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International Journal of Engineering Science Invention
ISSN (Online): 2319 – 6734, ISSN (Print): 2319 – 6726
www.ijesi.org ||Volume 3 Issue 12 || December 2014 || PP.01-03
www.ijesi.org 1 | Page
Natural Radioactivity Levels in Some Villages in Shahjahanpur,
Uttar Pradesh (India)
1,
Anil Kumar , 2,
R B S Rawat , 1,
Dharmendra Kumar , 1,
Prachi Sharma
1
Department of Physics, S S (P.G.) College, Mumukshu Ashram Shahjahanpur, Uttar Pradesh, India, 242001.
2
Department of Physics, M S (P.G.) College, Shaharanpur, Uttar Pradesh, India, 247001
ABSTRACT : Study of indoor radon and its progeny has been carried out in some dwellings of Shahjahanpur,
Uttar Pradesh, India using LR-115 type II plastic track detectors. Radon is an invisible radioactive gas that
occurs naturally in the indoor atmosphere. It comes from the natural breakdown of uranium in soils and rocks.
Lung cancer risk depends upon the concentration of radon and their decay products in air above
recommendation level. In the present study the value of concentration of radon ranges from 28 Bq/m3
to 69
Bq/m3
with an average of 40 Bq/m3
whereas the value of radon progeny ranges from 3.01 mWL to 7.46 mWL
with an average of 4.84 mWL. The results obtained with twin cup radon/thoron dosimeter shows that the
concentration of indoor radon and its progeny were found within recommended levels.
KEYWORDS: Indoor radon, Thoron, Solid state nuclear track detector, Natural Radioactivity.
I. INTRODUCTION
The radioactive element viz. uranium, thorium and potassium are present in traces in the earth’s crust
and are distributed more or less uniformly throughout the crust. These elements emit nuclear radiations, which
can hazards for human beings. Thus the monitoring of any release radioactivity to the environment is necessary
for environmental protection. Studies of natural radioactivity are necessary not only because of their radiological
impact, but also because they act as excellent biochemical and geochemical traces in the environment. Uranium,
the heaviest radioactive toxic elements is found in almost all types of soils, rocks, sands and waters. High values
of uranium in drinking water and foodstuffs may lead to harmful effects in human beings. Adverse effects from
natural uranium can be due to its radioactive and chemical properties. Chemically it can be harmful to the
kidneys from large exposures. Uranium is ultimate source of radium and radon. Radon is the decay product of
uranium present in radioactive series just after the radium. As an inert gas radon can diffuse through the soil and
enter the atmosphere. It is well knownthat (Henshaw et al; 1990) indoor radon exposure is associated with the
risk of leukaemia and certain other cancers such as malenomia and cancers of the kidney and prostate. If
uranium rich material lies close to surface of the earth, there can be high radon exposure hazards (Sevc et al;
1976,UNSCEAR,2000).
Radon is the most common in the environment because its half life of 3.825 days makes its diffusion
more feasible from its origin point towards external air. In the atmosphere, the decay of radon isotopes of
polonium, lead and bismuth (Nikezic and Yu, 2000) that are heavy metals and chemically active. By property,
they exist briefly as ions of free particles in air, forming the molecules in condensed phase or attached to
airborne particles as dust, typically with of size of micron, forming radioactive aerosols. A variable fraction of
airborne radon daughters can remain unattached and is referred as unattached airborne friction. This fraction,
after the inhalation by man, can be deposited in the respiratory tract, in which it releases alpha particles. The
alpha emitted radon progeny is entirely responsible for the absorbed dose due to radon exposure. Thus, the most
appropriate physical quantity associated with dose estimation is not the radon concentration, but the Potential
Alpha Energy Concentration (PAEC). The PAEC is sometimes expressed in terms of the so called equilibrium
equivalent radon concentration (EERC). Based upon current knowledge about health effects of inhaled radon
and its progeny, ICRP has made recommendations for the control of this exposure in dwellings. Keeping this in
mind the natural radioactive levels in Shahjahanpur has been carried out using twin cup radon/thoron dosimeter
with solid state nuclear track detector.
