1. The thesis proposes a new method for creating coherent superpositions among the ground states of a tripod atom using three frequency-chirped laser pulses. It shows that two different population redistribution mechanisms can be achieved by changing the sign of the Raman detuning of one pulse, while avoiding significant atomic excitation.
2. It proposes a method for writing and storing optical phase information in the populations of the ground states of a tripod atom using the same three chirped pulse arrangement. The phase difference between the two Raman resonant pulses maps the population of the third ground state, allowing long storage times.
3. It demonstrates that a pair of pulses, one constant frequency and one chirped, establishes maximum
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International Journal of Engineering Research and Development (IJERD)IJERD Editor
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(v3) Phonon as carrier of electromagnetic interaction between vibrating latti...Qiang LI
With emphasis on time-dependency of electron-lattice system, we suggest the fallacy of presumed quantization in the context of electron-lattice system and propose the definition of phonons as carriers of electromagnetic interaction between electrons and vibrating lattice. We have investigated behaviors of electron-lattice system relating to “measured” energy, identified non-stationary steady state of electrons engaging in “electron pairing by virtual stimulated transitions”, recognized some origins of binding energy of electron pairs in crystals, and explained the state of electrons under pairing. Moreover, we have recognized the behavior and role of threshold phonon, which exists in electron pairing and is released by the electron from excited state, and have recognized the redundancy of the threshold phonon when the electrons under pairing have entered non-stationary steady state. We have also studied the effect of the stability of lattice wave on the evolution of the function of transition probability and on the stability of phonon-mediated electron pairs, the competition among multiple pairings associated with one same ground state, and determination of presence/absence of superconductivity by such competition.
International Journal of Engineering Research and Applications (IJERA) is an open access online peer reviewed international journal that publishes research and review articles in the fields of Computer Science, Neural Networks, Electrical Engineering, Software Engineering, Information Technology, Mechanical Engineering, Chemical Engineering, Plastic Engineering, Food Technology, Textile Engineering, Nano Technology & science, Power Electronics, Electronics & Communication Engineering, Computational mathematics, Image processing, Civil Engineering, Structural Engineering, Environmental Engineering, VLSI Testing & Low Power VLSI Design etc.
Spatially adiabatic frequency conversion in opto-electro-mechanical arraysOndrej Cernotik
Optoelectromechanical systems offer a promising route towards frequency conversion between microwaves and light and towards building quantum networks of superconducting circuits. Current theoretical and experimental efforts focus on approaches based on either optomechanically induced transparency or adiabatic passage. The former has the advantage of working with time-independent control but only in a limited bandwidth (typically much smaller than the cavity linewidth); the latter can, in principle, be used to increase the bandwidth but at the expense of working with time-dependent control fields and with strong optomechanical coupling. In my presentation, I will show that an array of optoelectromechanical transducers can overcome this limitation and reach a bandwidth that is larger than the cavity linewidth. The coupling rates are varied in space throughout the array so that a mechanically dark mode of the propagating fields adiabatically changes from microwave to optical or vice versa. This strategy also leads to significantly reduced thermal noise with the collective optomechanical cooperativity being the relevant figure of merit. I will also demonstrate that, remarkably, the bandwidth enhancement per transducer element is largest for small arrays. With these features the scheme is particularly relevant for improving the conversion bandwidth in state-of-the-art experimental setups.
Measurement of the Lifetime of the 59.5keV excited State of 237Np from the Al...theijes
The International Journal of Engineering & Science is aimed at providing a platform for researchers, engineers, scientists, or educators to publish their original research results, to exchange new ideas, to disseminate information in innovative designs, engineering experiences and technological skills. It is also the Journal's objective to promote engineering and technology education. All papers submitted to the Journal will be blind peer-reviewed. Only original articles will be published.
(v3) Phonon as carrier of electromagnetic interaction between vibrating latti...Qiang LI
With emphasis on time-dependency of electron-lattice system, we suggest the fallacy of presumed quantization in the context of electron-lattice system and propose the definition of phonons as carriers of electromagnetic interaction between electrons and vibrating lattice. We have investigated behaviors of electron-lattice system relating to “measured” energy, identified non-stationary steady state of electrons engaging in “electron pairing by virtual stimulated transitions”, recognized some origins of binding energy of electron pairs in crystals, and explained the state of electrons under pairing. Moreover, we have recognized the behavior and role of threshold phonon, which exists in electron pairing and is released by the electron from excited state, and have recognized the redundancy of the threshold phonon when the electrons under pairing have entered non-stationary steady state. We have also studied the effect of the stability of lattice wave on the evolution of the function of transition probability and on the stability of phonon-mediated electron pairs, the competition among multiple pairings associated with one same ground state, and determination of presence/absence of superconductivity by such competition.
