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2nd ICOS science conference, September 27th, 2016, Helsinki, Finland
Tracking GHG emissions in a booming city
- urban atmospheric monitoring in Recife, Brazil
Work conducted/supported: F.R. Vogel, J. Staufer, G. Broquet, F. Baron, L. Bregonzio-
Rozier, P.R. Amaral, L. Nunes, S. Souza, L.R. Oliveira, V. Felix, L. Zanutto, F. Velay-
Lasry, M. Chiappero and P. Ciais
Thanks to the LSCE groups (RAMCES, ATC, SATINV and MOSAIC) for their support
Presenting author: F.R. Vogel
The future of urban emissions
The urban population will rise…
… but will the per capita emissions rise – stagnate – decrease?
2nd ICOS science conference, September 27th, 2016, Helsinki, Finland
Relevance of urban scale for GHGs
Cities are major sources of
greenhouse gases (and pollutants)
Cities are active stakeholders and have
ambitions reduction target and mitigation effort
Development of techniques within many projects and now also experience with
routinely operated monitoring network and inversion
Tools to assess GHG emissions
www.C40.org
Tools to assess GHG emissions
www.C40.org
Bottom-up and top-down…
…not bottom-up vs. top-down
Inversion system simplified
Emission inventory/model Transport model Observation system
Paris, France
Recife, Brasil
Atmospheric studies lead by LSCE
Mexico City, Mexico
CO2 - MEGAPARIS
CarboCountCity LOCATION
“Proof-of-concept” “Demonstration” “Scalability”
Paris, France
Recife, Brasil
Atmospheric studies lead by LSCE
Mexico City, Mexico
CO2 - MEGAPARIS
CarboCountCity LOCATION
“Proof-of-concept” “Demonstration” “Scalability”
Paris, France
Toronto, Canada
Recife, Brasil
Atmospheric studies lead by LSCE
Shenzhen, China
Mexico City, Mexico
Frankfurt, Germany
CO2 - MEGAPARIS
CarboCountCity LOCATION
Key “hands-on” scientific collaborations (e.g. PhD students, SOFIE, LoCal)
2nd ICOS science conference, September 27th, 2016, Helsinki, Finland
Key figures:
 Tropical city – 8o3’S, 24o54’W
 Inhabitants 1.6M (city), 3.8M (metro), 6th largest city in Brazil
 High density (7000-8000/km2) similar to Istanbul
 1%/a growth since 1980 ca. –> 300k-400k/decade
RECIFE
Exporting CarboCountCity to South America
2nd ICOS science conference, September 27th, 2016, Helsinki, Finland
Emission inventories for cities - towards common techniques
Toronto, Canada, 0.02ox0.02o
Based on air quality inventory
Collaboration LSCE, ECCC,
UoToronto
Existing inventories for Paris
AIRPARIF, IER and TNO
Here AIRPARIF 2km x 2km
2nd ICOS science conference, September 27th, 2016, Helsinki, Finland
Emission inventories for cities - towards common techniques
8.54%
0.37%
1.72%
34.67%
1.04%
2.30%0.20%
50.61%
0.54%
Emissions by fuel %
LPG - Residential Sector
LPG - Industrial Sector
LPG - Commercial Sector
Fuel Oil - Industrial Sector
Diesel -
Industrial/Agriculture Sector
Diesel -
Commercial/Institutional
Sector
Sector Power Source tCO2 Emissions
Residential Natural Gas 3,151.97
Residential Liquefied Petroleum Gas 131,810.54
Commercial Natural Gas 8,391.53
Commercial Liquefied Petroleum Gas 26,616.05
Commercial Diesel 35,518.47
Industrial Natural Gas 781,408.76
Industrial Diesel 16,119.09
Industrial Fuel Oil 535,354.37
