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Spatial resolution measurements of the advanced radiographic capability x-ray
imaging system at energies relevant to Compton radiography
G. N. Hall, N. Izumi, O. L. Landen, R. Tommasini, J. P. Holder, D. Hargrove, D. K. Bradley, A. Lumbard, J. G.
Cruz, K. Piston, J. J. Lee, E. Romano, P. M. Bell, A. C. Carpenter, N. E. Palmer, B. Felker, V. Rekow, and F.
V. Allen
Citation: Review of Scientific Instruments 87, 11E310 (2016); doi: 10.1063/1.4959948
View online: http://dx.doi.org/10.1063/1.4959948
View Table of Contents: http://scitation.aip.org/content/aip/journal/rsi/87/11?ver=pdfcov
Published by the AIP Publishing
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REVIEW OF SCIENTIFIC INSTRUMENTS 87, 11E310 (2016)
Spatial resolution measurements of the advanced radiographic capability
x-ray imaging system at energies relevant to Compton radiography
G. N. Hall,1,a)
N. Izumi,1
O. L. Landen,1
R. Tommasini,1
J. P. Holder,1
D. Hargrove,1
D. K. Bradley,1
A. Lumbard,1
J. G. Cruz,1
K. Piston,1
J. J. Lee,2
E. Romano,2
P. M. Bell,1
A. C. Carpenter,1
N. E. Palmer,1
B. Felker,1
V. Rekow,1
and F. V. Allen1
1
Lawrence Livermore National Laboratory, 7000 East Avenue, Livermore, California 94550, USA
2
National Security Technologies LLC, 161 S Vasco Rd., Livermore, California 94551, USA
(Presented 8 June 2016; received 13 June 2016; accepted 2 July 2016;
published online 3 August 2016)
Compton radiography provides a means to measure the integrity, ρR and symmetry of the DT
fuel in an inertial confinement fusion implosion near peak compression. Upcoming experiments at
the National Ignition Facility will use the ARC (Advanced Radiography Capability) laser to drive
backlighter sources for Compton radiography experiments and will use the newly commissioned
AXIS (ARC X-ray Imaging System) instrument as the detector. AXIS uses a dual-MCP (micro-
channel plate) to provide gating and high DQE at the 40–200 keV x-ray range required for Compton
radiography, but introduces many effects that contribute to the spatial resolution. Experiments were
performed at energies relevant to Compton radiography to begin characterization of the spatial reso-
lution of the AXIS diagnostic. Published by AIP Publishing. [http://dx.doi.org/10.1063/1.4959948]
I. INTRODUCTION
Compton radiography provides a means to measure the
density and asymmetries of the DT fuel in an inertial confine-
ment fusion capsule near the time of peak compression.1
The
ARC X-ray Imaging System (AXIS) instrument3
has recently
been commissioned at the National Ignition Facility (NIF) and
will be the detector for Compton radiography driven by the Ad-
vanced Radiography Capability (ARC) laser.2
ARC converts a
NIF quad into several 1 kJ, 30 ps beams (4 beams at present,
8 in the future) and will be used to produce bremsstrahlung
X-ray sources in the range of 40 keV–200 keV for Compton
radiography.
AXIS uses a dual-microchannel plate (MCP) configura-
tion to provide significantly improved detective quantum effi-
ciency (DQE) at high x-ray energies and to provide gating to
reduce background from neutrons and hard x-rays from laser-
plasma-interactions in the hohlraum. The dual-MCP system
uses a thick, low gain MCP as a volumetric photocathode in a
chevron configuration with a thinner, high gain MCP which
acts as an amplifier. This configuration has demonstrated a
DQE of ∼4.5% at 60 keV4
compared to a DQE of ∼1.1% for a
single MCP with the same overall gain. This enables AXIS
to provide a cleaner image that will allow the density and
distribution of the compressed DT fuel to be measured with
significantly greater accuracy as Inertial Confinement Fusion
(ICF) experiments are tuned for ignition.
In order to measure the density of the DT fuel to the
required accuracy, it is important to know the resolution of the
AXIS diagnostic at energies relevant to Compton radiography
Note: Contributed paper, published as part of the Proceedings of the 21st
Topical Conference on High-Temperature Plasma Diagnostics, Madison,
Wisconsin, USA, June 2016.
a)Author to whom correspondence should be addressed. Electronic mail:
hall98@llnl.gov.
experiments. Use of a chevron configuration at high x-ray ener-
gies introduces many effects that contribute to the spatial reso-
lution of the instrument. High energy X-rays produce detection
events throughout the volume of both MCPs, crossing many
pores, and the gaps between the MCPs and between the MCP
and the phosphor allow for the transverse spread of electrons.
Here we present measurements of the spatial resolution of
AXIS in DC mode at 4 x-ray energies between 20 keV and
100 keV.
II. EXPERIMENTAL SETUP AND ANALYSIS
These measurements were performed at the High Energy
X-ray (HEX) laboratory5
at National Security Technologies
LLC. The HEX generates characteristic fluorescence lines
from 8–111 keV and can provide continuous x-ray intensities
on the order of 106
photons/(s/cm2
). The HEX was operated
with four different fluorescer materials (Ag, W, Bi, U) and
appropriate filters such that the spectrum was dominated by
the Kα lines of each material at 22 keV, 59 keV, 77 keV, and
98 keV.