II. MATERIALS AND METHODS.
Radon and its progeny concentration were measured by using LR-115 Type II plastic track detector.
Three small pieces of detector films of size 2.5 cm x 2.5cm were fixed in a twin chamber radon dosimeter
having three different modes. The bare mode gives the values of radon/thoron concentrations and their progeny
while the filter and membrane modes records the values due to radon/thoron and pure radon gas, respectively.
The dosimeters were suspended inside the house at a height of about two meters from the ground floor. After an
Natural radioactivity levels in some villages in…
www.ijesi.org 2 | Page
exposure time of about three months, the detector films were removed, etched and scanned for the track density
measurements. The recorded track density was then converted in the Bq/m3
by using an appropriate calibration
factor [Ramola et. al., 1996].
3.12x10-2
tracks cm-2
d-1
=1 Bqm-3
………. (1)
CR (Bq/m3
) =PAEC (mWL) x 3700/F…….(2)
Where F is the equilibrium factor between radon and its progeny having values 0.4 (UNSCEAR, 1999).
This measurement was repeated on a time integrated four quarterly cycles to cover all the four seasons of a
calendar year.
A twin cup dosimeter based on the above considerations has been designed and developed in the
BARC laboratory for use in the radon-thoron mixed field. This has been effectively deployed in the field for the
measurement of radon-thoron and progeny concentrations in the High Background Radiation Areas (HBRAs)
and in several other areas of the country for a National survey programme. It is a twin chamber cylindrical
system using 12 µm thick, LR-115 type II cellulose nitrate based SSNTDs manufactured by Kodak Pathe,
France. Each chamber has a length of 4.1 cm and a radius of 3.1 cm. The SSNTD1 placed in compartment M
measures radon alone which diffuses into it from the ambient air through a semi-permeable membrane (e.g.
latex, cellulose nitrate etc.) of 25 µm thickness having diffusion coefficient in the range of 10-8
to 10-7
cm2
s-1
[Ilic and Sutej, 1997; Wafaa Arafa, 2002]. It allows the buildup of about 90% of the radon gas in the
compartment and suppresses thoron gas concentration by more than 99%. (The mean time for radon to reach the
steady state concentration inside the cup is about 4.5 h). On the other hand, the glass fiber filter paper of
thickness 0.56 mm in the compartment F allows both radon and thoron gases to diffuse in and hence the tracks
on SSNTD2 placed in this chamber are related to the concentrations of both the gases. The SSNTD3 exposed in
the bare mode (placed on the outer surface of the dosimeter) registers alpha tracks attributable to both the gases
and their alpha emitting progeny, namely
218
Po,
214
Po,
216
Po and
212
Po. The choice of the detector LR-115 is
made in view of the fact that LR-115 detectors do not develop tracks originating from the progeny alphas
deposited on them [Eappen et al, 1998; Nikolaev and Ilic, 1999; Durrani, 1997] and therefore is ideally suited
for air concentration measurements. Fig 1 gives the schematic diagram of the dosimeter.
Fig. 1: SCHEMATIC DIAGRAM OF TWIN CUP RADON-THORON DOSIMETER
III. RESULT AND DISCUSSION.
The concentration of indoor radon and its progeny are shown in table 1.
Based on the results it was found that the radon concentration in study area varied from 28 Bq/m3
to 69 Bq/m3
with an average of 45 Bq/m3
while radon progeny varied 3.01 mWL to 7.46 mWL with an average of 4.84
mWL. The levels of radon and its progeny are higher in villages of Hullapur and Mirjapur as compare to
Piprola, Katra and Jalalabad. Higher concentration in Hullapur and Mijrapur due to the mostly houses taken
under study is mud.The high values of radon and its progeny in the mud house may be due to typical
construction of the houses and the construction materials used. The emanation from the ground surface and from
the building materials of mud houses results in the high value of radon and thoron inside room (Ramola et al.,
1988). As the soil is an important source of indoor radon (Schery 1989), the emanation of radon is also higher
from the ground surface of the house.