International Journal of Engineering Research and Applications (IJERA) is an open access online peer reviewed international journal that publishes research and review articles in the fields of Computer Science, Neural Networks, Electrical Engineering, Software Engineering, Information Technology, Mechanical Engineering, Chemical Engineering, Plastic Engineering, Food Technology, Textile Engineering, Nano Technology & science, Power Electronics, Electronics & Communication Engineering, Computational mathematics, Image processing, Civil Engineering, Structural Engineering, Environmental Engineering, VLSI Testing & Low Power VLSI Design etc.
Spatially adiabatic frequency conversion in opto-electro-mechanical arraysOndrej Cernotik
Optoelectromechanical systems offer a promising route towards frequency conversion between microwaves and light and towards building quantum networks of superconducting circuits. Current theoretical and experimental efforts focus on approaches based on either optomechanically induced transparency or adiabatic passage. The former has the advantage of working with time-independent control but only in a limited bandwidth (typically much smaller than the cavity linewidth); the latter can, in principle, be used to increase the bandwidth but at the expense of working with time-dependent control fields and with strong optomechanical coupling. In my presentation, I will show that an array of optoelectromechanical transducers can overcome this limitation and reach a bandwidth that is larger than the cavity linewidth. The coupling rates are varied in space throughout the array so that a mechanically dark mode of the propagating fields adiabatically changes from microwave to optical or vice versa. This strategy also leads to significantly reduced thermal noise with the collective optomechanical cooperativity being the relevant figure of merit. I will also demonstrate that, remarkably, the bandwidth enhancement per transducer element is largest for small arrays. With these features the scheme is particularly relevant for improving the conversion bandwidth in state-of-the-art experimental setups.
Measurement of the Lifetime of the 59.5keV excited State of 237Np from the Al...theijes
The International Journal of Engineering & Science is aimed at providing a platform for researchers, engineers, scientists, or educators to publish their original research results, to exchange new ideas, to disseminate information in innovative designs, engineering experiences and technological skills. It is also the Journal's objective to promote engineering and technology education. All papers submitted to the Journal will be blind peer-reviewed. Only original articles will be published.
Alle prognoser for tungtrafikk lang E6 gjennom Mo i Rana peker oppover. I tillegg kommer økt trafikk til og fra en eventuell ny flyplass. Problemene med glatt veg over byåsen vinterstid er store og kostbare. I tillegg kommer helseproblemer knyttet til støy og støv i boområdene langs E6. Hovedferdselsåren gjennom Mo i Rana må legge i tunnel slik Statens Vegvesen bl.a. har gjort i Steinkjer.
When big vеhісlеѕ аrе іnvоlvеd in rоаd mіѕhарѕ, соmmеrсіаl tоwіng services соmе to the rеѕсuе tо оffеr lіght and heavy duty towing services. Clеаrіng the road promptly аftеr ассіdеntѕ іnvоlvіng bіg rigs, loaded trаіlеrѕ, buѕеѕ, tankers, mоtоr hоmеѕ, аnd оthеr large vеhісlеѕ, іѕ іmреrаtіvе аѕ these crashes may rеԛuіrе additional rоаd сlоѕurеѕ tо clean up the mess frоm spilled рrоduсt, glаѕѕ, аnd debris. Aѕ thе owner of thе vеhісlе involved, уоu also wаnt tо hаvе thе problem handled wіth the lеаѕt amount of lоѕѕ tо уоur соmраnу.
Game Lab promotes the research and development of interactive content, such as digital games, playful software applications.
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https://twitter.com/emgamelab
The Effect of RF Power on ion current and sheath current by electrical circui...irjes
Plasma is very important in the development of technology as it is applied in many electronic devices
such as global positioning system (GPS). In addition, fusion and process of plasma requires important elements,
namely, the electron energy distribution. However, plasma glow is a relatively new research field in physics.