In the experimental setup, shown in Fig. 1, the full area of
AXIS was exposed to x-rays incident at 87.5◦
in the horizontal
plane to reproduce the angle of incidence on a Compton radi-
ography experiment. The size of the HEX source was 5 mm
in diameter and 1429 mm from the surface of MCP1: this
would produce a ∼5 µm penumbra, which is much smaller
than the resolution of AXIS and therefore the HEX source can
be considered point-like for these experiments. A resolution
test mask, shown in an example AXIS image in Fig. 2, was
placed ∼1.5 mm in front of AXIS and consisted of a grid of
1 mm diameter rods of Ta, with one grid square covered by a
1 mm thick Ta sheet. The advantage of using rods rather than
a knife edge is that a cylindrical object requires no alignment
0034-6748/2016/87(11)/11E310/4/$30.00 87, 11E310-1 Published by AIP Publishing.
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2016 19:02:20
11E310-2 Hall et al. Rev. Sci. Instrum. 87, 11E310 (2016)
FIG. 1. Top down view of the experimental setup. The pore bias of each
MCP is in the horizontal plane.
relative to the x-ray source and the transmission through it can
be modeled analytically.
AXIS was operated in DC mode, as the x-ray intensity was
insufficient for pulsed mode, at all 4 energies both with and
without the resolution mask in place. On NIF experiments, a
film will be used to record the images, but for these experi-
ments a CCD was used.
An optimization routine is used to calculate a horizontal
and vertical line spread function (LSF) at each of the 4 ener-
gies. First, the image with the resolution grid is divided by
an image without the grid to produce a transmission image,
and a lineout is taken across a resolution mask feature. The
transmission of x-rays through the region sampled by the
lineout is calculated, then convolved with an initial guess of
the LSF to produce a model lineout. The model lineout is then
compared to the real lineout and the residual calculated. The
optimization routine then modifies the LSF iteratively until the
residual between the real and modeled lineout is minimized.
The end result is the best estimate of the actual LSF.
For this process, a function consisting of three Gaussians
is chosen to represent the LSF. The ease of analytical manip-
ulation of the Gaussian functional form was advantageous for
analysis, and three terms were the minimum number required
to obtain a satisfactory fit to the data. The form of the fitted
LSF is
LSF = A1e−x2/2σ2
1 + A2e−x2/2σ2
2 + A3e−x2/2σ2
3. (1)
The optimization routine was constrained such that σ3 >
σ2 > σ1 to give a long, medium, and short range component,
FIG. 2. An example AXIS image at 59 keV with the resolution mask. The
center-to-center distance of the rods is 8 mm.
and An was constrained such that the area under the LSF was
unity.
Analysis of different regions of the resolution mask was
used to improve the accuracy of the LSF fit. First, the Ta slab
section of the mask was analyzed. The slab is sufficiently wide
to observe the manner in which the signal decreases almost
to zero without interference from short and medium-range
effects. This allows the long range component of the LSF to
be measured more accurately, and by running the optimization
routine on multiple lineouts taken across the slab, the mean
value of A3 and σ3, and the standard deviation of each, is found.
Then, every rod feature in the image is analyzed with the values
of A3 and σ3 only being allowed to vary within 2 standard
deviations of the mean values found during the slab analysis.
This produces mean values and standard deviations for A1, A2,
σ1, and σ2.
III. RESULTS AND DISCUSSION
The LSF, shown in Fig. 3, varies as a function of both
x-ray energy and direction. For each energy and direction,
Fig. 4 shows the FWHM and contribution to the LSF for each
of the short, medium, and long-range Gaussian components.
It should be noted that the error bars are much larger for
the 77 keV and 98 keV measurements because the filtering
required to produce a clean spectrum dominated by Kα lines
at these energies reduced the x-ray intensity dramatically. As
a result, the signal level in the 77 keV and 98 keV images is
only ∼1% of the signal level in the 22 keV and 59 keV images,
resulting in substantially more noise and error bars that are
many times larger.
The short, medium, and long-range FWHMs are useful
for understanding the physical processes underlying each
component.
Several effects are likely to contribute to the short-range
component shown in Fig. 4(a), but the dominant effect is
likely the transverse spread of electrons in the gap between
the two MCPs, and also in the gap between the MCP and
the phosphor. Wiedwald et al.6
describe measurements of the
initial transverse energy of electrons between an MCP and
phosphor in the direction perpendicular and parallel to the pore
bias direction as a result of the electric field in the gap acquiring
a component in the direction of the pore bias. For an MCP
FIG. 3. Vertical and horizontal LSFs at 4 x-ray energies.
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2016 19:02:20
11E310-3 Hall et al. Rev. Sci. Instrum. 87, 11E310 (2016)
FIG. 4. The FWHM and contribution to the LSF (as a fraction of the area)
of the (a) short, (b) medium, and (c) long-range Gaussian components. Error
bars show the standard error.
in DC mode with a pore bias of 5◦
(similar to the 8◦
bias of
the AXIS MCPs), this energy was measured to have a mean
value of 1 eV and 2.4 eV in the perpendicular and parallel
directions, respectively. For a chevron MCP arrangement, it
might be expected that the perturbation to the electric field
from the upper and lower MCPs would cancel out in the
gap between them, leaving the perpendicular and parallel
transverse energies equal at ∼1 eV. In the gap between the
MCP and phosphor of a chevron arrangement, however, the
transverse energies should be as measured by Wiedwald et al.
