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Noise Resilience of Variational Quantum
Compiling
Kunal Sharma
GRA, Los Alamos National Lab
Phd Candidate, Louisiana State University
ksharm7@lsu.edu
APS March Meeting 2020
Joint work with
Sumeet Khatri, Marco Cerezo, and Patrick J. Coles
New Journal of Physics, arXiv:1908.04416, LA-UR-19-28095
1 / 17
Main Results
Noise resilience of Variational Quantum Compiling (VQC)
• Measurement noise (readout error).
• Incoherent gate noise and decoherence processes: Pauli
channels and non-unital Pauli channels.
Implementations of VQC on IBM’s noisy quantum simulator
• Quantum Fourier transform (QFT)
• Toffoli
• W-state preparation
Noise resilience in every case.
2 / 17
Background
Applications of quantum computing:
• Quantum simulation [Fey99].
• Factoring [Sho99].
• Optimization [Gro96].
3 / 17
Background
Noisy intermediate-scale quantum (NISQ) computers [Pre12]
Limitations of NISQ devices:
• Limited number of qubits.
• Limited connectivity between qubits.
• Restricted (hardware-specific) gate alphabets.
• Limited circuit depth due to noise.
4 / 17
Background
Noisy intermediate-scale quantum (NISQ) computers [Pre12]
Limitations of NISQ devices:
• Limited number of qubits.
• Limited connectivity between qubits.
• Restricted (hardware-specific) gate alphabets.
• Limited circuit depth due to noise.
What can be done with NISQ devices?
• Error mitigation [TBG17, LJF+17, SCC18, MBJA+19].
• Variational hybrid quantum-classical algorithm [MRBAG16].
• Inherent noise resilience to certain noise models
[MRBAG16, SKCC20].
4 / 17
Variational Quantum Compiling (VQC)
Quantum compiler
Conversion of an high-level algorithm into a lower-level machine
code [CFM17, HSST18, BDB+18].
5 / 17
Variational Quantum Compiling (VQC)
Main goal of VQC [KLP+19, JB18, HSNF18]
Target unitary = U
Trainable unitary = V
• Full unitary matrix compiling:
Compile U by using V (k, α) that has approximately the same
action as U on any given input state.
α: continuous, k: discrete
• Fixed input state compiling:
U|ψ0 = V |ψ0 or U |0 = V |0 .
5 / 17
Variational quantum compiling (VQC)
Applications of VQC:
• Algorithmic depth compression.
• Device specific compilation.
• Variational fast forwarding for quantum simulation [CHI+19].
6 / 17
Quantum-Classical Hybrid Algorithm
Classical computers
• Optimization.
• Quantum simulation. 
Noisy Quantum computers
• Quantum simulation.
• Optimization. 
7 / 17
Variational quantum compiling
Full unitary matrix compiling
Target unitary U
Trainable unitary V
Questions:
1. Cost function?
2. Task for a quantum computer?
3. Task for a classical computer?
4. How to perform optimization?
8 / 17
Variational quantum compiling
Quantum Computer
Input: U
Output: Vkopt(αopt)
Continuous
parameter
optimizer over α
Structure
parameter
optimizer over k
Classical Computer
If α optimal
If α not optimal
Gate
sequence
Vk(α)
Cost
C(U, Vk(α))
|0 H •
U
• H
|0 H • • H
...
|0 H • • H
|0
V ∗
|0
...
|0
HST
|0 H •
U
• H
|0 H •
...
|0 H •
|0
V ∗
|0
...
|0
LHST
OR
OR
(a) Variable structure approach
⊕
⊕
⊕
⊕
Fixed
structure
Variable
structure
with L = 4
⊕
⊕
Optimal L = 5
compilation
(b) Fixed structure approach
Ansatz with
each layer
parameterized by
two-qubit gates
Two
layers
Figure 1: Outline for Full Unitary Matrix Compiling [KLP+19].
9 / 17
Cost function for VQC
Lorem ipsum Lorem ipsum
Figure 2: a) The Hilbert-Schmidt Test (HST). b) The Local Hilbert-Schmidt Test
(LHST).
CHST = 1 − FHST = 1 − | Tr(V †
U)|2
/d2
,
CLHST = 1 − FLHST = 1 −
1
n
n
j=1
F
(j)
LHST.