There has not been found any previous study on the electric plasma modeling. Thus, this study was aimed to
study plasma modeling especially to find out what was the difference in the number of density and the
temperature of the electron in the plasma glow before and after heated and to discover how was the distribution
of electron and ion in the plasma. This research was conducted at Brawijaya University, Malang, Indonesia in
the Faculty of Science. This exploration began in the middle of June 2013. The data collection and data analysis
were done during a year around until August 2014. In this research, characteristics of plasma were studied to
build model of plasma. It utilized MATLAB dialect program examination framework which result in the
distribution of temperature and current density. The findings show that there has been a large increase in the
number of U, U2 with power, while figures of U1 is stable until middle of curve and then decrease as u but u2
after increase at point then stable. The differences appearing are probably due to the simplifying assumptions
considered in the present model. There was a curve between current in sheath and plasma. And time and sheath
current increased in the beginning then decreased before they experienced another increase.
The Monte Carlo Method of Random Sampling in Statistical PhysicsIOSR Journals
The Monte Carlo technique of random sampling was reviewed in this work. It plays an important role in Statistical Mechanics as well as in scientific computation especially when problems have a vast phase space. The purpose of this paper is to review a general method, suitable to fast electronic computing machines, for calculating the properties of any system which may be considered as composed of interacting particles. Concepts such as phase transition, the Ising model,ergodicity, simple sampling, Metropolis algorithm, quantum Monte Carlo and Non-Boltzmann sampling were discussed. The applications of Monte Carlo method in other areas of study aside Statistical Physics werealso mentioned.
AN INTRODUCTION TO BASIC PHENOMENA OF PLASMA PHYSICSDr. Ved Nath Jha
Plasma is a set of neutral and charged particles which reveals a number of collective behaviors. The very
long range coulomb forces enable the charged particles in plasma to work together with one another
simultaneously. The study of plasma is actually a really ancient area of investigation in plasma physics
and it remains to be among the vital fields due to the crucial role of its in most plasma uses including
plasma processing, fabrication of semiconductor systems, etching, etc. except the presence of just ions
and electrons, the plasma in many instances, has a number of other species of ions like negative ions
which impact the complete plasma behaviour. Within this paper we study about the fundamental ideas of
plasma physics.
The Equation Based on the Rotational and Orbital Motion of the PlanetsIJERA Editor
Equations of dependence of rotational and orbital motions of planets are given, their rotation angles are calculated. Wave principles of direct and reverse rotation of planets are established. The established dependencies are demonstrated at different scale levels of structural interactions, in biosystems as well. The accuracy of calculations corresponds to the accuracy of experimental data
Lattice Energy LLC - Two Facets of W-L Theorys LENR-active Sites Supported b...Lewis Larsen
“Spatial coherence and stability in a disordered organic polariton condensate”
K. Daskalakis et al. Physical Review Letters 115 pp. 035301 - 06 (2015)
Inside a laser-pumped microcavity, they demonstrated the formation of spatially localized, entangled plasmon condensates in 100 nm layer of organic TDAF molecules at room temperature in a disordered system. Created plasmon condensates have spatial dimensions that seem to max-out at diameters of ~100 μ; beyond this critical size limit they destabilize. First-order temporal coherence of condensates = 0.8 picoseconds (ps); this is in reasonable agreement with coherence decay time estimate of 1 ps which is calculated from the observed emission linewidth.
According to Widom-Larsen theory of LENRs, many-body collective quantum and electromagnetic effects are crucial and enabling to the operation of electroweak nuclear catalysis at ambient temperatures; quantum entanglement amongst protons and plasmons at LENR sites is inferred; 1 ps lifetime of plasmon condensate is very ample time for LENRs. In 2006 EPJC paper (Widom & Larsen) we originally estimated the size of many-body coherence domains in LENR sites on metallic hydride surfaces to be ~ 1 - 10 μ. As discussed in this document, in 2009 Larsen extended Widom-Larsen theory to cover occurrence of LENRs on organic aromatic molecules; at that time, maximum size of W-L coherence domains was re-estimated and increased up to ~ 100 μ. It is not known whether this striking similarity to Daskalakis et al.’s apparent size limit of 100 μ is coincidental. W-L active site functions like a microcavity; thus seems reasonable to speculate that the surface plasmons in LENR-active sites form condensates similar to what Daskalakis et al. observed.
Computational Chemistry aspects of Molecular Mechanics and Dynamics have been discussed in this presentation. Useful for the Undergraduate and Postgraduate students of Pharmacy, Drug Design and Computational Chemistry
FERROMAGNETIC-FERROELECTRIC COMPOSITE 1D NANOSTRUCTURE IN THE PURSUIT OF MAGN...ijrap
Nanocomposites of linear chain of ferroelectric-ferromagnetic crystal structure is considered. It is analyzed
theoretically in the motion equation method on the pursuit of magnonic excitations,lattice vibration
excitations and their interactions leading to a new collective mode of excitations,the electormagnons. In
this particular work, it is observed that the magnetizations and polarizations are tunable in a given temperature ranges for some specific values of the coupling order parameter.