Using the spacings and voltages specified in Fig. 1 for the
MCP gap and assuming 1 eV in both directions, the spread
is expected to be ∼94 µm. For the phosphor gap, 1 eV in the
vertical direction and 2.4 eV in the horizontal direction will
produce a spread of ∼70 µm and ∼108 µm, respectively. Added
in quadrature, this gives ∼117 µm in the vertical direction and
∼143 µm in the horizontal.
A second effect on the short range component is the range
of the primary electron, generated predominantly by photoion-
isation of the Pb dopant within the MCP glass. The mean
range of the primary electrons in solid lead glass is the CSDA
range divided by the detour factor. The detour factor can be
approximated by first calculating the mean atomic number of
the lead glass of the MCP from the elemental composition
given by Wiza,7
which gives ¯Z ≈ 17. From Tabata et al.,8
the
detour factor for ≤100 keV electrons in material with ¯Z ≈ 17 is
≈2.8. The increased range of electrons in the porous structure
of the MCP can be approximated by multiplying the mean
range in solid lead glass by (1 − A)−1
, where A is the open area
ratio of the MCP. AXIS uses MCPs with 10 µm diameter pores
at a 12 µm pitch, giving A = 0.628, and so the mean range
in the MCP is ≈2.7 times the mean range in solid lead glass.
The mean range of primary electrons in the MCP is there-
fore the CSDA range multiplied by 2.7/2.8 ≈ 1. For 22 keV,
59 keV, and 77 keV x-rays, 76% of the primary electrons are
from photoionization from the Pb L-shell, resulting in primary
electrons with 7 keV, 44 keV, and 62 keV, respectively. For the
98 keV x-rays, 79% of photoelectrons are ionized from the Pb
K-shell and have an energy of 10 keV. The mean range of these
primary electrons in the AXIS MCPs is expected to be ∼2 µm,
∼14 µm, ∼26 µm, and ∼1 µm for the 22 keV, 59 keV, 77 keV,
and 98 keV x-rays, respectively.
The effect of x-rays crossing multiple pores should also
be considered. For all the x-ray energies used in these experi-
ments, the MCPs can be considered optically thin. Therefore,
photoelectric events will occur throughout the entire volume,
but for gains >1 shallow events will contribute more to the final
signal than deep events. For an MCP operating with gain G, the
fraction of the plate thickness that contributes to the final signal
is ∼1/ln(G). AXIS operates MCP1 with a gain of ∼10, so only
the first ∼43% of the plate thickness contributes to the signal.
The x-rays are incident at 10.5◦
to the pores of MCP1, resulting
in a ∼157 µm horizontal displacement as the x-rays traverse
the plate. Assuming only the first ∼43% of MCP1 contributes
to the signal, this effect is expected to produce an additional
horizontal spread of ∼68 µm.
Lastly, the resolution of the CCD camera and fiber optic
components shown in Fig. 1 must be included. Calibration
of the CCD camera is discussed in Kimbrough et al.9
which
states that the contrast transfer function is 0.5 at 33.5l p/mm.
Assuming a Gaussian LSF, this corresponds to a FWHM of
∼15 µm. The fiber optic faceplate and fiber optic extension are
both constructed from 6 µm fibers, which enables 102l p/mm
to be resolved.10
Assuming at least 5% contrast is required to
resolve, and a Gaussian LSF, this corresponds to a FWHM of
∼10 µm for each of these components.
Adding all these effects in quadrature for the vertical
direction gives 137 µm, 140 µm, 146 µm, and 137 µm for
22 keV, 59 keV, 77 keV, and 98 keV x-rays, respectively, which
is within ∼10 µm of the measured values for all energies except
22 keV. In the horizontal direction, the quadrature sum gives
160 µm, 162 µm, 168 µm, and 160 µm for 22 keV, 59 keV,
77 keV, and 98 keV x-rays, respectively, which is ∼25–40 µm
above the measured values for all energies. It is possible that
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2016 19:02:20
11E310-4 Hall et al. Rev. Sci. Instrum. 87, 11E310 (2016)
the direction of the pore bias in MCP2, which would translate
the signal in the opposite horizontal direction to the pore bias in
MCP1, could be responsible for the actual horizontal FWHM
being lower than the estimated value.
The medium-range component is shown in Fig. 4(b). A
contribution to the medium range component could be due
to Compton scattering of incident x-rays from the Ta rods
comprising the resolution mask. Using the Klein-Nishina for-
mula to calculate the probability of scattering over an angular
range from 0◦
to 90◦
from the incident angle (i.e., angles where
the scattered photon can still hit the MCP) gives the mean
scattering angle as 36◦
–38◦
for 22 keV–98 keV. The most
likely region of a rod to produce scattering that will eventually
be detected by the MCP is the region near the lateral edges,
i.e., close to the surface of the rod ∼2 mm above MCP1.