CHST might exhibit barren plateau [MBS+18, CSV+20].
10 / 17
Cost function for FUMC
Global Cost Function
CHST = 1 − FHST = 1 − | Tr(V †
U)|2
/d2
,
CHST =
d + 1
d
(1 − F(U, V )).
Faithfulness of CLHST:
CLHST ≤ CHST ≤ nCLHST.
• Cost functions are zero iff U = V (up to global phase).
• Efficient to compute on a quantum computer.
11 / 17
Noise models
Pauli noise
• E(XkZl ) = ckl
XkZl .
• T2 process as a special case (dephasing channel).
• Depolarizing noise ρ → pρ + (1 − p)I/2n.
Non-unital Pauli noise
• E(I) = I + (k,l)=(0,0)
dkl
XkZl .
• For (k, l) = (0, 0), E(XkZl ) = ckl
XkZl .
• T1 process as a special case (amplitude damping channel).
Measurement noise
Ideal: {P0 = |0 0|, P1 = |1 1|}.
Noisy:{P0, P1} with P0 = p00|0 0| + p01|1 1| and
P1 = p10|0 0| + p11|1 1|, where p00 + p10 = 1, p01 + p11 = 1. 12 / 17
Main results: Optimal parameter resilience
Lorem ipsum
Figure 3: Noise Model 1. PGN = Pauli gate noise, MN = Measurement noise,
PN=Pauli noise, DN = depolarizing noise, NUPN = non-unital Pauli noise.
13 / 17
Main results: Optimal parameter resilience
• Quantum circuit = QC.
• Cost function = CQC(V ).
• Noisy cost function (QC is run in the presence of some noise
process N) = CQC(V ).
Optimal solutions:
Vopt
d = {V ∈ Vd : CQC(V ) = min
V ∈Vd
CQC(V )} ,
Vopt
d = {V ∈ Vd : CQC(V ) = min
V ∈Vd
CQC(V )} .
CQC(V ) exhibits strong-optimal parameter resilience to N if
Vopt
d = Vopt
d .
13 / 17
Main results: Optimal parameter resilience
Lorem ipsum
Figure 3: Noise Model 1. PGN = Pauli gate noise, MN = Measurement noise,
PN=Pauli noise, DN = depolarizing noise, NUPN = non-unital Pauli noise.
13 / 17
Implementations
Figure 4: (a) The dressed CNOT is composed of a CNOT preceded and followed by
single-qubit gates Vk (αk ). (b) Two layers of the alternating-pair ansatz in the case of
four qubits. Each layer is composed of dressed CNOTs acting on alternating pairs of
neighboring qubits. (c) Schematic representation of the target-inspired ansatz. In this
approach, the gate sequence of dressed CNOTs is obtained from the gate sequence of
the target unitary U.
Vk(αk) = e−iαk,3σz /2
e−iαk,2σy /2
e−iαk,1σz /2
.
14 / 17
Implementations
Figure 5: Quantum circuits for: (a) Toffoli Gate, (b) Three-qubit Quantum Fourier
Transform, and (c) Three-qubit W-state preparation. Here, Rm stands for the
controlled phase gate with a phase shift of φ = e2πi/2m
. For the three-qubit W-state
preparation circuit we have β1 = (2 arccos( 1/3), 0, 0) and β2 = (π/2, 0, 0).
Vk(αk) = e−iαk,3σz /2
e−iαk,2σy /2
e−iαk,1σz /2
.
15 / 17
Implementations
Figure 6: VQC implementations: the Toffoli gate (top) and three-qubit QFT
(bottom). The ansatz for V (α) is: (a) one layer of the alternating-pair (AP) ansatz,
(b) two layers of the AP ansatz, (c) the target-inspired ansatz. The blue and green
curves respectively plot the values of CHST and CLHST obtained by noisy training. The
green and pink curves respectively plot the values of CHST and CLHST evaluated at the
variational parameters α obtained from the noisy optimization of V (α). The blue and
red dashed lines in (a) and (b) correspond to the minimum value of CHST and CLHST,
respectively, determined by optimizing V (α) in a noise-free environment.
16 / 17
Conclusion
Noise resilience of Variational Quantum Compiling (VQC)
• Measurement noise (readout error).
• Incoherent gate noise and decoherence processes: Pauli
channels and non-unital Pauli channels.