Ferromagnetic-Ferroelectric Composite 1D Nanostructure in the Pursuit of Magn...ijrap
Nanocomposites of linear chain of ferroelectric-ferromagnetic crystal structure is considered. It is analyzed
theoretically in the motion equation method on the pursuit of magnonic excitations,lattice vibration
excitations and their interactions leading to a new collective mode of excitations,the electormagnons. In
this particular work, it is observed that the magnetizations and polarizations are tunable in a given
temperature ranges for some specific values of the coupling order parameter
Molecular Mechanics in Molecular ModelingAkshay Kank
In this slide you learn about the computational chemistry and its role in designing a drug molecule. Also learn concept about the molecular mechanics and its application to Computer Aided Drug Design. difference between the Quantum mechanics and Molecular Mechanics.
1. UNIVERSITY OF P´ECS
Doctoral School in Physics
Quantumoptics and Quantuminformation Programme
Coherent Control of Atomic Quantum States using
Frequency-chirped Laser Pulses
PhD Thesis
N´ora S´andor
Supervisor:
Dr. Gagik Djotjan
scientific advisor
P´ECS, 2013.
2.
3. Introduction
Understanding the interaction of matter and light was the problem which led to the birth of
quantum mechanics a hundred year ago. One of the most important discoveries which burst the
frames of classical physics was the discovery of spectral lines of atoms. The first model suitable
to explain this observation was by Niels Bohr in 1913: according to his model, only specific
orbits of electrons can exist inside an atom, with well-defined energies. When jumping between
the orbits, the electron would absorb or emit light corresponding to the energy difference of the
orbits.
In 1917, as an extension to Bohr’s model, Einstein introduced the concepts of absorption,
and spontaneous and stimulated emission, with which he created the foundation for the dis-
covery of the laser.
The appearance of lasers created new directions for the investigations of matter-light in-
teractions by providing an intense, monochromatic and coherent light source. By using laser
radiation, better and better coherent control of quantum states of atoms or atomic ensembles
can be achieved since it becomes possible to address specific atomic transitions.
By now, laser control of atoms has become an important and rapidly developing field of
quantum optics. One of the reasons is that the basic concepts of quantum mechanics can be
spectacularly demonstrated by experiments on atom-laser interaction. The significance of such
investigations was also highlighted recently by the Nobel-prize.
An important subfield of laser control of atoms is the control of the atoms’ valence elec-
trons using laser radiation. The development of this subject is motivated by the possibility of
numerous important applications in various fields of modern physics [1–4].
By coherently preparing the atoms, one can modify the optical (refractive and absorptive)
properties of the medium composed of said atoms. As a result, several interesting and important
nonlinear optical effects may occur or be enhanced [5–10].
The ability to precisely control internal atomic states can be also widely applied in quan-
tum information science. Using atoms as quantum memory devices seems to be especially
promising [11–13].
1
4. Previous work in the field
There is a large variety of techniques for the coherent control of atomic states. The simplest
solution is applying a laser pulse resonant with the atomic transition to be addressed. In this
case Rabi-oscillations occur between the coupled states and the proportion of the populations
in each state after the interaction depends on the area of the coupling pulse [14]. For example, if
this area equals an odd integer multiple of π, complete population inversion can be established.
The drawback of this method is that it is very sensitive even to relatively small variations of
the pulse area and to the resonance conditions, which may result in additional difficulties for
certain experimental setups.
In contrast, coherent control schemes based on adiabatic following, being less sensitive
to variations in the experimental parameters, ensure more robust control of atomic quantum
states. In these techniques, one of the parameters characteristic to the atom-laser interaction
is gradually changed over time, which allows the tuning of the atom’s inner state.
One possibility to realize adiabatic following is to change the coupling between the atomic
states over time. This is the basic principle of Stimulated Raman Adiabatic Passage (STI-
RAP) [15,16]. Here the control of a Λ-atom’s states is achieved by two time-shifted laser pulses
which interact with the atomic transitions in a so-called counter-intuitive order. As a result, the
population of one of the ground states is transferred to the other ground state without excita-
tion of the atom, provided that the two-photon resonance condition for the interacting pulses is
fulfilled. With extensions to the STIRAP scheme, coherence creation among metastable states
of the atom is also possible [17].