Photons will arrive at this region with minimal likelihood of
already having been absorbed by the rod and can continue
onwards with minimal likelihood of being absorbed. A photon
scattered from ∼2 mm above the surface of MCP1 at 37◦
will
be deflected up to ∼1.5 mm in a direction perpendicular to
the rod, which closely matches the FWHM of the medium-
range component. However, in order for an incident x-ray to
penetrate the rod, scatter, and then emerge and be detected, its
path length before and after scattering cannot be much greater
than the mean free path (MFP) in the rod material. Assuming
the energy of the scattered photon is approximately the same
as the incident photon (a good approximation for the x-ray
energies considered here) then the maximum total path length
through the rod (pre- plus post- scattering) is ∼25 µm for
22 keV x-rays, and ∼200–300 µm for the higher energies. A
path restricted to this length can only occur in a layer within
∼0.2 µm of the surface of the rod for 22 keV x-rays, and within
∼10–40 µm of the surface of the rod for the higher energies,
and therefore only photons that pass within this distance of the
rod surface can contribute significantly to the scattering signal.
Compared to the length of the lineout affected by the medium
range component, the fraction of total incident photons that
can contribute to the scattering signal is ≪1% for the 22 keV
x-rays, and <2% for the higher energies. It therefore seems
unlikely that scattering can be responsible for more than a very
small amount of the large 20%-40% contribution of the me-
dium range component to the LSF. An upcoming experiment
will seek to confirm this by repeating the measurement using
an image plate as the detector, as any scattering from the Ta
rods will be independent of the detection device
The majority of the medium range signal is likely due to
visible photons emitted from the phosphor into the gap being
reflected back from the rear surface of MCP2. This effect is
a strong possibility since the surface of the phosphor is not
aluminized, and it is expected that this effect would occur on
scale lengths similar to the ∼1 mm MCP-phosphor gap. The
use of aluminized phosphors to reduce this effect is discussed
in the literature,11
but aluminizing phosphors to withstand
pulsed operation ≥5 kV (typically value for NIF) has been
unsuccessful.
The long-range component is shown in Fig. 4(c). The lack
of x-ray energy dependence and very long FWHM
suggests that it might be due to electrons incident on the
phosphor undergoing scattering in the transverse direction.
FIG. 5. 1D vertical and horizontal MTFs at 4 x-ray energies.
Multiple scattering events can result in electrons traveling
a long transverse distance in the gap. Electron scattering is
another effect that can be mitigated by aluminizing the phosp-
hor,11
and therefore, development of aluminized phosphors
that can survive high pulsed voltages would be extremely
valuable for improving the spatial resolution of AXIS and
other NIF framing cameras.
LSFs were used to calculate 1D modulation transfer func-
tions at the object plane as a function of wavelength for an
imaging system with magnification of 100, the magnification
of the Compton radiography platform on NIF, and are shown
in Fig. 5.
IV. CONCLUSIONS
AXIS is a gated detector that has recently been commis-
sioned at the NIF for Compton radiography. AXIS uses a
dual-MCP configuration that improves DQE at high x-ray
energies, but limits spatial resolution. The spatial resolution
was characterized at 22 keV, 59 keV, 77 keV, and 98 keV in
DC mode in the horizontal and vertical directions. Line spread
functions were fitted using a combination of 3 Gaussians, and
the 1D modulation transfer function was calculated at each
energy, suggesting that contrast will be reduced by ∼50% for
scale lengths at the source-size resolution limit for Compton
radiography on the NIF.
ACKNOWLEDGMENTS
Lawrence Livermore National Laboratory is operated by
Lawrence Livermore National Security, LLC, for the U.S. De-
partment of Energy, National Nuclear Security Administration
under Contract No. DE-AC52-07NA27344 (Grant No. LLNL-
PROC-694818).
1R. Tommasini et al., Phys. Plasmas 18, 056309 (2011).
2J. K. Crane et al., J. Phys.: Conf. Ser. 244, 032003 (2010).
3G. N. Hall et al., Rev. Sci. Instrum. 85, 11D624 (2014).
4N. Izumi et al., Rev. Sci. Instrum. 85, 11D623 (2014).
5J. J. Lee et al., Proc. SPIE 8505, 850508 (2012).
6J. D. Wiedwald et al., Proc. SPIE 1346, 449 (1991).
7J. L. Wiza, Nucl. Instrum. Methods 162, 587 (1979).
8T. Tabata et al., Nucl. Instrum. Methods Phys. Res. Sect. B 108, 11-17
(1996).
9J. R. Kimbrough et al., Rev. Sci. Instrum. 75, 4060 (2004).
10See http://www.us.schott.com/lightingimaging/english/defenseproducts/
faceplates.html for resolution of fiber optic faceplates.
11C. J. Pawley, Rev. Sci. Instrum. 71, 1286 (2000).
