This document summarizes a project on using metal-organic frameworks (MOFs) for post-combustion carbon capture. It discusses (1) developing MOF materials with high CO2 selectivity and capacity through scale-up synthesis and formulation methods, (2) testing MOF performance for CO2/N2 separation through breakthrough experiments using a dual-piston vacuum swing adsorption system, and (3) optimizing the vacuum pressure swing adsorption process through modeling. The project involves partners from the University of Edinburgh, SINTEF Materials and Chemistry, and the Centre for Research and Technology. Some results showed the successful formulation of MOFs into stable spheres using an alginate method and their high CO2 ad