Industrial Liquefied Petroleum Gas 5,649.94
2nd ICOS science conference, September 27th, 2016, Helsinki, Finland
Industrial Consumption by
Sector (2013 year)
Natural Gas Diesel Oil Fuel Oil LPG
106
m3 %
103
m3 %
103
m3 %
103
m3 %
CEMENT 35 0.3% 80 5.9% 18 0.6% 0 0.0%
PIG-IRON AND STEEL 1,159 10.5% 44 3.2% 42 1.5% 31 1.8%
IRON-ALLOYS 25 0.2% 0 0.0% 64 2.3% 0 0.0%
MINING/PELLETIZATION 720 6.5% 467 34.3% 212 7.6% 62 3.7%
NON-FERROUS/OTHER
METALLURGICAL
1,070 9.7% 0 0.0% 1,200 42.9% 72 4.3%
CHEMICAL
2,315 20.9% 27 2.0% 443 15.8% 315
18.8
%
FOODS AND
BEVERAGES
781 7.1% 306 22.5% 207 7.4% 305
18.2
%
TEXTILES 355 3.2% 7 0.5% 48 1.7% 51 3.0%
PAPER AND PULP 919 8.3% 161 11.8% 318 11.4% 98 5.8%
CERAMICS
1,538 13.9% 29 2.1% 130 4.6% 267
15.9
%
OTHERS
2,148 19.4% 240 17.6% 116 4.1% 479
28.5
%
TOTAL INDUSTRIAL
11,06
5 100% 1,361 100% 2,798 100% 1,680 100%
Emission inventories for cities - towards common techniques
Industrial sources in the Recife area
2nd ICOS science conference, September 27th, 2016, Helsinki, Finland
Industrial Consumption by
Sector (2013 year)
Natural Gas Diesel Oil Fuel Oil LPG
106
m3 %
103
m3 %
103
m3 %
103
m3 %
CEMENT 35 0.3% 80 5.9% 18 0.6% 0 0.0%
PIG-IRON AND STEEL 1,159 10.5% 44 3.2% 42 1.5% 31 1.8%
IRON-ALLOYS 25 0.2% 0 0.0% 64 2.3% 0 0.0%
MINING/PELLETIZATION 720 6.5% 467 34.3% 212 7.6% 62 3.7%
NON-FERROUS/OTHER
METALLURGICAL
1,070 9.7% 0 0.0% 1,200 42.9% 72 4.3%
CHEMICAL
2,315 20.9% 27 2.0% 443 15.8% 315
18.8
%
FOODS AND
BEVERAGES
781 7.1% 306 22.5% 207 7.4% 305
18.2
%
TEXTILES 355 3.2% 7 0.5% 48 1.7% 51 3.0%
PAPER AND PULP 919 8.3% 161 11.8% 318 11.4% 98 5.8%
CERAMICS
1,538 13.9% 29 2.1% 130 4.6% 267
15.9
%
OTHERS
2,148 19.4% 240 17.6% 116 4.1% 479
28.5
%
TOTAL INDUSTRIAL
11,06
5 100% 1,361 100% 2,798 100% 1,680 100%
Emission inventories for cities - towards common techniques
Industrial sources in the Recife area
2nd ICOS science conference, September 27th, 2016, Helsinki, Finland
Emission inventories for cities - towards common techniques
41.73%
21.83%
3.40% 5.96%
Road Traffic - Emissions by fuel %
Gasoline
Diesel
Ethanol
Natural Vehicular Gas - NVG
Road map of Recife
Power Source tCO2 Emissions
Gasoline 833.496,29
Diesel 436.062,53
Ethanol 67.977,76
Natural Vehicular Gas 119.095,22
2nd ICOS science conference, September 27th, 2016, Helsinki, Finland
Emission inventories for cities - towards common techniques
41.73%
21.83%
3.40% 5.96%
Road Traffic - Emissions by fuel %
Gasoline
Diesel
Ethanol
Natural Vehicular Gas - NVG
Road map of Recife
Power Source tCO2 Emissions
Gasoline 833.496,29
Diesel 436.062,53
Ethanol 67.977,76
Natural Vehicular Gas 119.095,22
2nd ICOS science conference, September 27th, 2016, Helsinki, Finland
Emission inventories for cities - towards common techniques
Recife, Brazil,1km x 1km,
based on IPCC and GPC
Collaboration LSCE, ARIA tech.
5.52 MtCO2
Toronto, Canada, 0.02ox0.02o
Based on air quality inventory
Collaboration LSCE, UoToronto
Existing inventories for Paris
AIRPARIF, IER and TNO
2nd ICOS science conference, September 27th, 2016, Helsinki, Finland
Emission inventories for cities - towards common techniques
Recife, Brazil,1km x 1km,
based on IPCC and GPC
Collaboration LSCE, ARIA tech.
