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SECONDHAND SMOKE IN MINNESOTA MULTI-UNIT HOUSING : 
Using physicochemical properties of tobacco smoke to identify SHS incursion in multi-unit housing 
Zheng Zhou, S.D., David Bohac, P.E., Martha Hewett, Joshua Novacheck 
Lara A. Gundel, Ph.D. (LBNL) 
October 15, 2014
Pg. 2 
Introduction 
•26% of U.S. households live in multi-unit housing (34 million households) 
•Nearly half report SHS incursions in the past 12 months (King et al. 2010, Hewett et al. 2007) 
•Air moves between units: 
•Bohac et al. (2011) found upper floor units in 6 Minnesota buildings got 2-65% of their air from other units (median 16%) 
•Residents in multi-unit housing have little control over their exposure to SHS 
•Households in smoking-permitted buildings had higher PM2.5 concentration than households in smoke-free buildings (Russo et al. 2014)
Pg. 3 
Measuring SHS Exposure at Homes 
•Fine particle (PM2.5) 
•Pros: 
•easy to measure 
•real-time 
•Cons: 
•not specific to tobacco smoke 
•rely on resident’s activity log 
•Nicotine 
•Pros: 
•highly specific to tobacco smoke 
•Cons: 
•not very sensitive at low concentration, 
•time-weighted average, 
•may not transfer at the same rate as other SHS constitutes
Pg. 4 
Objectives 
•Develop a cost-effective approach to identify and quantify SHS transfer in multi- unit housing 
•Assess non-smokers’ exposure to SHS in multi-unit housing in the Minneapolis-St. Paul metropolitan area
Pg. 5 
Ultraviolet-absorbing Particulate Matter (UVPM) 
•Combustion-derived 
•Contains organic compounds (e.g. PAHs) and black carbon 
•(UVPM-BC)/UVPM distinguish tobacco smoke from other common indoor sources
Pg. 6 
Study Design 
•Chamber test 
•Cigarette smoke, wood smoke, stick incense, candle and cooking activities 
•Field test 
•Three units (1 smoker’s; 1 adjacent non-smoker’s, and 1 above non-smoker’s) 
•Field monitoring 
•65 nonsmoker’s units in smoking-permitted buildings in winter (42 were re-monitored in mild weather) 
•14 nonsmoker’s units in smoke-free buildings in winter (8 were re-monitored in mild weather)
Pg. 7 
Measurements 
•Real-time UVPM and BC (1 min interval) 
•Dual-Channel Aethalometer (Magee Scientific) 
•Wavelengths: 880 nm for BC, 370 nm for UVPM 
•Real-time PM2.5 (1 min interval) 
•Sidepak AM510 (TSI) 
•Integrated gas phase sample 
•Active sampling in Tenax TA sorbent tube 
•Nicotine, 3-Ethenylpyridine (3-EP)
Pg. 8 
Other Measurements 
•Room temperature and relative humidity 
•Hobo logger (Onset) 
•Pressure difference between units and hallway/outdoor 
•APT digital micromanometer (TEC)/Rabbit 
•Range/oven use 
•iButton logger (Maxim) 
•Toaster, microwave oven use 
•Current transducer w/logger 
•Resident’s hourly activity log
Pg. 9 
Chamber Test: a Smolder-smoked 
Cigarette 
16:00 17:00 18:00 19:00 20:00 21:00 22:00 
0 
100 
200 
300 
400 
500 
600 
0.0 
0.2 
0.4 
0.6 
0.8 
1.0 
PM 
UVPM 
BC 
(UVPM-BC)/UVPM 
PM2.5 , UVPM and BC (mg/m3) 
(UVPM-BC)/UVPM 
PM 
UVPM 
BC 
(UVPM-BC)/UVPM
Pg. 10 
Chamber Test: Cooking (Frying Bacon) 
15:00 16:00 17:00 18:00 19:00 20:00 
0 
100 
200 
300 
400 
500 
600 
0.0 
0.2 
0.4 
0.6 
0.8 
1.0 
PM 
UVPM 
BC 
(UVPM-BC)/UVPM 