Natural radioactivity levels in some villages in…
www.ijesi.org 3 | Page
Table 1 radon and its progeny concentration during summer season.
S. No. Villages No. of dwellings Radon Concentration (Bq/m3
) Radon progeny(mWL)
1 KANT 5 38 4.11
2 JALALABAD 4 32 3.46
3 ALLAHAGANJ 3 35 3.77
4 MIRJAPUR 5 66 7.11
5 TILHAR 8 43 4.65
6 KATRA 3 28 3.01
7 MADNAPUR 4 57 6.14
8 DADRAUL 5 41 4.48
9 BANTHRA 4 39 4.22
10 KALAN 6 54 5.84
11 HULLAPUR 2 69 7.46
12 PIPROLA 2 28 3.03
Min. 28 3.01
Max. 69 7.46
Average 45 4.84
IV. CONCLUSION.
Based on the results it is concluded that the concentration of radon and its progeny levels in mud
houses are higher compared to the other houses. The high concentration of radon and its progeny in mud houses
is possibly because of the poor ventilation condition in the houses. Emanation from the ground surface and from
the building materials of mud houses results high value of radon and its progeny concentration in the houses.
Acknowledgement
Authors are thankful to the house owner’s for their co-operation during this work.
REFERENCE
[1] Durrani, S.A., 1997. Alpha particle etched track detectors. In: Durrani, S.A., Ilic, R. (Eds.), Radon Measurements by Etched Track
Detectors: Application in Radiation Protection, Earth Sciences and the Environment. World Scienti2c, Singapore, pp. 77–101.
[2] Eappen, K.P., Ramachandran, T.V., Mayya, Y.S., Nambi, K.S.V., 1998. LR-115detector response to alpha energies above 5:0 MeV:
application to thoron dosimetry. Proceedings of the Seventh National Symposium of Environment Dhanbad, India. Terrestrial
radiation pro2les in India. Technical Report, BARC.
[3] Henshaw D. L., Eatough J.P.,Richardson R.B.,(1990). Radon as a causative factor in induction of myeloid leukaemia and other
cancers. Lancet.355:1008.
[4] Ilic, R., Sutej, J., 1997. Radon monitoring devices based on etched track detectors. In: Durrani, S.A., Iliac, R. (Eds.), Radon
Measurements by Etched Track Detectors, Applications in Radiation Protection, Earth Sciences and the Environment. World
Scienti2c, Singapore, pp. 103–128.
[5] Nikezic, D. and Yu, K.N. (2000) Relationship between the 210
Po activity incorporated in the surface on an object and the potential
alpha energy concentration, J. environmental Radioactivity.,47,45-55.
[6] Nikolaev, V.A., Iliac, R., 1999. Etched track radiometers in radon measurements: a review. Radiat. Meas. 30, 1–13.
[7] Ramola, R.C., Rawat, R.B.S., Kandari, M.S., Ramachandran, T.V., Eappen, K.P. and Subba Ramu, M.C. (1996) Calibration of LR-
115 Plastic track detector for environmental radon measurements. Indoor Built Environ. 5, 364-366.
[8] Ramola, R.C. Rawat, R.B.S., Kandari, M.S., Ramachandran, T.V., & Choubey, V.M., 1998. A study of seasonal variation of radon
levels in different types of houses. Jour. Environ. Radioactivity. 39 (1), 1-7.
[9] Schery, S.D., Whittlestone, S., Hart, K.P. and Hill, S.E. (1989) the flux of radon and thoron from Australian soils, J. Geophys. Res.
94, 8567-8576.
[10] Sevc J., kunz E., Placek V. Lung cancer in uranium miners and long term exposure to radon daughter products. Health Phys.
1976;30:433.
[11] UNSCEAR (United Nations Scientific Committee on Effects of Atomic Radiation). “Sources and effects of ionizing radiation”.
Report to General Assembly with annexes. United Nations sales Publications E.94.IX.2. United Nations New York. (1999).
[12] UNSCEAR (2000), United Nations Scientific committee on the effects of Atomic Radiations, Report to the General Assembly,
United Nations, New York.