Another popular group of the adiabatic control schemes is based on a slowly time-changing
detuning between the atomic transition(s) and coupling laser field(s). One possibility for re-
alizing this time-variation is to shift the energy of the atomic levels as is done by a strong
non-resonant laser field in the case of Stark-chirped Rapid Adiabatic Passage (SCRAP), mak-
ing use of the Stark-effect.
An alternative is the temporal modulation of the frequency of the interacting laser pulse(s).
The usage of chirped laser pulses for coherent control of atoms has been the main focus of
2
5. the group of “Cold plasma and atomic physics” in the Wigner Research Center of Hungarian
Academy of Sciences, where I was working as a PhD-student and prepared my dissertation. As
direct antecedent to my work, this group made several proposals for solving different control
problems, making use of the advantages of chirped pulses.
For example, they proposed an alternative to the STIRAP-scheme by proving that, along
with negligible excitation of the atom, complete population-transfer can be achieved between
the two ground states of a Λ-atom with a single chirped pulse that couples both atomic transi-
tions [18,19]. By generalizing this scheme to a tripod-atom they showed that it is also possible
to create a coherent superposition among the atomic ground states with a single chirped pulse,
again, without significant excitation [20]. The main drawback of the latter method was that
the proportion of each state in the created superposition was determined by the properties of
the atom (e.g. energy-difference of the atomic levels, strength of the transitions between them).
The advantage of these schemes is that — due to the chirp — they are generally less
sensitive to resonance-conditions and thus may be successfully applied in both homogeneously
and inhomogeneously broadened media. It is important to avoid the atomic excitation, on one
hand, to avoid losing coherence due to spontaneous emission. On the other hand, as was shown
in [21] for Λ-atoms, the back-action of the atoms on the interacting laser pulses is small when
the atomic excitation is negligible, therefore, this scheme can be also applied for controlling the
atoms of a optically thick medium.
By applying more than one laser pulse it becomes possible to reach a wider range of atomic
states by varying the parameters of the interacting pulses. For example, when two chirped laser
pulses in Raman-resonance interact with a Λ-atom, initially prepared in a coherent superposi-
tion of its ground states, the final state of the atom established by these two pulses depends
on their constant phase-difference [22,23]. Making use of this peculiarity, the scheme was pro-
posed to be used for encoding of optical information into quantum states. The drawback of
this scheme is that the atom gets excited during the interaction.
3
6. Objectives
Motivated by these results, I concentrated in my thesis, on one hand, on upgrading the previous
control schemes using FC pulses in order to unify their advantages and to eliminate their
drawbacks. That is, one of my objectives was to develop a control scheme using a limited
number of chirped pulses which possesses the following characteristics. It is suitable for creating
coherent superpositions of the ground state of the atom, which can be adjusted by easily
controllable parameters of the interacting laser pulses such as the peak intensities or constant
phase difference. In order to avoid decoherence effects due to the finite lifetime of the excited
state, I regarded the avoiding of the excitation of the atom as a top priority.
Another goal of mine was to widen the range of possible applicability of chirped pulses by
combining them with constant-frequency pulses. I aimed to consider control schemes in Λ-atoms
which incorporate instantaneous Raman-resonance and to prove them useful in applications.
In optically thick media, the coherent control processes may be modified by the back-action
of the medium on the interacting pulses and other propagation effects. For nonlinear optical
applications it is necessary to take these effects into consideration. In my work, I had the
aim to discover an interaction scheme using chirped pulses which is applicable for preparing
the majority of the atoms in a coherent superposition of their ground states, in an externally
adjustable way if possible.
Applied scientific methods
In my thesis, I studied the interaction of atoms and atomic ensembles with a few (2 or 3)
frequency-modulated optical laser pulses in a semiclassical approach. From all the effects that
the electromagnetic field can possible have on atoms, I was interested in the transitions of the
valence electron among the atomic levels. The atoms are modeled as few dimensional quantum-
systems. This is possible because the considered laser pulses are all close to resonance with
a limited number of atomic transitions and thus transitions are only induced with a non-
negligible probability among the corresponding atomic levels. The interacting laser pulses are
4
7. strong, hence they can be well described as a classical potential in the Hamiltonian describing
the atom-laser interaction.