(UVPM-BC)/UVPM 
PM 
UVPM 
BC 
(UVPM-BC)/UVPM 
PM2.5 , UVPM and BC (mg/m3)
Pg. 11 
Chamber Test Results 
0.9 
(UVPM-BC)/UVPM 
Average PM2.5 (mg/m3) 
0.0 
0.2 
0.4 
0.6 
0.8 
1.0 
Candle_0828 
Candle_0824 
Popcorn_0709 
Hamburger_0904 
Onion_0904 
FriedEgg_0828 
Poptart_0904 
Bacon_0828 
Bread_0831 
BurntBread_0825 
BurntPopcorn_0719 
WoodSmoke_1228 
WoodSmoke_1230 
WoodSmoke_1231 
Incense_0903 
Incense_0821 
Cigarette_1116 
Cigarette_1229 
Cigarette_1023 
Cigarette_1028 
Cigarette_1029 
Cigarette_1014 
Cigarette_1015 
Cigarette_1026 
Cigarette_1027 
Cigarette_1113 
0 
200 
400 
600 
800 
Tobacco 
smoke 
Wood smoke, 
Incense, burnt 
food
Pg. 12 
Field Test 
•Three units in a two-floor smoking-permitted building for 10 days 
•One smoker’s unit in the first floor 
•One non-smoker’s unit above the smoker’s unit 
•One non-smoker’s unit adjacent to the smoker’s unit
Pg. 13 
Example: 24-hour Measurements 
Self-reported Smoking 
Ratio: 0.9 to 0.96 
Self-reported 
Smoking + Candle 
+ Burnt food 
Ratio: 0.8 to 0.9 
Ratio: 0.9 
0 
500 
1000 
1500 
2000 
0 
10 
20 
30 
40 
50 
00:00 02:00 04:00 06:00 08:00 10:00 12:00 14:00 16:00 18:00 20:00 22:00 00:00 
Smoker unit 
Above NS unit 
Ratio: 0.81 
Smoker’s unit PM2.5 (mg/m3) 
Non-smoker’s unit PM2.5 (mg/m3)
Pg. 14 
PM Events in Smoker’s Unit 
0.9 
(UVPM-BC)/UVPM 
Self-reported 
Smoking 
Average PM2.5 (mg/m3) 
Self-reported smoking 
+ Other 
Unknown 
0.0 
0.2 
0.4 
0.6 
0.8 
1.0 
0 
200 
400 
600 
800 
1000 
Burnt food 
+ candle 
cooking
Pg. 15 
PM Events in Above Non-smoker’s Unit 
(UVPM-BC)/UVPM 
0.9 
Average PM2.5 (mg/m3) 
Burnt food 
Burnt food 
0.0 
0.2 
0.4 
0.6 
0.8 
1.0 
0 
5 
10 
15 
20 
25 
30 
Suspected SHS 
transfer from the 
smoker’s unit 
Self-reported 
non-smoking 
activities 
Unknown 
Stove & 
toaster
Pg. 16 
Field Test Results 
UNIT 
# OF PM2.5 EVENTS 
# OF SHS EVENTS 
TOTAL SHS EXPOSURE* (mg/m3•hr) 
3-EP (ng/m3) 
NICOTINE (ng/m3) 
SMOKER’S UNIT 
31 
26 
6093 
472.8 
530.0 
ABOVE NON- SMOKER’S UNIT 
18 
11 
1492 
203.8 
88.5 
ADJACENT NON- SMOKER’S UNIT 
25 
10 
220 
49.1 
140.1 
* SHS Exposure is quantified using PM2.5 concentration
Pg. 17 
Field Monitoring 
•65 nonsmoker's units in smoking-permitted buildings in winter (of which 42 were re- monitored in mild weather) 
•14 nonsmoker's units in smoke-free buildings in winter (of which 8 were re- monitored in mild weather)
Pg. 18 
Field Monitoring Results 
Building 
# of units 
Average # of SHS events per unit (6 days) 
Average SHS exposure per unit in 6 days * (mg/m3•hr) 
Average 3- EP level (ng/m3) 
Average Nicotine level (ng/m3) 
Smoke- permitted (winter) 
65 
2.4 
245.4 
52.4 
41.1 
Smoke-free (winter) 
14 
0.9 
36.7 
17.0 
12.8 
Smoke- permitted (mild) 
42 
1.1 
94.3 
52.5 
33.5 
Smoke-free (mild) 
8 
0.4 
48.9 
16.4 
28.5 
* SHS Exposure is quantified using PM2.5 concentration
Pg. 19 
Conclusion 
•Findings 
•Non-smoker resident’s activity log often miss SHS incursion 
•(UVPM – BC)/UVPM > 0.9 indicates tobacco smoke 
•Many determinants affect SHS transfer 
•SHS incursion and exposure were lower in smoke- free buildings than in smoking-permitted buildings 
•Limitations 
•Mix of sources 
•Potential confounders: burning wood and incense, grilling or charring food