5.52 MtCO2 +/- ???
Toronto, Canada, 0.02ox0.02o
Based on air quality inventory
Collaboration LSCE, UoToronto
Existing inventories for Paris
AIRPARIF, IER and TNO
2nd ICOS science conference, September 27th, 2016, Helsinki, Finland
Simplified biogenic inputs
Land-use data within the domain
ORCHIDEE
(based on long-term climatology)
Thanks to the MOSAIC team
NEE(gm-2h-1)
Mean daily cycle
2nd ICOS science conference, September 27th, 2016, Helsinki, Finland
Nested domain
0‐6 6‐12 12‐18 18‐24 0‐6
Run 1
Run 2
Run 3
Run 4
Atmospheric modelling
 NCEP-WRF for meteorological forcing
 Horizontal resolution: 27km, 9km, 3km
 Transport model CHIMERE
 Lowest model layers: 5m, 25m, 50m, 90m
 CO2 boundary conditions from MACC2
2nd ICOS science conference, September 27th, 2016, Helsinki, Finland
Atmospheric modelling
2nd ICOS science conference, September 27th, 2016, Helsinki, Finland
Wind roses as tool to design observational network
Recife urban monitoring program
Recife urban monitoring program
Recife urban monitoring program
23:00 01:00 03:00 05:00 07:00 09:00 11:00 13:00
380
400
420
440
460
480
500
520
540
CO2
(ppm)
UTC (HH:mm)
LAFEPE site
 Weekly calibrations using 3 reference gases (390ppm to 510ppm)
 Daily target measurements
 Performance CO2 repeatability better than 0.1ppm
Recife urban monitoring program
Recife urban monitoring program
Dona Lindu
“Coastal station”
 Combine information of wind direction and concentration to understand
source regions!
Lafepe
Dona Lindu
CO2
CH4 CO
Recife urban monitoring program
Lafepe
Dona Lindu
CH4
Recife urban monitoring program
Mangrove park Recife
Large span for potential Mangrove
emissions:
4mgCH4m-2d-1 – 82mgCH4m-2d-1
Sotomayor et al. Puerto Rico
ΔCO2
(Lafepe – Dona Lindu)
Concentration gradient afternoon (13h-15h)
Inversion system simplified
Emission inventory/model Transport model Observation system
Inversion system Recife - first results
 Definition of wind sectors and minimal wind speed
 Data selected for the afternoon window
 Identification of appropriate model level
Inversion system Recife - first results
Inversion system Recife - first results
 No uncertainty reduction for biogenic CO2
 No uncertainty reduction in the morning
 Large uncertainty reduction during daytime
 More balanced biosphere
 More FFCO2 emissions
Inversion system Recife - first results
Inversion system Recife - first results
-0.4
-0.2
0.0
0.2
0.4
0.6
CO2
fluxes(MtCO2
/month)
biogenic
fossil fuel
Prior
emissions
Reference
setup
Relaxed
Uncertainty (2x)
Inversion system Recife - first results
-0.4
-0.2
0.0
0.2
0.4
0.6
CO2
fluxes(MtCO2
/month)
biogenic
fossil fuel
Prior
emissions
Reference
setup
Relaxed
Uncertainty (2x)
 More sensitivity tests conducted for: intake height, assimilation time-
window, correlation of fluxes, …
Summary
- Spatialized emission inventory constructed from statistical data
(cookbook to be released in 2016)
- Successfully installed network and trained local staff
- CO2 (and CO) concentrations in “expected” range and linked to sources
- Very high CH4 concentrations at both sites – Mangrove and canals
- Forward modelling completed (and automated)
- First inversion conducted and first results on fossil fuel CO2 emissions
and bio fluxes (more work planned for 2016)
- Project continuation within LOCATION and IG3IS core activities
Summary
- Spatialized emission inventory constructed from statistical data
(cookbook to be released in 2016)
- Successfully installed network and trained local staff
- CO2 (and CO) concentrations in “expected” range and linked to sources
- Very high CH4 concentrations at both sites – Mangrove and canals
- Forward modelling completed (and automated)
- First inversion conducted and first results on fossil fuel CO2 emissions
and bio fluxes (more work planned for 2016)
- Project continuation within LOCATION and IG3IS core activities

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Tracking GHG emissions in a booming city -urban atmospheric monitoring in Recife, Brazil

  • 1. 2nd ICOS science conference, September 27th, 2016, Helsinki, Finland Tracking GHG emissions in a booming city - urban atmospheric monitoring in Recife, Brazil Work conducted/supported: F.R. Vogel, J. Staufer, G. Broquet, F. Baron, L. Bregonzio- Rozier, P.R. Amaral, L. Nunes, S. Souza, L.R. Oliveira, V. Felix, L. Zanutto, F. Velay- Lasry, M. Chiappero and P. Ciais Thanks to the LSCE groups (RAMCES, ATC, SATINV and MOSAIC) for their support Presenting author: F.R. Vogel
  • 2. The future of urban emissions The urban population will rise… … but will the per capita emissions rise – stagnate – decrease?