As the wavelength of optical electromagnetic fields is several orders of magnitude greater
than the size of an atom, the atoms can be treated as point-like compared to the interacting
light, which allows the application of the dipole-approximation for describing the atom-field
interaction. The coupling terms (Rabi-frequencies) between the atomic levels, which represents
the interaction of the atoms with the laser pulses, are small compared to the frequency of the
lasers and change slowly compared to the timescale defined by the reciprocal of the optical
frequency. In order to be consistent with the few-state atom models, the detuning between
the frequency of the interacting laser pulses (chirp included) and the frequencies of the atomic
transitions driven by them must remain several orders of magnitude smaller than the pulses’
frequency during the whole interaction. These features of the interaction described here allows
for the application of the rotating wave approximation.
In the majority of the schemes investigated in my dissertation, I assumed that each atomic
transition is driven by a separate laser pulse. This assumption can be realized for example by
using laser pulses with different polarization for inducing transitions between Zeeman-sublevels.
In the first part of the thesis, when my aim was to create schemes applicable for the coherent
preparation of a single atom (or an optically dilute medium), I have described the effect of the
laser pulses on the atoms in an interaction picture, by regarding them as external parameters.
The frequency-modulation of the pulses was taken into account by time-varing phase of the
coupling terms (Rabi-frequencies).
When investigating the interaction between a tripod-atom and three chirped pulses (theses
1. and 2.), I described the atomic dynamics using the master-equation, taking into account
the relaxation processes (both longitudinal and transverse) that occur inside the system, but
neglecting the decay towards the environment. The equations were numerically solved with
parameters plausible in experimental situations. The effect of certain factors (spontaneous
emission, dephasing, Doppler-broadening, parameters of laser pulses) on the proposed control
schemes was investigated. In the case of Doppler-broadening I averaged the results for different
values of detuning by weighting them with a probability-function obtained from the Maxwell-
5
8. Boltzmann distribution.
In the case of the interaction of a Λ-atom with a combination of a chirped and a constant-
frequency pulse (theses 3. and 4.), I made the assumption that the interaction time is sig-
nificantly shorter than the lifetime of the excited state and I calculated the atomic dynamics
by numerically solving the Schr´odinger-equation. The effect of the variation in the interac-
tion parameters was again investigated by numerical simulations for a wide range of parameter
values.
In thesis 4., I investigated the interaction of an atom having two ground states with a
combination of a chirped and a constant-frequency pulse, both far detuned from the possible
atomic transitions, through the example of the |5S1/2, F = 1 → |5P3/2 transition of 87
Rb.
I took into account all the possible atomic transitions allowed by the selection rules, which
resulted in a 7-level atom model.
When describing the interaction of a pair of Raman-resonant chirped pulses with an optically
dense medium (thesis 5.), it was necessary to take into account the back-action of the medium
on the electromagnetic fields. Therefore, the model treats the Rabi-frequencies as dynamical
variables (as opposed to external parameters) in this model, of which the dynamics is given by
the Maxwell-equations in the frame of slowly varying envelope approximation. The effect of the
medium’s atoms on the laser pulses is described by the macroscopic polarization. This quantity
is given in each spatial location by the average of the dipole moments of the atoms which are
in the infinitesimal proximity of the said location. The slowly varying envelope approximation
could be applied as the envelope of the laser pulses was slowly changing on the scales defined
by the frequency and wavelength of the laser pulses.
The majority of the interaction schemes proposed in this dissertation were based on the
gradual (adiabatic) change of the interacting laser pulses’ frequency. Therefore, the dynamics of
the atomic states could be described by using the adiabatic approximation. This approximation
gives information about the change of the atomic states over time by analyzing the eigenvalues
and eigenvectors of the interaction Hamiltonian of the atom-laser system. In addition to the
numerical methods described above, I also applied the ‘adiabatic following method’ for the
majority of the schemes in order to describe the underlying physical mechanisms behind the
6
9. numerical results.
Theses
1. I have proposed a new interaction scheme for creating coherent superposition among the
metastable (‘ground’) states of an atom having tripod-structure as working levels (‘tripod-
atom’), along with negligible excitation. The method is based on adiabatic control of the
atomic states by three laser pulses with the same (linear) modulation (‘chirp’) in their
carrier frequencies, each of them separately coupling one dipole allowed transition of
the atom. I have shown by analyzing the time evolution of the adiabatic states that if
two pulses are in Raman-resonance with the corresponding atomic transitions and the
third one is Raman-detuned, two different population-redistribution mechanism may be
achieved by changing the sign of the Raman-detuning, without significant population
appearing in the excited state during the interaction.