Second Hand Smoke in Minnesota Muli-Unit Housing

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Second Hand Smoke in Minnesota Muli-Unit Housing

  • 1. SECONDHAND SMOKE IN MINNESOTA MULTI-UNIT HOUSING : Using physicochemical properties of tobacco smoke to identify SHS incursion in multi-unit housing Zheng Zhou, S.D., David Bohac, P.E., Martha Hewett, Joshua Novacheck Lara A. Gundel, Ph.D. (LBNL) October 15, 2014
  • 2. Pg. 2 Introduction •26% of U.S. households live in multi-unit housing (34 million households) •Nearly half report SHS incursions in the past 12 months (King et al. 2010, Hewett et al. 2007) •Air moves between units: •Bohac et al. (2011) found upper floor units in 6 Minnesota buildings got 2-65% of their air from other units (median 16%) •Residents in multi-unit housing have little control over their exposure to SHS •Households in smoking-permitted buildings had higher PM2.5 concentration than households in smoke-free buildings (Russo et al. 2014)
  • 3. Pg. 3 Measuring SHS Exposure at Homes •Fine particle (PM2.5) •Pros: •easy to measure •real-time •Cons: •not specific to tobacco smoke •rely on resident’s activity log •Nicotine •Pros: •highly specific to tobacco smoke •Cons: •not very sensitive at low concentration, •time-weighted average, •may not transfer at the same rate as other SHS constitutes
  • 4. Pg. 4 Objectives •Develop a cost-effective approach to identify and quantify SHS transfer in multi- unit housing •Assess non-smokers’ exposure to SHS in multi-unit housing in the Minneapolis-St. Paul metropolitan area
  • 5. Pg. 5 Ultraviolet-absorbing Particulate Matter (UVPM) •Combustion-derived •Contains organic compounds (e.g. PAHs) and black carbon •(UVPM-BC)/UVPM distinguish tobacco smoke from other common indoor sources
  • 6. Pg. 6 Study Design •Chamber test •Cigarette smoke, wood smoke, stick incense, candle and cooking activities •Field test •Three units (1 smoker’s; 1 adjacent non-smoker’s, and 1 above non-smoker’s) •Field monitoring •65 nonsmoker’s units in smoking-permitted buildings in winter (42 were re-monitored in mild weather) •14 nonsmoker’s units in smoke-free buildings in winter (8 were re-monitored in mild weather)
  • 7. Pg. 7 Measurements •Real-time UVPM and BC (1 min interval) •Dual-Channel Aethalometer (Magee Scientific) •Wavelengths: 880 nm for BC, 370 nm for UVPM •Real-time PM2.5 (1 min interval) •Sidepak AM510 (TSI) •Integrated gas phase sample •Active sampling in Tenax TA sorbent tube •Nicotine, 3-Ethenylpyridine (3-EP)
  • 8. Pg. 8 Other Measurements •Room temperature and relative humidity •Hobo logger (Onset) •Pressure difference between units and hallway/outdoor •APT digital micromanometer (TEC)/Rabbit •Range/oven use •iButton logger (Maxim) •Toaster, microwave oven use •Current transducer w/logger •Resident’s hourly activity log
  • 9. Pg. 9 Chamber Test: a Smolder-smoked Cigarette 16:00 17:00 18:00 19:00 20:00 21:00 22:00 0 100 200 300 400 500 600 0.0 0.2 0.4 0.6 0.8 1.0 PM UVPM BC (UVPM-BC)/UVPM PM2.5 , UVPM and BC (mg/m3) (UVPM-BC)/UVPM PM UVPM BC (UVPM-BC)/UVPM