  • 3. 2nd ICOS science conference, September 27th, 2016, Helsinki, Finland Relevance of urban scale for GHGs Cities are major sources of greenhouse gases (and pollutants) Cities are active stakeholders and have ambitions reduction target and mitigation effort Development of techniques within many projects and now also experience with routinely operated monitoring network and inversion
  • 4. Tools to assess GHG emissions www.C40.org
  • 5. Tools to assess GHG emissions www.C40.org Bottom-up and top-down… …not bottom-up vs. top-down
  • 6. Inversion system simplified Emission inventory/model Transport model Observation system
  • 7. Paris, France Recife, Brasil Atmospheric studies lead by LSCE Mexico City, Mexico CO2 - MEGAPARIS CarboCountCity LOCATION “Proof-of-concept” “Demonstration” “Scalability”
  • 8. Paris, France Recife, Brasil Atmospheric studies lead by LSCE Mexico City, Mexico CO2 - MEGAPARIS CarboCountCity LOCATION “Proof-of-concept” “Demonstration” “Scalability”
  • 9. Paris, France Toronto, Canada Recife, Brasil Atmospheric studies lead by LSCE Shenzhen, China Mexico City, Mexico Frankfurt, Germany CO2 - MEGAPARIS CarboCountCity LOCATION Key “hands-on” scientific collaborations (e.g. PhD students, SOFIE, LoCal)
  • 10. 2nd ICOS science conference, September 27th, 2016, Helsinki, Finland Key figures:  Tropical city – 8o3’S, 24o54’W  Inhabitants 1.6M (city), 3.8M (metro), 6th largest city in Brazil  High density (7000-8000/km2) similar to Istanbul  1%/a growth since 1980 ca. –> 300k-400k/decade RECIFE Exporting CarboCountCity to South America
  • 11. 2nd ICOS science conference, September 27th, 2016, Helsinki, Finland Emission inventories for cities - towards common techniques Toronto, Canada, 0.02ox0.02o Based on air quality inventory Collaboration LSCE, ECCC, UoToronto Existing inventories for Paris AIRPARIF, IER and TNO Here AIRPARIF 2km x 2km
  • 12. 2nd ICOS science conference, September 27th, 2016, Helsinki, Finland Emission inventories for cities - towards common techniques 8.54% 0.37% 1.72% 34.67% 1.04% 2.30%0.20% 50.61% 0.54% Emissions by fuel % LPG - Residential Sector LPG - Industrial Sector LPG - Commercial Sector Fuel Oil - Industrial Sector Diesel - Industrial/Agriculture Sector Diesel - Commercial/Institutional Sector Sector Power Source tCO2 Emissions Residential Natural Gas 3,151.97 Residential Liquefied Petroleum Gas 131,810.54 Commercial Natural Gas 8,391.53 Commercial Liquefied Petroleum Gas 26,616.05 Commercial Diesel 35,518.47 Industrial Natural Gas 781,408.76 Industrial Diesel 16,119.09 Industrial Fuel Oil 535,354.37 Industrial Liquefied Petroleum Gas 5,649.94
  • 13. 2nd ICOS science conference, September 27th, 2016, Helsinki, Finland Industrial Consumption by Sector (2013 year) Natural Gas Diesel Oil Fuel Oil LPG 106 m3 % 103 m3 % 103 m3 % 103 m3 % CEMENT 35 0.3% 80 5.9% 18 0.6% 0 0.0% PIG-IRON AND STEEL 1,159 10.5% 44 3.2% 42 1.5% 31 1.8% IRON-ALLOYS 25 0.2% 0 0.0% 64 2.3% 0 0.0% MINING/PELLETIZATION 720 6.5% 467 34.3% 212 7.6% 62 3.7% NON-FERROUS/OTHER METALLURGICAL 1,070 9.7% 0 0.0% 1,200 42.9% 72 4.3% CHEMICAL 2,315 20.9% 27 2.0% 443 15.8% 315 18.8 % FOODS AND BEVERAGES 781 7.1% 306 22.5% 207 7.4% 305 18.2 % TEXTILES 355 3.2% 7 0.5% 48 1.7% 51 3.0% PAPER AND PULP 919 8.3% 161 11.8% 318 11.4% 98 5.8% CERAMICS 1,538 13.9% 29 2.1% 130 4.6% 267 15.9 % OTHERS 2,148 19.4% 240 17.6% 116 4.1% 479 28.5 % TOTAL INDUSTRIAL 11,06 5 100% 1,361 100% 2,798 100% 1,680 100% Emission inventories for cities - towards common techniques Industrial sources in the Recife area