Future directions
• Practically useful applications of VQC with a NISQ device.
• Noise resilience of other variational quantum algorithms.
Example: VQE.
17 / 17
[BDB+18] K. E. C. Booth, M. Do, J. C. Beck, E. Rieffel,
D. Venturelli, and J. Frank. Comparing and
integrating constraint programming and
temporal planning for quantum circuit
compilation. arXiv:1803.06775, 2018.
[CFM17] F. T. Chong, D. Franklin, and M. Martonosi.
Programming languages and compiler design for
realistic quantum hardware. Nature,
549(7671):180, 2017.
[CHI+19] Cristina Cirstoiu, Zoe Holmes, Joseph Iosue, Lukasz
Cincio, Patrick J Coles, and Andrew Sornborger.
Variational fast forwarding for quantum
simulation beyond the coherence time. arXiv
preprint arXiv:1910.04292, 2019.
17 / 17
[CSV+20] M Cerezo, Akira Sone, Tyler Volkoff, Lukasz Cincio,
and Patrick J Coles. Cost-function-dependent
barren plateaus in shallow quantum neural
networks. arXiv preprint arXiv:2001.00550, 2020.
[Fey99] Richard P Feynman. Simulating physics with
computers. Int. J. Theor. Phys, 21(6/7), 1999.
[Gro96] Lov K Grover. A fast quantum mechanical
algorithm for database search. In Proceedings of
the twenty-eighth annual ACM symposium on Theory
of computing, pages 212–219, 1996.
[HSNF18] Kentaro Heya, Yasunari Suzuki, Yasunobu Nakamura,
and Keisuke Fujii. Variational quantum gate
optimization. arXiv preprint arXiv:1810.12745, 2018.
[HSST18] Thomas H¨aner, Damian S Steiger, Krysta Svore, and
Matthias Troyer. A software methodology for
17 / 17
compiling quantum programs. Quantum Science
and Technology, 3(2):020501, 2018.
[JB18] T. Jones and S. C. Benjamin. Quantum
compilation and circuit optimisation via energy
dissipation. arXiv:1811.03147, 2018.
[KLP+19] Sumeet Khatri, Ryan LaRose, Alexander Poremba,
Lukasz Cincio, Andrew T. Sornborger, and Patrick J.
Coles. Quantum-assisted quantum compiling.
Quantum, 3:140, May 2019.
[LJF+17] N. M. Linke, S. Johri, C. Figgatt, K. A. Landsman,
A. Y. Matsuura, and C. Monroe. Measuring the
R´enyi entropy of a two-site Fermi-Hubbard
model on a trapped ion quantum computer.
arXiv:1712.08581, 2017.
17 / 17
[MBJA+19] Prakash Murali, Jonathan M Baker, Ali
Javadi-Abhari, Frederic T Chong, and Margaret
Martonosi. Noise-adaptive compiler mappings for
noisy intermediate-scale quantum computers. In
Proceedings of the Twenty-Fourth International
Conference on Architectural Support for
Programming Languages and Operating Systems,
pages 1015–1029. ACM, 2019.
[MBS+18] J. R. McClean, S. Boixo, V. N. Smelyanskiy,
R. Babbush, and H. Neven. Barren plateaus in
quantum neural network training landscapes.
Nature Communications, 9:4812, Nov 2018.
[MRBAG16] J. R. McClean, J. Romero, R. Babbush, and
A. Aspuru-Guzik. The theory of variational hybrid
quantum-classical algorithms. New Journal of
Physics, 18(2):023023, 2016.
17 / 17
[Pre12] J. Preskill. Quantum computing and the
entanglement frontier. arXiv:1203.5813, 2012.
[SCC18] Yigit Subasi, Lukasz Cincio, and Patrick J Coles.
Entanglement spectroscopy with a depth-two
quantum circuit. Journal of Physics A:
Mathematical and Theoretical, 2018.
[Sho99] Peter W Shor. Polynomial-time algorithms for
prime factorization and discrete logarithms on a
quantum computer. SIAM review, 41(2):303–332,
1999.
[SKCC20] Kunal Sharma, Sumeet Khatri, Marco Cerezo, and
Patrick Coles. Noise resilience of variational
quantum compiling. New Journal of Physics, 2020.
17 / 17
[TBG17] K. Temme, S. Bravyi, and J. M. Gambetta. Error
mitigation for short-depth quantum circuits.
