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Quantum oscillations in strongly
correlated electron systems
S.R. Julian
Department of Physics, University of Toronto
•Measuring the Fermi surface:
•Basic theory: Onsager relation
•examples
•Effect of scattering
•Measuring the quasiparticle mass
•Spin dependent effects
•Application to the cuprates
Electron motion is quantized in a
magnetic field.
Fermi surface
Landau tubes
k
∂
∂
=
ε

1
v
B
q
F ×
= v
•Quasiparticles follow lines of constant
energy
• orbit area in k-space is quantized
k-space quantization: (semi)-
classical derivation
Landau tubes
B
ε
n(ε)
εF
k
ε
Landau tubes
The Onsager relation.
Lifshitz-Kosevich Theory
ext
2
A
e
F
π

=
;
2
sin
*
1
~
0
1
2
/
3






+
∝ ∑
∞
=
−
φ
π
B
F
p
p
m
M
p
B1
Applied field B
ε
n(ε)
Harmonic content of dHvA signals
The Fermi surface of Sr2RuO4
C. Bergemann
The Fermi surface of
Sr2RuO4
Mackenzie et al., PRL 1996
B
Electronic structure:
Bergemann, Adv. Phys, 2003
ARPES Fermi surface:
Damascelli et al., Yokoya et al., etc….
Warping patterns on the Fermi surface
Data:amplitude vs field
Bergemann, Adv. Phys, 2003
Amplitude vs field and angle
Allowed warping patterns on the Fermi
surface
Bergemann et al., PRL 85 (2000) 2662.
Impurity and temperature damping
of dHvA signals
Impurity scattering: broadening of Landau levels
o
c l
r
e /
π
−
Applying the Dingle factor to the
surface state in a topological
insulator:
Xiong et al., arXiv:1101.1315:
- Quantum oscillations arise from surface
state.
- Analysis of Dingle factor yields surface
mobility 2,800 cm2/Vs, compared with
about 50 in the bulk
o
c l
r
e /
π
−
Effect of temperature: Fermi function
Derivation of conventional T dependence in dHvA
1
1
/
)
(
)
(
2
+
∝ −
−
∫ kT
e
e
d
N c
i
µ
ε
ω
µ
ε
π
ε 
ε
n(ε)
c
kT
X
X
X
R
T
ω
π 
/
2
sinh
2
where =
=
*
m
eB
c =
ω
Mackenzie et al., PRL 1996
Spin splitting:
A. McCollam, Ph D thesis, 2004
CeRu2Ge2: a ferromagnet with a “small” Fermi
surface
King and Lonzarich,
Physica B 171 (1991) 161.
Backprojection of dHvA frequencies:
Pauli susceptibility is invisible
( )






+
∂
∂
−
=





 +
∂
∂
−
+
=






φ
π
π
π
B
B
F
B
F
B
B
F
B
B
F
B
B
F /
2
sin
/
)
(
2
sin
)
(
2
sin 0
0
0
0 
McCollam et al., PRL, Physica B 2006
Quantum
oscillations in
cuprates
Shubnikov-de Hass
oscillations in ortho-II
ordered YBCO
Doiron-Leyraud et al., Nature 2007
dHvA oscillations in
ortho-II ordered YBCO
Jaudet et al.,
Cond-mat, 26 Nov 07.
Quantum oscillations in the
specific heat:
Riggs et al., Nature Physics, 2011.
F = 531 T
B dependence of C(T) -> sample
is superconducting at high field
How Many Pockets,
and where?
Doiron-Leyraud et al., Nature 2007,
deBoef et al., Nature 2007
How many pockets, and where?
Hossain et al., Nature Physics 2008.
Observation of hole
pocket in
underdoped YBCO?
Sebastian et
al., Nature,
2008
How many pockets, and where?
Audouard et al., PRL 2009: The
main frequency is composed of at
least three components.
How many pockets, and where?
Sebastian et al., PRB2010: similarly sized
electron and hole pockets, with different
corrugations. Electron pocket disappears at
xc.
How many pockets and where?
…
Sebastian et al., Nature
Communications, 2011
Harmonic analysis suggests
only one pocket, probably
nodal, split by bi-layer
splitting?
Carrier density from FS size:
Yelland et al., 2008
What causes the large Fermi
surface to reconstruct?
Chakravarty and Kee, 2007
Spin-splitting of the Fermi surface
Sebastian et al., PRL 2009, no
spin-zeroes. This means SDW is
the symmetry breaking field that
gives small Fermi pockets
More spin-
splitting …
Ramshaw et al., Nature Physics
2011: there are spin zeroes, but
they occur at different angles for
the different oscillatory
components
More spin splitting, more how
many pockets and where …
Sebastian et al., Nature
Communications, 2011: spin
zeroes do exist.
Doping Dependence:
Quantum oscillations in Y124
Yelland et al., PRL, 2007; Bangura et al, PRL 2007.
Doping dependence:
Singleton et al., PRL 2010:
-Higher pulsed field magnets
allow more disordered samples
to be studied
-m* and F vs. doping
Quantum oscillations
in the cuprates
Hussey et al.,
Nature 2003
SdH oscillations in overdoped Tl-
cuprate
Vignolle et al., Nature 2008
Overdoped thallium cuprate ….
The main issue is reconstruction of the Fermi
surface near optimal doping in the cuprates
Conclusions
• Quantum oscillations are a powerful probe of
quasiparticle properties, giving Fermi surface size, and
quasiparticle scattering rates and effective masses
• Impurities are both a problem (you need pure crystals)
and a blessing (you know you are looking at the cleanest
part of your sample)
• In the cuprates, quantum oscillations have established
the existence of long-lived quasiparticles, with
conventional spins, on both the under and over-doped
sides of the phase diagram, and strongly support that the
Fermi surface reconstructs at optimal doping. But the
details of the Fermi surface on the underdoped side are
still controversial.
Thanks: NSERC, CIFAR

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Julian_Toronto_cifar_2012.pdf