By numerically solving the master-equation of the system, I have demonstrated that the
scheme can be used even if the lifetime of the excited state is one tenth of the interaction
time. I have found that coherence can also be created between the ground state in the
presence of stronger spontaneous decay from the excited state, with a factor of π difference
in phase compared to the non-decaying case.
I have demonstrated that the presented scheme may be applicable in an (optically dilute)
atomic gas at room temperature in the case of fast enough frequency modulation and
copropagating pulses, since the chirp is capable to compensate for the Doppler-effect. [I,
II]
2. I have proposed a method for robust writing and storage of optical phase information in
the populations of the ground states of a tripod atom using three frequency-chirped laser
pulses, two in Raman resonance and the third Raman-detuned from the corresponding
atomic transition (the same arrangement as in thesis 1). The scheme is based on the
fact that after preparing the atom in a coherent superposition of the two ground states
coupled by two pulses in Raman resonance, the population of the third ground state
7
10. established by the interacting pulses is a cosine-function of the phase difference of the
pulses in Raman resonance. Since the information is mapped to the populations of the
atomic ground states, the proposed method provides much longer storage times compared
to the schemes based on collective atomic spin coherences, being only restricted by the
lifetime of the ground states.
I have shown that the presence of weak longitudinal and transverse relaxation affects the
contrast of the mapping process: 50% of contrast can be achieved if the duration of the
interaction is smaller than a tenth of the coherence lifetime and 10 times the excited state
lifetime, respectively [III].
3. I have demonstrated that a pair of laser pulses, one with constant and the other with
monotonously modulated carrier frequency, establishes a maximum coherence between
a ground and the excited state of a λ-atom. The initially unpopulated ground state
is resonantly coupled by a constant-frequency laser pulse to the excited state, forming
an Autler-Townes doublet, while the other pulse having a frequency sweeping through
one-photon and two photon resonance adiabatically transfers the population from the
ground state to that member of the doublet with which it first become resonant. I have
shown that the mechanism, provided the resonance condition of the constant-frequency
pulse is fulfilled, is extremely robust to the parameters of the laser pulses such as the
Rabi-frequencies or the chirp rate [IV].
4. I have proposed a novel scheme for creating coherent superposition between two magnetic
sublevels of the F = 1 hyperfine ground state of 87
Rb atoms. It is based on the interaction
of the atom with a frequency-modulated (chirped) laser pulse having σ+
and a pulse of
a constant carrier-frequency having σ−
circular polarization, both far detuned from one-
photon resonance but with the chirped pulse sweeping through two-photon resonance.
Taking into account all the possible atomic transitions allowed by the selection rules, I
have shown numerically that the scheme yields a maximum possible degree of coherence
of superposed states with negligible atomic excitation, which eliminates decoherence by
spontaneous emission [V].
8
11. 5. I have demonstrated a matching effect for a pair of frequency-modulated (chirped) Raman-
resonant laser pulses which simultaneously propagate in an optically thick medium of
lambda-structured atoms. That is, the laser pulses become distorted by the interaction
with the medium in such a way that it no longer causes excitation in the atoms, reducing
the back-action of the atoms on the pulses and allowing a quasi-lossless propagation. By
introducing a coordinate transformation, I separated a symmetric and an asymmetric
mode of the lasers, with the latter being 0 at the boundary of the medium. I have
shown that due to the excitation of the atoms at the boundary, the asymmetric mode
appears, changing the population transfer mechanism in such a way that the majority of
the population is transferred to the same coherent superposition of the atomic ground
states throughout the medium. I have also shown that the composition of this coherent
superposition can be controlled by the peak amplitudes of the these laser pulses at the
boundary of the medium [VI,VII].
Conclusion
In my PhD-thesis, I investigated adiabatic control schemes — suitable for preparation of atoms
or atomic ensembles in specific internal states — based on using frequency-modulated laser
pulses. I have shown that the proposed schemes are suitable for robustly creating coherent
superpositions between atomic quantum states in a way that it is possible to adjust the pro-
portion of each state in the superposition by external parameters (the proportion of the peak
amplitudes, and the difference of the complex phases of the interacting laser pulses). Since
these parameters are relatively easy to adjust in experiments, these schemes may easily find
applications in nonlinear optics or quantum information science. I also proposed a possible
application of the scheme for optical information writing.
By analyzing the propagation of a Raman-resonant chirped pulse pair in a medium consisting
of Λ-atoms I showed that control of the state of the atoms within the medium can be achieved
with a good efficiency. I have found that the chirped pulse pair can propagate in a quasi-lossless
way in the medium due to a self-organizing (matching) mechanism which is different from the
9
12. effect known for the propagation of constant-frequency pulses.