Physical Review Letters, 119(18):180509, 2017.
17 / 17

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Noise Resilience of Variational Quantum Compiling

  • 1. Noise Resilience of Variational Quantum Compiling Kunal Sharma GRA, Los Alamos National Lab Phd Candidate, Louisiana State University ksharm7@lsu.edu APS March Meeting 2020 Joint work with Sumeet Khatri, Marco Cerezo, and Patrick J. Coles New Journal of Physics, arXiv:1908.04416, LA-UR-19-28095 1 / 17
  • 2. Main Results Noise resilience of Variational Quantum Compiling (VQC) • Measurement noise (readout error). • Incoherent gate noise and decoherence processes: Pauli channels and non-unital Pauli channels. Implementations of VQC on IBM’s noisy quantum simulator • Quantum Fourier transform (QFT) • Toffoli • W-state preparation Noise resilience in every case. 2 / 17
  • 3. Background Applications of quantum computing: • Quantum simulation [Fey99]. • Factoring [Sho99]. • Optimization [Gro96]. 3 / 17
  • 4. Background Noisy intermediate-scale quantum (NISQ) computers [Pre12] Limitations of NISQ devices: • Limited number of qubits. • Limited connectivity between qubits. • Restricted (hardware-specific) gate alphabets. • Limited circuit depth due to noise. 4 / 17
  • 5. Background Noisy intermediate-scale quantum (NISQ) computers [Pre12] Limitations of NISQ devices: • Limited number of qubits. • Limited connectivity between qubits. • Restricted (hardware-specific) gate alphabets. • Limited circuit depth due to noise. What can be done with NISQ devices? • Error mitigation [TBG17, LJF+17, SCC18, MBJA+19]. • Variational hybrid quantum-classical algorithm [MRBAG16]. • Inherent noise resilience to certain noise models [MRBAG16, SKCC20]. 4 / 17
  • 6. Variational Quantum Compiling (VQC) Quantum compiler Conversion of an high-level algorithm into a lower-level machine code [CFM17, HSST18, BDB+18]. 5 / 17
  • 7. Variational Quantum Compiling (VQC) Main goal of VQC [KLP+19, JB18, HSNF18] Target unitary = U Trainable unitary = V • Full unitary matrix compiling: Compile U by using V (k, α) that has approximately the same action as U on any given input state. α: continuous, k: discrete • Fixed input state compiling: U|ψ0 = V |ψ0 or U |0 = V |0 . 5 / 17
  • 8. Variational quantum compiling (VQC) Applications of VQC: • Algorithmic depth compression. • Device specific compilation. • Variational fast forwarding for quantum simulation [CHI+19]. 6 / 17
  • 9. Quantum-Classical Hybrid Algorithm Classical computers • Optimization. • Quantum simulation. Noisy Quantum computers • Quantum simulation. • Optimization. 7 / 17
  • 10. Variational quantum compiling Full unitary matrix compiling Target unitary U Trainable unitary V Questions: 1. Cost function? 2. Task for a quantum computer? 3. Task for a classical computer? 4. How to perform optimization? 8 / 17
  • 11. Variational quantum compiling Quantum Computer Input: U Output: Vkopt(αopt) Continuous parameter optimizer over α Structure parameter optimizer over k Classical Computer If α optimal If α not optimal Gate sequence Vk(α) Cost C(U, Vk(α)) |0 H • U • H |0 H • • H ... |0 H • • H |0 V ∗ |0 ... |0 HST |0 H • U • H |0 H • ... |0 H • |0 V ∗ |0 ... |0 LHST OR OR (a) Variable structure approach ⊕ ⊕ ⊕ ⊕ Fixed structure Variable structure with L = 4 ⊕ ⊕ Optimal L = 5 compilation (b) Fixed structure approach Ansatz with each layer parameterized by two-qubit gates Two layers Figure 1: Outline for Full Unitary Matrix Compiling [KLP+19]. 9 / 17
