1) The document describes a study on the synthesis of waterborne polyurethanes (WPUs) using bio-based polyols from vegetable oils for coating applications. 2) Two commercially available bio-based polyols, a fully renewable fatty dimer polyol and a partially renewable amorphous polyester polyol, were functionalized with isophorone diisocyanate or dicyclohexylmethane-4,4'-diisocyanate in the presence of a ionic chain extender. 3) The functionalized polyols formed stable aqueous dispersions with particle sizes between 60-150 nm and zeta potentials less than -30 mV. Films of the WPUs