The physical system which served as a base of my investigations was a cold atomic cloud
of alkali atoms. More specifically, I modeled transitions of the atoms’ valence electron between
their metastable and first excited states. In future work I plan to investigate the applicability of
these schemes to other physical systems. One possible aim may be to create Rydberg-excitations
in atoms by applying chirped pulses. Another possible direction is to find applications of the
proposed schemes in solid-state systems, especially for the control of the states of artificial
atoms created in quantum dots.
10
13. Publications
Publications related to the theses:
[I] N. Sandor, J. S. Bakos, Zs. S¨orlei, and G. P. Djotyan,Creation of coherent superposition
states in inhomogeneously broadened media with relaxation. J. Opt. Soc. Am. B,
28:2785-2796, (2011).
[II] N. Sandor, J. S. Bakos, Zs. S¨orlei, and G. P. Djotyan. Creation of coherent superpositions
between metastable atomic states in doppler-broadened media. J. Phys. - Conf. Ser.,
350:012002, (2012).
[III] G. P. Djotyan, N. Sandor, J. S. Bakos, and Zs. Sorlei. Optical phase information writing
and storage in populations of metastable quantum states. J. Opt. Soc. Am. B., 26:1959-
1966, (2009).
[IV] G. P. Djotyan, N. Sandor, J. S. Bakos, and Zs. S¨orlei. An extremely robust strong-field
control of atomic coherence. Opt. Exp., 19:17493-17499, (2011).
[V] G. P. Djotyan, N. Sandor, J. S. Bakos, Zs. S¨orlei, W. Gawlik, A. Wojciechowski, J.
Zachorowski, S. Pustelny, G. Yu. Kryuchkyan. Creation and measurement of coherent
superposition states in multilevel atoms. Proc. SPIE 01/2011; 7998:79981A- 1. (2011).
[VI] N. Sandor, G. P. Djotyan. Propagation of Raman-resonant frequency chirped laser pulses
in a medium of lambda-atoms. Proc. SPIE 8773; 87730Z (2013).
[VII] N. Sandor, G. Demeter, D. Dzsotjan, G. P. Djotyan. Matched propagation of Raman-
resonant frequency chirped laser pulses. Under publication in Phys. Rev. A, arXiv:1302.7266
[quant-ph]
Other publications:
[VIII] G. P. Djotyan, J. S. Bakos, Zs. S¨orlei, G. Demeter, N Sandor, D. Dzsotjan, M. A. Kedves,
B. Raczkevi, P. N. Ignacz, and J. Szigeti. Modern Optics and Photonics - Atoms and
11
14. Structured Media, chapter Frequency chirped laser pulses in atomic physics: Coherent
control of inner and translational quantum states, pages 77-91. Singapore: World Scien-
tific, (2010).
[IX] G. P. Djotyan, N. Sandor, J. S. Bakos, and Zs. S¨orlei. Optical storage in quantized media.
Proc. SPIE, 8414: 84140X, (2011).
[X] G. P. Djotyan, J. S. Bakos, Zs. S¨orlei, G. Demeter, N. Sandor, D. Dzsotjan, M. A. Kedves,
and B. Raczkevi. Atom physics with frequency chirped laser pulses. In Proceedings of the
International Conference LASER-PHYSICS-2009, p. 21-24, Astharak, Armenia, (2009).
[XI] G. P. Djotyan, N Sandor, J. S. Bakos, and Zs. S¨orlei. Optical phase information writing
and storage in populations of metastable quantum states. In A Papoyan, E Sharoyan, R
Kostanyan, G Grigoryan, editor, Proceedings of the Conference on Laser Physics-2008,
p. 166-169, Astharak, Armenia, (2009).
[XII] G. P. Djotyan, N. Sandor, J. S. Bakos, Zs. S¨orlei, and D. Dzsotjan Robust optical
information writing in populations of metastable quantum states. In Laser Physics 2008.
40th National Conference Ashtarak, Astharak, Armenia, (2008).
[XIII] G. P. Djotyan, J. S. Bakos, Zs. S¨orlei, D. Dzsotjan, N. Sandor, A. P. Jotyan, and A. A.
Avetisyan All-optical writing and storage of images using multilevel quantum systems and
frequency-chirped laser pulses. In Proceedings of Conference on Laser Physics, Astharak,
Armenia, (2007).
12
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14