  • 12. Cost function for VQC Lorem ipsum Lorem ipsum Figure 2: a) The Hilbert-Schmidt Test (HST). b) The Local Hilbert-Schmidt Test (LHST). CHST = 1 − FHST = 1 − | Tr(V † U)|2 /d2 , CLHST = 1 − FLHST = 1 − 1 n n j=1 F (j) LHST. CHST might exhibit barren plateau [MBS+18, CSV+20]. 10 / 17
  • 13. Cost function for FUMC Global Cost Function CHST = 1 − FHST = 1 − | Tr(V † U)|2 /d2 , CHST = d + 1 d (1 − F(U, V )). Faithfulness of CLHST: CLHST ≤ CHST ≤ nCLHST. • Cost functions are zero iff U = V (up to global phase). • Efficient to compute on a quantum computer. 11 / 17
  • 14. Noise models Pauli noise • E(XkZl ) = ckl XkZl . • T2 process as a special case (dephasing channel). • Depolarizing noise ρ → pρ + (1 − p)I/2n. Non-unital Pauli noise • E(I) = I + (k,l)=(0,0) dkl XkZl . • For (k, l) = (0, 0), E(XkZl ) = ckl XkZl . • T1 process as a special case (amplitude damping channel). Measurement noise Ideal: {P0 = |0 0|, P1 = |1 1|}. Noisy:{P0, P1} with P0 = p00|0 0| + p01|1 1| and P1 = p10|0 0| + p11|1 1|, where p00 + p10 = 1, p01 + p11 = 1. 12 / 17
  • 15. Main results: Optimal parameter resilience Lorem ipsum Figure 3: Noise Model 1. PGN = Pauli gate noise, MN = Measurement noise, PN=Pauli noise, DN = depolarizing noise, NUPN = non-unital Pauli noise. 13 / 17
  • 16. Main results: Optimal parameter resilience • Quantum circuit = QC. • Cost function = CQC(V ). • Noisy cost function (QC is run in the presence of some noise process N) = CQC(V ). Optimal solutions: Vopt d = {V ∈ Vd : CQC(V ) = min V ∈Vd CQC(V )} , Vopt d = {V ∈ Vd : CQC(V ) = min V ∈Vd CQC(V )} . CQC(V ) exhibits strong-optimal parameter resilience to N if Vopt d = Vopt d . 13 / 17
  • 17. Main results: Optimal parameter resilience Lorem ipsum Figure 3: Noise Model 1. PGN = Pauli gate noise, MN = Measurement noise, PN=Pauli noise, DN = depolarizing noise, NUPN = non-unital Pauli noise. 13 / 17
  • 18. Implementations Figure 4: (a) The dressed CNOT is composed of a CNOT preceded and followed by single-qubit gates Vk (αk ). (b) Two layers of the alternating-pair ansatz in the case of four qubits. Each layer is composed of dressed CNOTs acting on alternating pairs of neighboring qubits. (c) Schematic representation of the target-inspired ansatz. In this approach, the gate sequence of dressed CNOTs is obtained from the gate sequence of the target unitary U. Vk(αk) = e−iαk,3σz /2 e−iαk,2σy /2 e−iαk,1σz /2 . 14 / 17
  • 19. Implementations Figure 5: Quantum circuits for: (a) Toffoli Gate, (b) Three-qubit Quantum Fourier Transform, and (c) Three-qubit W-state preparation. Here, Rm stands for the controlled phase gate with a phase shift of φ = e2πi/2m . For the three-qubit W-state preparation circuit we have β1 = (2 arccos( 1/3), 0, 0) and β2 = (π/2, 0, 0). Vk(αk) = e−iαk,3σz /2 e−iαk,2σy /2 e−iαk,1σz /2 . 15 / 17
  • 20. Implementations Figure 6: VQC implementations: the Toffoli gate (top) and three-qubit QFT (bottom). The ansatz for V (α) is: (a) one layer of the alternating-pair (AP) ansatz, (b) two layers of the AP ansatz, (c) the target-inspired ansatz. The blue and green curves respectively plot the values of CHST and CLHST obtained by noisy training. The green and pink curves respectively plot the values of CHST and CLHST evaluated at the variational parameters α obtained from the noisy optimization of V (α). The blue and red dashed lines in (a) and (b) correspond to the minimum value of CHST and CLHST, respectively, determined by optimizing V (α) in a noise-free environment. 16 / 17
  • 21. Conclusion Noise resilience of Variational Quantum Compiling (VQC) • Measurement noise (readout error). • Incoherent gate noise and decoherence processes: Pauli channels and non-unital Pauli channels. Future directions • Practically useful applications of VQC with a NISQ device. • Noise resilience of other variational quantum algorithms. Example: VQE. 17 / 17