[13] Wafaa Arafa, 2002. Permeability of radon-222 through some material. Radiat. Meas. 35, 207–211.

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A0312010103

  • 1. International Journal of Engineering Science Invention ISSN (Online): 2319 – 6734, ISSN (Print): 2319 – 6726 www.ijesi.org ||Volume 3 Issue 12 || December 2014 || PP.01-03 www.ijesi.org 1 | Page Natural Radioactivity Levels in Some Villages in Shahjahanpur, Uttar Pradesh (India) 1, Anil Kumar , 2, R B S Rawat , 1, Dharmendra Kumar , 1, Prachi Sharma 1 Department of Physics, S S (P.G.) College, Mumukshu Ashram Shahjahanpur, Uttar Pradesh, India, 242001. 2 Department of Physics, M S (P.G.) College, Shaharanpur, Uttar Pradesh, India, 247001 ABSTRACT : Study of indoor radon and its progeny has been carried out in some dwellings of Shahjahanpur, Uttar Pradesh, India using LR-115 type II plastic track detectors. Radon is an invisible radioactive gas that occurs naturally in the indoor atmosphere. It comes from the natural breakdown of uranium in soils and rocks. Lung cancer risk depends upon the concentration of radon and their decay products in air above recommendation level. In the present study the value of concentration of radon ranges from 28 Bq/m3 to 69 Bq/m3 with an average of 40 Bq/m3 whereas the value of radon progeny ranges from 3.01 mWL to 7.46 mWL with an average of 4.84 mWL. The results obtained with twin cup radon/thoron dosimeter shows that the concentration of indoor radon and its progeny were found within recommended levels. KEYWORDS: Indoor radon, Thoron, Solid state nuclear track detector, Natural Radioactivity. I. INTRODUCTION The radioactive element viz. uranium, thorium and potassium are present in traces in the earth’s crust and are distributed more or less uniformly throughout the crust. These elements emit nuclear radiations, which can hazards for human beings. Thus the monitoring of any release radioactivity to the environment is necessary for environmental protection. Studies of natural radioactivity are necessary not only because of their radiological impact, but also because they act as excellent biochemical and geochemical traces in the environment. Uranium, the heaviest radioactive toxic elements is found in almost all types of soils, rocks, sands and waters. High values of uranium in drinking water and foodstuffs may lead to harmful effects in human beings. Adverse effects from natural uranium can be due to its radioactive and chemical properties. Chemically it can be harmful to the kidneys from large exposures. Uranium is ultimate source of radium and radon. Radon is the decay product of uranium present in radioactive series just after the radium. As an inert gas radon can diffuse through the soil and enter the atmosphere. It is well knownthat (Henshaw et al; 1990) indoor radon exposure is associated with the risk of leukaemia and certain other cancers such as malenomia and cancers of the kidney and prostate. If uranium rich material lies close to surface of the earth, there can be high radon exposure hazards (Sevc et al; 1976,UNSCEAR,2000). Radon is the most common in the environment because its half life of 3.825 days makes its diffusion more feasible from its origin point towards external air. In the atmosphere, the decay of radon isotopes of polonium, lead and bismuth (Nikezic and Yu, 2000) that are heavy metals and chemically active. By property, they exist briefly as ions of free particles in air, forming the molecules in condensed phase or attached to airborne particles as dust, typically with of size of micron, forming radioactive aerosols. A variable fraction of airborne radon daughters can remain unattached and is referred as unattached airborne friction. This fraction, after the inhalation by man, can be deposited in the respiratory tract, in which it releases alpha particles. The alpha emitted radon progeny is entirely responsible for the absorbed dose due to radon exposure. Thus, the most appropriate physical quantity associated with dose estimation is not the radon concentration, but the Potential Alpha Energy Concentration (PAEC). The PAEC is sometimes expressed in terms of the so called equilibrium equivalent radon concentration (EERC). Based upon current knowledge about health effects of inhaled radon and its progeny, ICRP has made recommendations for the control