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2016 19:02:20

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AXIS paper

  • 1. Spatial resolution measurements of the advanced radiographic capability x-ray imaging system at energies relevant to Compton radiography G. N. Hall, N. Izumi, O. L. Landen, R. Tommasini, J. P. Holder, D. Hargrove, D. K. Bradley, A. Lumbard, J. G. Cruz, K. Piston, J. J. Lee, E. Romano, P. M. Bell, A. C. Carpenter, N. E. Palmer, B. Felker, V. Rekow, and F. V. Allen Citation: Review of Scientific Instruments 87, 11E310 (2016); doi: 10.1063/1.4959948 View online: http://dx.doi.org/10.1063/1.4959948 View Table of Contents: http://scitation.aip.org/content/aip/journal/rsi/87/11?ver=pdfcov Published by the AIP Publishing Articles you may be interested in The x-ray light valve: A low-cost, digital radiographic imaging system—Spatial resolution Med. Phys. 35, 4216 (2008); 10.1118/1.2968093 Fundamental x-ray interaction limits in diagnostic imaging detectors: Spatial resolution Med. Phys. 35, 3180 (2008); 10.1118/1.2924219 Image quality evaluation of flat panel and image intensifier digital magnification in x-ray fluoroscopy Med. Phys. 29, 1611 (2002); 10.1118/1.1487858 A comprehensive physical image quality evaluation of a selenium based digital x-ray imaging system for thorax radiography Med. Phys. 25, 986 (1998); 10.1118/1.598276 Are storage phosphors a useful tool for soft x-ray imaging diagnostics? Spectral sensitivity and spatial resolution in the 0.07 to 14 nm range J. Appl. Phys. 83, 2276 (1998); 10.1063/1.366968 Reuse of AIP Publishing content is subject to the terms at: https://publishing.aip.org/authors/rights-and-permissions. Download to IP: 128.115.190.41 On: Wed, 03 Aug 2016 19:02:20
  • 2. REVIEW OF SCIENTIFIC INSTRUMENTS 87, 11E310 (2016) Spatial resolution measurements of the advanced radiographic capability x-ray imaging system at energies relevant to Compton radiography G. N. Hall,1,a) N. Izumi,1 O. L. Landen,1 R. Tommasini,1 J. P. Holder,1 D. Hargrove,1 D. K. Bradley,1 A. Lumbard,1 J. G. Cruz,1 K. Piston,1 J. J. Lee,2 E. Romano,2 P. M. Bell,1 A. C. Carpenter,1 N. E. Palmer,1 B. Felker,1 V. Rekow,1 and F. V. Allen1 1 Lawrence Livermore National Laboratory, 7000 East Avenue, Livermore, California 94550, USA 2 National Security Technologies LLC, 161 S Vasco Rd., Livermore, California 94551, USA (Presented 8 June 2016; received 13 June 2016; accepted 2 July 2016; published online 3 August 2016) Compton radiography provides a means to measure the integrity, ρR and symmetry of the DT fuel in an inertial confinement fusion implosion near peak compression. Upcoming experiments at the National Ignition Facility will use the ARC (Advanced Radiography Capability) laser to drive backlighter sources for Compton radiography experiments and will use the newly commissioned AXIS (ARC X-ray Imaging System) instrument as the detector. AXIS uses a dual-MCP (micro- channel plate) to provide gating and high DQE at the 40–200 keV x-ray range required for Compton radiography, but introduces many effects that contribute to the spatial resolution. Experiments were performed at energies relevant to Compton radiography to begin characterization of the spatial reso- lution of the AXIS diagnostic. Published by AIP Publishing. [http://dx.doi.org/10.1063/1.4959948] I. INTRODUCTION Compton radiography provides a means to measure the density and asymmetries of the DT fuel in an inertial confine- ment fusion capsule near the time of peak compression.1 The ARC X-ray Imaging System (AXIS) instrument3 has recently been commissioned at the National Ignition Facility (NIF) and will be the detector for Compton radiography driven by the Ad- vanced Radiography Capability (ARC) laser.2 ARC converts a NIF quad into several 1 kJ, 30 ps beams (4 beams at present, 8 in the future) and will be used to produce bremsstrahlung X-ray sources in the range of 40 keV–200 keV for Compton radiography. AXIS uses a dual-microchannel plate (MCP) configura- tion to provide significantly improved detective quantum effi- ciency (DQE) at high x-ray energies and to provide gating to reduce background from neutrons and hard x-rays from laser- plasma-interactions in the hohlraum. The dual-MCP system uses a thick, low gain MCP as a volumetric photocathode in a chevron configuration with a thinner, high gain MCP which acts as an amplifier. This configuration has demonstrated a DQE of ∼4.5% at 60 keV4 compared to a DQE of ∼1.1% for a single MCP with the same overall gain. This enables AXIS to provide a cleaner image that will allow the density and distribution of the compressed DT fuel to be measured with significantly greater accuracy as Inertial Confinement Fusion (ICF) experiments are tuned for ignition. In order to measure the density of the DT fuel to the required accuracy, it is important to know the resolution of the AXIS diagnostic at energies relevant to Compton radiography Note: Contributed paper, published as part of the Proceedings of the 21st Topical Conference on High-Temperature Plasma Diagnostics, Madison, Wisconsin, USA, June 2016. a)Author to whom correspondence should be addressed. Electronic mail: hall98@llnl.gov. experiments. Use of a chevron configuration at high x-ray ener- gies introduces many effects that contribute to the spatial reso- lution of the instrument. High energy X-rays produce detection events throughout the volume of both MCPs, crossing many pores, and the gaps between the MCPs and between the MCP and the phosphor allow for the transverse spread of electrons. Here we present