  • 14. 2nd ICOS science conference, September 27th, 2016, Helsinki, Finland Industrial Consumption by Sector (2013 year) Natural Gas Diesel Oil Fuel Oil LPG 106 m3 % 103 m3 % 103 m3 % 103 m3 % CEMENT 35 0.3% 80 5.9% 18 0.6% 0 0.0% PIG-IRON AND STEEL 1,159 10.5% 44 3.2% 42 1.5% 31 1.8% IRON-ALLOYS 25 0.2% 0 0.0% 64 2.3% 0 0.0% MINING/PELLETIZATION 720 6.5% 467 34.3% 212 7.6% 62 3.7% NON-FERROUS/OTHER METALLURGICAL 1,070 9.7% 0 0.0% 1,200 42.9% 72 4.3% CHEMICAL 2,315 20.9% 27 2.0% 443 15.8% 315 18.8 % FOODS AND BEVERAGES 781 7.1% 306 22.5% 207 7.4% 305 18.2 % TEXTILES 355 3.2% 7 0.5% 48 1.7% 51 3.0% PAPER AND PULP 919 8.3% 161 11.8% 318 11.4% 98 5.8% CERAMICS 1,538 13.9% 29 2.1% 130 4.6% 267 15.9 % OTHERS 2,148 19.4% 240 17.6% 116 4.1% 479 28.5 % TOTAL INDUSTRIAL 11,06 5 100% 1,361 100% 2,798 100% 1,680 100% Emission inventories for cities - towards common techniques Industrial sources in the Recife area
  • 15. 2nd ICOS science conference, September 27th, 2016, Helsinki, Finland Emission inventories for cities - towards common techniques 41.73% 21.83% 3.40% 5.96% Road Traffic - Emissions by fuel % Gasoline Diesel Ethanol Natural Vehicular Gas - NVG Road map of Recife Power Source tCO2 Emissions Gasoline 833.496,29 Diesel 436.062,53 Ethanol 67.977,76 Natural Vehicular Gas 119.095,22
  • 16. 2nd ICOS science conference, September 27th, 2016, Helsinki, Finland Emission inventories for cities - towards common techniques 41.73% 21.83% 3.40% 5.96% Road Traffic - Emissions by fuel % Gasoline Diesel Ethanol Natural Vehicular Gas - NVG Road map of Recife Power Source tCO2 Emissions Gasoline 833.496,29 Diesel 436.062,53 Ethanol 67.977,76 Natural Vehicular Gas 119.095,22
  • 17. 2nd ICOS science conference, September 27th, 2016, Helsinki, Finland Emission inventories for cities - towards common techniques Recife, Brazil,1km x 1km, based on IPCC and GPC Collaboration LSCE, ARIA tech. 5.52 MtCO2 Toronto, Canada, 0.02ox0.02o Based on air quality inventory Collaboration LSCE, UoToronto Existing inventories for Paris AIRPARIF, IER and TNO
  • 18. 2nd ICOS science conference, September 27th, 2016, Helsinki, Finland Emission inventories for cities - towards common techniques Recife, Brazil,1km x 1km, based on IPCC and GPC Collaboration LSCE, ARIA tech. 5.52 MtCO2 +/- ??? Toronto, Canada, 0.02ox0.02o Based on air quality inventory Collaboration LSCE, UoToronto Existing inventories for Paris AIRPARIF, IER and TNO
  • 19. 2nd ICOS science conference, September 27th, 2016, Helsinki, Finland Simplified biogenic inputs Land-use data within the domain ORCHIDEE (based on long-term climatology) Thanks to the MOSAIC team NEE(gm-2h-1) Mean daily cycle
  • 20. 2nd ICOS science conference, September 27th, 2016, Helsinki, Finland Nested domain 0‐6 6‐12 12‐18 18‐24 0‐6 Run 1 Run 2 Run 3 Run 4 Atmospheric modelling  NCEP-WRF for meteorological forcing  Horizontal resolution: 27km, 9km, 3km  Transport model CHIMERE  Lowest model layers: 5m, 25m, 50m, 90m  CO2 boundary conditions from MACC2
