsson, Lucia Guti´errez-Loza,
Anna Rutgersson
ICOS Science Conference 2020
15.09.2020
Leonie Esters Turbulence-based description of the air-water gas transfer velocity 1
Turbulence and Air-Sea Gas Transfer
• The gas transfer velocity k
is usually parametrised as
function of wind speed
• There are attempts to
relate k directly to
near-surface turbulence
⇒ k = A · ( ν)1/4 Sc−n
(Lamont and Scott, 1970)
: dissipation rate of TKE
ν: viscosity of water
Sc: Schmidt number
n: Sc exponent
1/2 ≤ n ≤ 2/3
A: proportionality coefficient
0 2 4 6 8 10 12 14 16
0
20
40
60
80
100
120
Wanninkhof (1992)
Wanninkhof + Mc Gillis (1999)
Liss + Merlivat (1986)
k660
[cmhr
−1
]
u
10
[m s−1
]
Leonie Esters Turbulence-based description of the air-water gas transfer velocity 2
5-beam Acoustic Doppler Current Profiler (ADCP)
Simpson et al. 2001
• ADCPs measure the 3D current
field
• They send sound waves, which are
reflected by particles in the water
• The particles velocity is
determined using the Doppler
effect
• Measurements of:
• water current speed
• water turbulence
• wave characteristics
Leonie Esters Turbulence-based description of the air-water gas transfer velocity 3
Deployment in lake Erken
Leonie Esters Turbulence-based description of the air-water gas transfer velocity 4
Observations 2018
• 21 days of data
• No reliable
observations of k
• Waves follow the
wind
• Deepening of the
mixing layer depth
(XLD) coincide with
increased winds and
waves
Leonie Esters Turbulence-based description of the air-water gas transfer velocity 5
Observations
• 73 days of data
• No observations of k
• Waves follow the
wind
• Deepening of the
XLD coincide with
increased winds,
waves, and positive
buoyancy flux
Leonie Esters Turbulence-based description of the air-water gas transfer velocity 6
Surface turbulence versus wind speed
• Total of 94 days
of data
• Filled circles:
2018,
open circles:
2019
• Linear relation
between surface
turbulence and
wind speed
⇒ Turbulence is
wind-driven
-9.5 -9 -8.5 -8 -7.5 -7 -6.5 -6
log10( 05
) [m2
s-3
]
0
2
4
6
8
10
12
14
u10
[ms-1
]
Leonie Esters Turbulence-based description of the air-water gas transfer velocity 7
Relating surface turbulence to k
• Wind-speed based
parametrisation for
k by Cole and
Caraco (1998):
k600 = 2.07+0.215u1.7
10
⇒ turbulence-based
model explains the
gas transfer velocity
calculated following
Cole and Caraco
(1998).
100
101
A Sc-n
( 05
)1/4
[cm hr-1
]
100
101
k600
CC
[cmhr-1
]
A = 1.3
R2
= 0.797
2
4
6
8
10
12
14
u10[ms-1
]
Leonie Esters Turbulence-based description of the air-water gas transfer velocity 8
Outlook: ¨Ostergarnsholm
• At the moment, the ADCP is deployed in
the footprint of the flux tower on
¨Ostergarnsholm Island in the Baltic Sea.
• There, we have observations of k.
⇒ Surface turbulence can be directly related
to the measured k.
Leonie Esters Turbulence-based description of the air-water gas transfer velocity 9

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Esters, Leonie: Evaluation of a turbulence-based description of the air-water gas transfer velocity

  • 1. Evaluation of a turbulence-based description of the air-water gas transfer velocity Leonie Esters, Erik Sahl´ee, Erik Nilsson, Lucia Guti´errez-Loza, Anna Rutgersson ICOS Science Conference 2020 15.09.2020 Leonie Esters Turbulence-based description of the air-water gas transfer velocity 1
  • 2. Turbulence and Air-Sea Gas Transfer • The gas transfer velocity k is usually parametrised as function of wind speed • There are attempts to relate k directly to near-surface turbulence ⇒ k = A · ( ν)1/4 Sc−n (Lamont and Scott, 1970) : dissipation rate of TKE ν: viscosity of water Sc: Schmidt number n: Sc exponent 1/2 ≤ n ≤ 2/3 A: proportionality coefficient 0 2 4 6 8 10 12 14 16 0 20 40 60 80 100 120 Wanninkhof (1992) Wanninkhof + Mc Gillis (1999) Liss + Merlivat (1986) k660 [cmhr −1 ] u 10 [m s−1 ] Leonie Esters Turbulence-based description of the air-water gas transfer velocity 2
  • 3. 5-beam Acoustic Doppler Current Profiler (ADCP) Simpson et al. 2001 • ADCPs measure the 3D current field • They send sound waves, which are reflected by particles in the water • The particles velocity is determined using the Doppler effect • Measurements of: • water current speed • water turbulence • wave characteristics Leonie Esters Turbulence-based description of the air-water gas transfer velocity 3
  • 4. Deployment in lake Erken Leonie Esters Turbulence-based description of the air-water gas transfer velocity 4
  • 5. Observations 2018 • 21 days of data • No reliable observations of k • Waves follow the wind • Deepening of the mixing layer depth (XLD) coincide with increased winds and waves Leonie Esters Turbulence-based description of the air-water gas transfer velocity 5
  • 6. Observations • 73 days of data • No observations of k • Waves follow the wind • Deepening of the XLD coincide with increased winds, waves, and positive buoyancy flux Leonie Esters Turbulence-based description of the air-water gas transfer velocity 6
  • 7. Surface turbulence versus wind speed • Total of 94 days of data • Filled circles: 2018, open circles: 2019 • Linear relation between surface turbulence and wind speed ⇒ Turbulence is wind-driven -9.5 -9 -8.5 -8 -7.5 -7 -6.5 -6 log10( 05 ) [m2 s-3 ] 0 2 4 6 8 10 12 14 u10 [ms-1 ] Leonie Esters Turbulence-based description of the air-water gas transfer velocity 7
  • 8. Relating surface turbulence to k • Wind-speed based parametrisation for k by Cole and Caraco (1998): k600 = 2.07+0.215u1.7 10 ⇒ turbulence-based model explains the gas transfer velocity calculated following Cole and Caraco (1998). 100 101 A Sc-n ( 05 )1/4 [cm hr-1 ] 100 101 k600 CC [cmhr-1 ] A = 1.3 R2 = 0.797 2 4 6 8 10 12 14 u10[ms-1 ] Leonie Esters Turbulence-based description of the air-water gas transfer velocity 8
  • 9. Outlook: ¨Ostergarnsholm • At the moment, the ADCP is deployed in the footprint of the flux tower on ¨Ostergarnsholm Island in the Baltic Sea. • There, we have observations of k. ⇒ Surface turbulence can be directly related to the measured k. Leonie Esters Turbulence-based description of the air-water gas transfer velocity 9