measurements of the spatial resolution of AXIS in DC mode at 4 x-ray energies between 20 keV and 100 keV. II. EXPERIMENTAL SETUP AND ANALYSIS These measurements were performed at the High Energy X-ray (HEX) laboratory5 at National Security Technologies LLC. The HEX generates characteristic fluorescence lines from 8–111 keV and can provide continuous x-ray intensities on the order of 106 photons/(s/cm2 ). The HEX was operated with four different fluorescer materials (Ag, W, Bi, U) and appropriate filters such that the spectrum was dominated by the Kα lines of each material at 22 keV, 59 keV, 77 keV, and 98 keV. In the experimental setup, shown in Fig. 1, the full area of AXIS was exposed to x-rays incident at 87.5◦ in the horizontal plane to reproduce the angle of incidence on a Compton radi- ography experiment. The size of the HEX source was 5 mm in diameter and 1429 mm from the surface of MCP1: this would produce a ∼5 µm penumbra, which is much smaller than the resolution of AXIS and therefore the HEX source can be considered point-like for these experiments. A resolution test mask, shown in an example AXIS image in Fig. 2, was placed ∼1.5 mm in front of AXIS and consisted of a grid of 1 mm diameter rods of Ta, with one grid square covered by a 1 mm thick Ta sheet. The advantage of using rods rather than a knife edge is that a cylindrical object requires no alignment 0034-6748/2016/87(11)/11E310/4/$30.00 87, 11E310-1 Published by AIP Publishing. Reuse of AIP Publishing content is subject to the terms at: https://publishing.aip.org/authors/rights-and-permissions. Download to IP: 128.115.190.41 On: Wed, 03 Aug 2016 19:02:20
  • 3. 11E310-2 Hall et al. Rev. Sci. Instrum. 87, 11E310 (2016) FIG. 1. Top down view of the experimental setup. The pore bias of each MCP is in the horizontal plane. relative to the x-ray source and the transmission through it can be modeled analytically. AXIS was operated in DC mode, as the x-ray intensity was insufficient for pulsed mode, at all 4 energies both with and without the resolution mask in place. On NIF experiments, a film will be used to record the images, but for these experi- ments a CCD was used. An optimization routine is used to calculate a horizontal and vertical line spread function (LSF) at each of the 4 ener- gies. First, the image with the resolution grid is divided by an image without the grid to produce a transmission image, and a lineout is taken across a resolution mask feature. The transmission of x-rays through the region sampled by the lineout is calculated, then convolved with an initial guess of the LSF to produce a model lineout. The model lineout is then compared to the real lineout and the residual calculated. The optimization routine then modifies the LSF iteratively until the residual between the real and modeled lineout is minimized. The end result is the best estimate of the actual LSF. For this process, a function consisting of three Gaussians is chosen to represent the LSF. The ease of analytical manip- ulation of the Gaussian functional form was advantageous for analysis, and three terms were the minimum number required to obtain a satisfactory fit to the data. The form of the fitted LSF is LSF = A1e−x2/2σ2 1 + A2e−x2/2σ2 2 + A3e−x2/2σ2 3. (1) The optimization routine was constrained such that σ3 > σ2 > σ1 to give a long, medium, and short range component, FIG. 2. An example AXIS image at 59 keV with the resolution mask. The center-to-center distance of the rods is 8 mm. and An was constrained such that the area under the LSF was unity. Analysis of different regions of the resolution mask was used to improve the accuracy of the LSF fit. First, the Ta slab section of the mask was analyzed. The slab is sufficiently wide to observe the manner in which the signal decreases almost to zero without interference from short and medium-range effects. This allows the long range component of the LSF to be measured more accurately, and by running the optimization routine on multiple lineouts taken across the slab, the mean value of A3 and σ3, and the standard deviation of each, is found. Then, every rod feature in the image is analyzed with the values of A3 and σ3 only being allowed to vary within 2 standard deviations of the mean values found during the slab analysis. This produces mean values and standard deviations for A1, A2, σ1, and σ2. III. RESULTS AND DISCUSSION The LSF, shown in Fig. 3, varies as a function of both x-ray energy and direction. For each energy and direction, Fig. 4 shows the FWHM and contribution to the LSF for each of the short, medium, and long-range Gaussian components. It should be noted that the error bars are much larger for the 77 keV and 98 keV measurements because the filtering required to produce a clean spectrum dominated by Kα lines at these energies reduced the x-ray intensity dramatically. As a result, the signal level in the 77 keV and 98 keV images is only ∼1% of the signal level in the 22 keV and 59 keV images, resulting in substantially more noise and error bars that are many times larger. The short, medium, and long-range FWHMs are useful for understanding the physical processes underlying each component. Several effects are likely to contribute to the short-range component shown in Fig. 4(a), but the dominant effect is likely the transverse spread of electrons in the gap between the two MCPs, and also in the gap between the MCP and the phosphor. Wiedwald et al.6 describe measurements of the initial transverse energy of electrons between an MCP and phosphor in the direction perpendicular and parallel to the pore bias direction as a result of the electric field in the gap acquiring a component in the direction of the pore bias. For an MCP FIG. 3. Vertical and horizontal LSFs at 4 x-ray energies. Reuse of AIP Publishing content is subject to the terms at: https://publishing.aip.org/authors/rights-and-permissions. Download to IP: 128.115.190.41 On: Wed, 03 Aug 2016 19:02:20