of this exposure in dwellings. Keeping this in mind the natural radioactive levels in Shahjahanpur has been carried out using twin cup radon/thoron dosimeter with solid state nuclear track detector. II. MATERIALS AND METHODS. Radon and its progeny concentration were measured by using LR-115 Type II plastic track detector. Three small pieces of detector films of size 2.5 cm x 2.5cm were fixed in a twin chamber radon dosimeter having three different modes. The bare mode gives the values of radon/thoron concentrations and their progeny while the filter and membrane modes records the values due to radon/thoron and pure radon gas, respectively. The dosimeters were suspended inside the house at a height of about two meters from the ground floor. After an
  • 2. Natural radioactivity levels in some villages in… www.ijesi.org 2 | Page exposure time of about three months, the detector films were removed, etched and scanned for the track density measurements. The recorded track density was then converted in the Bq/m3 by using an appropriate calibration factor [Ramola et. al., 1996]. 3.12x10-2 tracks cm-2 d-1 =1 Bqm-3 ………. (1) CR (Bq/m3 ) =PAEC (mWL) x 3700/F…….(2) Where F is the equilibrium factor between radon and its progeny having values 0.4 (UNSCEAR, 1999). This measurement was repeated on a time integrated four quarterly cycles to cover all the four seasons of a calendar year. A twin cup dosimeter based on the above considerations has been designed and developed in the BARC laboratory for use in the radon-thoron mixed field. This has been effectively deployed in the field for the measurement of radon-thoron and progeny concentrations in the High Background Radiation Areas (HBRAs) and in several other areas of the country for a National survey programme. It is a twin chamber cylindrical system using 12 µm thick, LR-115 type II cellulose nitrate based SSNTDs manufactured by Kodak Pathe, France. Each chamber has a length of 4.1 cm and a radius of 3.1 cm. The SSNTD1 placed in compartment M measures radon alone which diffuses into it from the ambient air through a semi-permeable membrane (e.g. latex, cellulose nitrate etc.) of 25 µm thickness having diffusion coefficient in the range of 10-8 to 10-7 cm2 s-1 [Ilic and Sutej, 1997; Wafaa Arafa, 2002]. It allows the buildup of about 90% of the radon gas in the compartment and suppresses thoron gas concentration by more than 99%. (The mean time for radon to reach the steady state concentration inside the cup is about 4.5 h). On the other hand, the glass fiber filter paper of thickness 0.56 mm in the compartment F allows both radon and thoron gases to diffuse in and hence the tracks on SSNTD2 placed in this chamber are related to the concentrations of both the gases. The SSNTD3 exposed in the bare mode (placed on the outer surface of the dosimeter) registers alpha tracks attributable to both the gases and their alpha emitting progeny, namely 218 Po, 214 Po, 216 Po and 212 Po. The choice of the detector LR-115 is made in view of the fact that LR-115 detectors do not develop tracks originating from the progeny alphas deposited on them [Eappen et al, 1998; Nikolaev and Ilic, 1999; Durrani, 1997] and therefore is ideally suited for air concentration measurements. Fig 1 gives the schematic diagram of the dosimeter. Fig. 1: SCHEMATIC DIAGRAM OF TWIN CUP RADON-THORON DOSIMETER III. RESULT AND DISCUSSION. The concentration of indoor radon and its progeny are shown in table 1. Based on the results it was found that the radon concentration in study area varied from 28 Bq/m3 to 69 Bq/m3 with an average of 45 Bq/m3 while radon progeny varied 3.01 mWL to 7.46 mWL with an average of 4.84 mWL. The levels of radon and its progeny are higher in villages of Hullapur and Mirjapur as compare to Piprola, Katra and Jalalabad. Higher concentration in Hullapur and Mijrapur due to the mostly houses taken under study is mud.The high values of radon and its progeny in the mud house may be due to typical construction of the houses and the construction materials used. The emanation from the ground surface and from the building materials of mud houses results in the high value of radon and thoron inside room (Ramola et al., 1988). As the soil is an important source of indoor radon (Schery 1989), the emanation of radon is also higher from the ground surface of the house.