  • 21. 2nd ICOS science conference, September 27th, 2016, Helsinki, Finland Atmospheric modelling
  • 22. 2nd ICOS science conference, September 27th, 2016, Helsinki, Finland Wind roses as tool to design observational network
  • 25. Recife urban monitoring program 23:00 01:00 03:00 05:00 07:00 09:00 11:00 13:00 380 400 420 440 460 480 500 520 540 CO2 (ppm) UTC (HH:mm) LAFEPE site  Weekly calibrations using 3 reference gases (390ppm to 510ppm)  Daily target measurements  Performance CO2 repeatability better than 0.1ppm
  • 27. Recife urban monitoring program Dona Lindu “Coastal station”  Combine information of wind direction and concentration to understand source regions!
  • 28. Lafepe Dona Lindu CO2 CH4 CO Recife urban monitoring program
  • 29. Lafepe Dona Lindu CH4 Recife urban monitoring program Mangrove park Recife Large span for potential Mangrove emissions: 4mgCH4m-2d-1 – 82mgCH4m-2d-1 Sotomayor et al. Puerto Rico
  • 30. ΔCO2 (Lafepe – Dona Lindu) Concentration gradient afternoon (13h-15h)
  • 31. Inversion system simplified Emission inventory/model Transport model Observation system
  • 32. Inversion system Recife - first results  Definition of wind sectors and minimal wind speed  Data selected for the afternoon window  Identification of appropriate model level
  • 33. Inversion system Recife - first results
  • 34. Inversion system Recife - first results  No uncertainty reduction for biogenic CO2  No uncertainty reduction in the morning  Large uncertainty reduction during daytime  More balanced biosphere  More FFCO2 emissions
  • 35. Inversion system Recife - first results
  • 36. Inversion system Recife - first results -0.4 -0.2 0.0 0.2 0.4 0.6 CO2 fluxes(MtCO2 /month) biogenic fossil fuel Prior emissions Reference setup Relaxed Uncertainty (2x)
  • 37. Inversion system Recife - first results -0.4 -0.2 0.0 0.2 0.4 0.6 CO2 fluxes(MtCO2 /month) biogenic fossil fuel Prior emissions Reference setup Relaxed Uncertainty (2x)  More sensitivity tests conducted for: intake height, assimilation time- window, correlation of fluxes, …
  • 38. Summary - Spatialized emission inventory constructed from statistical data (cookbook to be released in 2016) - Successfully installed network and trained local staff - CO2 (and CO) concentrations in “expected” range and linked to sources - Very high CH4 concentrations at both sites – Mangrove and canals - Forward modelling completed (and automated) - First inversion conducted and first results on fossil fuel CO2 emissions and bio fluxes (more work planned for 2016) - Project continuation within LOCATION and IG3IS core activities
  • 39. Summary - Spatialized emission inventory constructed from statistical data (cookbook to be released in 2016) - Successfully installed network and trained local staff - CO2 (and CO) concentrations in “expected” range and linked to sources - Very high CH4 concentrations at both sites – Mangrove and canals - Forward modelling completed (and automated) - First inversion conducted and first results on fossil fuel CO2 emissions and bio fluxes (more work planned for 2016) - Project continuation within LOCATION and IG3IS core activities