  • 4. 11E310-3 Hall et al. Rev. Sci. Instrum. 87, 11E310 (2016) FIG. 4. The FWHM and contribution to the LSF (as a fraction of the area) of the (a) short, (b) medium, and (c) long-range Gaussian components. Error bars show the standard error. in DC mode with a pore bias of 5◦ (similar to the 8◦ bias of the AXIS MCPs), this energy was measured to have a mean value of 1 eV and 2.4 eV in the perpendicular and parallel directions, respectively. For a chevron MCP arrangement, it might be expected that the perturbation to the electric field from the upper and lower MCPs would cancel out in the gap between them, leaving the perpendicular and parallel transverse energies equal at ∼1 eV. In the gap between the MCP and phosphor of a chevron arrangement, however, the transverse energies should be as measured by Wiedwald et al. Using the spacings and voltages specified in Fig. 1 for the MCP gap and assuming 1 eV in both directions, the spread is expected to be ∼94 µm. For the phosphor gap, 1 eV in the vertical direction and 2.4 eV in the horizontal direction will produce a spread of ∼70 µm and ∼108 µm, respectively. Added in quadrature, this gives ∼117 µm in the vertical direction and ∼143 µm in the horizontal. A second effect on the short range component is the range of the primary electron, generated predominantly by photoion- isation of the Pb dopant within the MCP glass. The mean range of the primary electrons in solid lead glass is the CSDA range divided by the detour factor. The detour factor can be approximated by first calculating the mean atomic number of the lead glass of the MCP from the elemental composition given by Wiza,7 which gives ¯Z ≈ 17. From Tabata et al.,8 the detour factor for ≤100 keV electrons in material with ¯Z ≈ 17 is ≈2.8. The increased range of electrons in the porous structure of the MCP can be approximated by multiplying the mean range in solid lead glass by (1 − A)−1 , where A is the open area ratio of the MCP. AXIS uses MCPs with 10 µm diameter pores at a 12 µm pitch, giving A = 0.628, and so the mean range in the MCP is ≈2.7 times the mean range in solid lead glass. The mean range of primary electrons in the MCP is there- fore the CSDA range multiplied by 2.7/2.8 ≈ 1. For 22 keV, 59 keV, and 77 keV x-rays, 76% of the primary electrons are from photoionization from the Pb L-shell, resulting in primary electrons with 7 keV, 44 keV, and 62 keV, respectively. For the 98 keV x-rays, 79% of photoelectrons are ionized from the Pb K-shell and have an energy of 10 keV. The mean range of these primary electrons in the AXIS MCPs is expected to be ∼2 µm, ∼14 µm, ∼26 µm, and ∼1 µm for the 22 keV, 59 keV, 77 keV, and 98 keV x-rays, respectively. The effect of x-rays crossing multiple pores should also be considered. For all the x-ray energies used in these experi- ments, the MCPs can be considered optically thin. Therefore, photoelectric events will occur throughout the entire volume, but for gains >1 shallow events will contribute more to the final signal than deep events. For an MCP operating with gain G, the fraction of the plate thickness that contributes to the final signal is ∼1/ln(G). AXIS operates MCP1 with a gain of ∼10, so only the first ∼43% of the plate thickness contributes to the signal. The x-rays are incident at 10.5◦ to the pores of MCP1, resulting in a ∼157 µm horizontal displacement as the x-rays traverse the plate. Assuming only the first ∼43% of MCP1 contributes to the signal, this effect is expected to produce an additional horizontal spread of ∼68 µm. Lastly, the resolution of the CCD camera and fiber optic components shown in Fig. 1 must be included. Calibration of the CCD camera is discussed in Kimbrough et al.9 which states that the contrast transfer function is 0.5 at 33.5l p/mm. Assuming a Gaussian LSF, this corresponds to a FWHM of ∼15 µm. The fiber optic faceplate and fiber optic extension are both constructed from 6 µm fibers, which enables 102l p/mm to be resolved.10 Assuming at least 5% contrast is required to resolve, and a Gaussian LSF, this corresponds to a FWHM of ∼10 µm for each of these components. Adding all these effects in quadrature for the vertical direction gives 137 µm, 140 µm, 146 µm, and 137 µm for 22 keV, 59 keV, 77 keV, and 98 keV x-rays, respectively, which is within ∼10 µm of the measured values for all energies except 22 keV. In the horizontal direction, the quadrature sum gives 160 µm, 162 µm, 168 µm, and 160 µm for 22 keV, 59 keV, 77 keV, and 98 keV x-rays, respectively, which is ∼25–40 µm above the measured values for all energies. It is possible that Reuse of AIP Publishing content is subject to the terms at: https://publishing.aip.org/authors/rights-and-permissions. Download to IP: 128.115.190.41 On: Wed, 03 Aug 2016 19:02:20