  • 3. Natural radioactivity levels in some villages in… www.ijesi.org 3 | Page Table 1 radon and its progeny concentration during summer season. S. No. Villages No. of dwellings Radon Concentration (Bq/m3 ) Radon progeny(mWL) 1 KANT 5 38 4.11 2 JALALABAD 4 32 3.46 3 ALLAHAGANJ 3 35 3.77 4 MIRJAPUR 5 66 7.11 5 TILHAR 8 43 4.65 6 KATRA 3 28 3.01 7 MADNAPUR 4 57 6.14 8 DADRAUL 5 41 4.48 9 BANTHRA 4 39 4.22 10 KALAN 6 54 5.84 11 HULLAPUR 2 69 7.46 12 PIPROLA 2 28 3.03 Min. 28 3.01 Max. 69 7.46 Average 45 4.84 IV. CONCLUSION. Based on the results it is concluded that the concentration of radon and its progeny levels in mud houses are higher compared to the other houses. The high concentration of radon and its progeny in mud houses is possibly because of the poor ventilation condition in the houses. Emanation from the ground surface and from the building materials of mud houses results high value of radon and its progeny concentration in the houses. Acknowledgement Authors are thankful to the house owner’s for their co-operation during this work. REFERENCE [1] Durrani, S.A., 1997. Alpha particle etched track detectors. In: Durrani, S.A., Ilic, R. (Eds.), Radon Measurements by Etched Track Detectors: Application in Radiation Protection, Earth Sciences and the Environment. World Scienti2c, Singapore, pp. 77–101. [2] Eappen, K.P., Ramachandran, T.V., Mayya, Y.S., Nambi, K.S.V., 1998. LR-115detector response to alpha energies above 5:0 MeV: application to thoron dosimetry. Proceedings of the Seventh National Symposium of Environment Dhanbad, India. Terrestrial radiation pro2les in India. Technical Report, BARC. [3] Henshaw D. L., Eatough J.P.,Richardson R.B.,(1990). Radon as a causative factor in induction of myeloid leukaemia and other cancers. Lancet.355:1008. [4] Ilic, R., Sutej, J., 1997. Radon monitoring devices based on etched track detectors. In: Durrani, S.A., Iliac, R. (Eds.), Radon Measurements by Etched Track Detectors, Applications in Radiation Protection, Earth Sciences and the Environment. World Scienti2c, Singapore, pp. 103–128. [5] Nikezic, D. and Yu, K.N. (2000) Relationship between the 210 Po activity incorporated in the surface on an object and the potential alpha energy concentration, J. environmental Radioactivity.,47,45-55. [6] Nikolaev, V.A., Iliac, R., 1999. Etched track radiometers in radon measurements: a review. Radiat. Meas. 30, 1–13. [7] Ramola, R.C., Rawat, R.B.S., Kandari, M.S., Ramachandran, T.V., Eappen, K.P. and Subba Ramu, M.C. (1996) Calibration of LR- 115 Plastic track detector for environmental radon measurements. Indoor Built Environ. 5, 364-366. [8] Ramola, R.C. Rawat, R.B.S., Kandari, M.S., Ramachandran, T.V., & Choubey, V.M., 1998. A study of seasonal variation of radon levels in different types of houses. Jour. Environ. Radioactivity. 39 (1), 1-7. [9] Schery, S.D., Whittlestone, S., Hart, K.P. and Hill, S.E. (1989) the flux of radon and thoron from Australian soils, J. Geophys. Res. 94, 8567-8576. [10] Sevc J., kunz E., Placek V. Lung cancer in uranium miners and long term exposure to radon daughter products. Health Phys. 1976;30:433. [11] UNSCEAR (United Nations Scientific Committee on Effects of Atomic Radiation). “Sources and effects of ionizing radiation”. Report to General Assembly with annexes. United Nations sales Publications E.94.IX.2. United Nations New York. (1999). [12] UNSCEAR (2000), United Nations Scientific committee on the effects of Atomic Radiations, Report to the General Assembly, United Nations, New York. [13] Wafaa Arafa, 2002. Permeability of radon-222 through some material. Radiat. Meas. 35, 207–211.