  • 10. Pg. 10 Chamber Test: Cooking (Frying Bacon) 15:00 16:00 17:00 18:00 19:00 20:00 0 100 200 300 400 500 600 0.0 0.2 0.4 0.6 0.8 1.0 PM UVPM BC (UVPM-BC)/UVPM (UVPM-BC)/UVPM PM UVPM BC (UVPM-BC)/UVPM PM2.5 , UVPM and BC (mg/m3)
  • 11. Pg. 11 Chamber Test Results 0.9 (UVPM-BC)/UVPM Average PM2.5 (mg/m3) 0.0 0.2 0.4 0.6 0.8 1.0 Candle_0828 Candle_0824 Popcorn_0709 Hamburger_0904 Onion_0904 FriedEgg_0828 Poptart_0904 Bacon_0828 Bread_0831 BurntBread_0825 BurntPopcorn_0719 WoodSmoke_1228 WoodSmoke_1230 WoodSmoke_1231 Incense_0903 Incense_0821 Cigarette_1116 Cigarette_1229 Cigarette_1023 Cigarette_1028 Cigarette_1029 Cigarette_1014 Cigarette_1015 Cigarette_1026 Cigarette_1027 Cigarette_1113 0 200 400 600 800 Tobacco smoke Wood smoke, Incense, burnt food
  • 12. Pg. 12 Field Test •Three units in a two-floor smoking-permitted building for 10 days •One smoker’s unit in the first floor •One non-smoker’s unit above the smoker’s unit •One non-smoker’s unit adjacent to the smoker’s unit
  • 13. Pg. 13 Example: 24-hour Measurements Self-reported Smoking Ratio: 0.9 to 0.96 Self-reported Smoking + Candle + Burnt food Ratio: 0.8 to 0.9 Ratio: 0.9 0 500 1000 1500 2000 0 10 20 30 40 50 00:00 02:00 04:00 06:00 08:00 10:00 12:00 14:00 16:00 18:00 20:00 22:00 00:00 Smoker unit Above NS unit Ratio: 0.81 Smoker’s unit PM2.5 (mg/m3) Non-smoker’s unit PM2.5 (mg/m3)
  • 14. Pg. 14 PM Events in Smoker’s Unit 0.9 (UVPM-BC)/UVPM Self-reported Smoking Average PM2.5 (mg/m3) Self-reported smoking + Other Unknown 0.0 0.2 0.4 0.6 0.8 1.0 0 200 400 600 800 1000 Burnt food + candle cooking
  • 15. Pg. 15 PM Events in Above Non-smoker’s Unit (UVPM-BC)/UVPM 0.9 Average PM2.5 (mg/m3) Burnt food Burnt food 0.0 0.2 0.4 0.6 0.8 1.0 0 5 10 15 20 25 30 Suspected SHS transfer from the smoker’s unit Self-reported non-smoking activities Unknown Stove & toaster
  • 16. Pg. 16 Field Test Results UNIT # OF PM2.5 EVENTS # OF SHS EVENTS TOTAL SHS EXPOSURE* (mg/m3•hr) 3-EP (ng/m3) NICOTINE (ng/m3) SMOKER’S UNIT 31 26 6093 472.8 530.0 ABOVE NON- SMOKER’S UNIT 18 11 1492 203.8 88.5 ADJACENT NON- SMOKER’S UNIT 25 10 220 49.1 140.1 * SHS Exposure is quantified using PM2.5 concentration
  • 17. Pg. 17 Field Monitoring •65 nonsmoker's units in smoking-permitted buildings in winter (of which 42 were re- monitored in mild weather) •14 nonsmoker's units in smoke-free buildings in winter (of which 8 were re- monitored in mild weather)
  • 18. Pg. 18 Field Monitoring Results Building # of units Average # of SHS events per unit (6 days) Average SHS exposure per unit in 6 days * (mg/m3•hr) Average 3- EP level (ng/m3) Average Nicotine level (ng/m3) Smoke- permitted (winter) 65 2.4 245.4 52.4 41.1 Smoke-free (winter) 14 0.9 36.7 17.0 12.8 Smoke- permitted (mild) 42 1.1 94.3 52.5 33.5 Smoke-free (mild) 8 0.4 48.9 16.4 28.5 * SHS Exposure is quantified using PM2.5 concentration
  • 19. Pg. 19 Conclusion •Findings •Non-smoker resident’s activity log often miss SHS incursion •(UVPM – BC)/UVPM > 0.9 indicates tobacco smoke •Many determinants affect SHS transfer •SHS incursion and exposure were lower in smoke- free buildings than in smoking-permitted buildings •Limitations •Mix of sources •Potential confounders: burning wood and incense, grilling or charring food