  • 22. [BDB+18] K. E. C. Booth, M. Do, J. C. Beck, E. Rieffel, D. Venturelli, and J. Frank. Comparing and integrating constraint programming and temporal planning for quantum circuit compilation. arXiv:1803.06775, 2018. [CFM17] F. T. Chong, D. Franklin, and M. Martonosi. Programming languages and compiler design for realistic quantum hardware. Nature, 549(7671):180, 2017. [CHI+19] Cristina Cirstoiu, Zoe Holmes, Joseph Iosue, Lukasz Cincio, Patrick J Coles, and Andrew Sornborger. Variational fast forwarding for quantum simulation beyond the coherence time. arXiv preprint arXiv:1910.04292, 2019. 17 / 17
  • 23. [CSV+20] M Cerezo, Akira Sone, Tyler Volkoff, Lukasz Cincio, and Patrick J Coles. Cost-function-dependent barren plateaus in shallow quantum neural networks. arXiv preprint arXiv:2001.00550, 2020. [Fey99] Richard P Feynman. Simulating physics with computers. Int. J. Theor. Phys, 21(6/7), 1999. [Gro96] Lov K Grover. A fast quantum mechanical algorithm for database search. In Proceedings of the twenty-eighth annual ACM symposium on Theory of computing, pages 212–219, 1996. [HSNF18] Kentaro Heya, Yasunari Suzuki, Yasunobu Nakamura, and Keisuke Fujii. Variational quantum gate optimization. arXiv preprint arXiv:1810.12745, 2018. [HSST18] Thomas H¨aner, Damian S Steiger, Krysta Svore, and Matthias Troyer. A software methodology for 17 / 17
  • 24. compiling quantum programs. Quantum Science and Technology, 3(2):020501, 2018. [JB18] T. Jones and S. C. Benjamin. Quantum compilation and circuit optimisation via energy dissipation. arXiv:1811.03147, 2018. [KLP+19] Sumeet Khatri, Ryan LaRose, Alexander Poremba, Lukasz Cincio, Andrew T. Sornborger, and Patrick J. Coles. Quantum-assisted quantum compiling. Quantum, 3:140, May 2019. [LJF+17] N. M. Linke, S. Johri, C. Figgatt, K. A. Landsman, A. Y. Matsuura, and C. Monroe. Measuring the R´enyi entropy of a two-site Fermi-Hubbard model on a trapped ion quantum computer. arXiv:1712.08581, 2017. 17 / 17
  • 25. [MBJA+19] Prakash Murali, Jonathan M Baker, Ali Javadi-Abhari, Frederic T Chong, and Margaret Martonosi. Noise-adaptive compiler mappings for noisy intermediate-scale quantum computers. In Proceedings of the Twenty-Fourth International Conference on Architectural Support for Programming Languages and Operating Systems, pages 1015–1029. ACM, 2019. [MBS+18] J. R. McClean, S. Boixo, V. N. Smelyanskiy, R. Babbush, and H. Neven. Barren plateaus in quantum neural network training landscapes. Nature Communications, 9:4812, Nov 2018. [MRBAG16] J. R. McClean, J. Romero, R. Babbush, and A. Aspuru-Guzik. The theory of variational hybrid quantum-classical algorithms. New Journal of Physics, 18(2):023023, 2016. 17 / 17
  • 26. [Pre12] J. Preskill. Quantum computing and the entanglement frontier. arXiv:1203.5813, 2012. [SCC18] Yigit Subasi, Lukasz Cincio, and Patrick J Coles. Entanglement spectroscopy with a depth-two quantum circuit. Journal of Physics A: Mathematical and Theoretical, 2018. [Sho99] Peter W Shor. Polynomial-time algorithms for prime factorization and discrete logarithms on a quantum computer. SIAM review, 41(2):303–332, 1999. [SKCC20] Kunal Sharma, Sumeet Khatri, Marco Cerezo, and Patrick Coles. Noise resilience of variational quantum compiling. New Journal of Physics, 2020. 17 / 17
  • 27. [TBG17] K. Temme, S. Bravyi, and J. M. Gambetta. Error mitigation for short-depth quantum circuits. Physical Review Letters, 119(18):180509, 2017. 17 / 17