  • 5. 11E310-4 Hall et al. Rev. Sci. Instrum. 87, 11E310 (2016) the direction of the pore bias in MCP2, which would translate the signal in the opposite horizontal direction to the pore bias in MCP1, could be responsible for the actual horizontal FWHM being lower than the estimated value. The medium-range component is shown in Fig. 4(b). A contribution to the medium range component could be due to Compton scattering of incident x-rays from the Ta rods comprising the resolution mask. Using the Klein-Nishina for- mula to calculate the probability of scattering over an angular range from 0◦ to 90◦ from the incident angle (i.e., angles where the scattered photon can still hit the MCP) gives the mean scattering angle as 36◦ –38◦ for 22 keV–98 keV. The most likely region of a rod to produce scattering that will eventually be detected by the MCP is the region near the lateral edges, i.e., close to the surface of the rod ∼2 mm above MCP1. Photons will arrive at this region with minimal likelihood of already having been absorbed by the rod and can continue onwards with minimal likelihood of being absorbed. A photon scattered from ∼2 mm above the surface of MCP1 at 37◦ will be deflected up to ∼1.5 mm in a direction perpendicular to the rod, which closely matches the FWHM of the medium- range component. However, in order for an incident x-ray to penetrate the rod, scatter, and then emerge and be detected, its path length before and after scattering cannot be much greater than the mean free path (MFP) in the rod material. Assuming the energy of the scattered photon is approximately the same as the incident photon (a good approximation for the x-ray energies considered here) then the maximum total path length through the rod (pre- plus post- scattering) is ∼25 µm for 22 keV x-rays, and ∼200–300 µm for the higher energies. A path restricted to this length can only occur in a layer within ∼0.2 µm of the surface of the rod for 22 keV x-rays, and within ∼10–40 µm of the surface of the rod for the higher energies, and therefore only photons that pass within this distance of the rod surface can contribute significantly to the scattering signal. Compared to the length of the lineout affected by the medium range component, the fraction of total incident photons that can contribute to the scattering signal is ≪1% for the 22 keV x-rays, and <2% for the higher energies. It therefore seems unlikely that scattering can be responsible for more than a very small amount of the large 20%-40% contribution of the me- dium range component to the LSF. An upcoming experiment will seek to confirm this by repeating the measurement using an image plate as the detector, as any scattering from the Ta rods will be independent of the detection device The majority of the medium range signal is likely due to visible photons emitted from the phosphor into the gap being reflected back from the rear surface of MCP2. This effect is a strong possibility since the surface of the phosphor is not aluminized, and it is expected that this effect would occur on scale lengths similar to the ∼1 mm MCP-phosphor gap. The use of aluminized phosphors to reduce this effect is discussed in the literature,11 but aluminizing phosphors to withstand pulsed operation ≥5 kV (typically value for NIF) has been unsuccessful. The long-range component is shown in Fig. 4(c). The lack of x-ray energy dependence and very long FWHM suggests that it might be due to electrons incident on the phosphor undergoing scattering in the transverse direction. FIG. 5. 1D vertical and horizontal MTFs at 4 x-ray energies. Multiple scattering events can result in electrons traveling a long transverse distance in the gap. Electron scattering is another effect that can be mitigated by aluminizing the phosp- hor,11 and therefore, development of aluminized phosphors that can survive high pulsed voltages would be extremely valuable for improving the spatial resolution of AXIS and other NIF framing cameras. LSFs were used to calculate 1D modulation transfer func- tions at the object plane as a function of wavelength for an imaging system with magnification of 100, the magnification of the Compton radiography platform on NIF, and are shown in Fig. 5. IV. CONCLUSIONS AXIS is a gated detector that has recently been commis- sioned at the NIF for Compton radiography. AXIS uses a dual-MCP configuration that improves DQE at high x-ray energies, but limits spatial resolution. The spatial resolution was characterized at 22 keV, 59 keV, 77 keV, and 98 keV in DC mode in the horizontal and vertical directions. Line spread functions were fitted using a combination of 3 Gaussians, and the 1D modulation transfer function was calculated at each energy, suggesting that contrast will be reduced by ∼50% for scale lengths at the source-size resolution limit for Compton radiography on the NIF. ACKNOWLEDGMENTS Lawrence Livermore National Laboratory is operated by Lawrence Livermore National Security, LLC, for the U.S. De- partment of Energy, National Nuclear Security Administration under Contract No. DE-AC52-07NA27344 (Grant No. LLNL- PROC-694818). 1R. Tommasini et al., Phys. Plasmas 18, 056309 (2011). 2J. K. Crane et al., J. Phys.: Conf. Ser. 244, 032003 (2010). 3G. N. Hall et al., Rev. Sci. Instrum. 85, 11D624 (2014). 4N. Izumi et al., Rev. Sci. Instrum. 85, 11D623 (2014). 5J. J. Lee et al., Proc. SPIE 8505, 850508 (2012). 6J. D. Wiedwald et al., Proc. SPIE 1346, 449 (1991). 7J. L. Wiza, Nucl. Instrum. Methods 162, 587 (1979). 8T. Tabata et al., Nucl. Instrum. Methods Phys. Res. Sect. B 108, 11-17 (1996). 9J. R. Kimbrough et al., Rev. Sci. Instrum. 75, 4060 (2004). 10See http://www.us.schott.com/lightingimaging/english/defenseproducts/ faceplates.html for resolution of fiber optic faceplates. 11C. J. Pawley, Rev. Sci. Instrum. 71, 1286 (2000). Reuse of AIP Publishing content is subject to the terms at: https://publishing.aip.org/authors/rights-and-permissions. Download to IP: 128.115.190.41 On: Wed, 03 Aug 2016 19:02:20