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International Journal of Trend in Scientific Research and Development (IJTSRD)
Volume 6 Issue 6, September-October 2022 Available Online: www.ijtsrd.com e-ISSN: 2456 – 6470
@ IJTSRD | Unique Paper ID – IJTSRD52250 | Volume – 6 | Issue – 6 | September-October 2022 Page 2163
Radioactivity of Some Soil Samples from Kuba, Butura Ward,
Bokkos Local Government Area, Plateau State, Nigeria
Chenko G. Y. N1
, Mangset W. E2
, Terve S. J3
1
Department of Physics, Faculty of Natural Sciences, Plateau State University, Bokkos, Nigeria
2
Department of Physics, Faculty of Natural Sciences, University of Jos, Jos, Nigeria
3
Department of Chemistry Faculty of Natural Sciences, Plateau State University, Bokkos, Nigeria
ABSTRACT
The activity concentration of naturally occurring radionuclide 40
K,
226
Ra and 232
Th were measured in some soil samples from Kuba
village, Bokkos Local Government Area, Plateau State, Nigeria using
gamma ray spectroscopy. The soil activity ranges from 246.40±
11.32, 129.40± 6.44 and 57.92± 22 Bq.kg-1
respectively 116.70± 9.24
to 397.2± 13.32Bq.Kg -1
for 40
K, 35.87± 1.02 to 88.09±1.14 Bq.kg-1
for 226
Ra, and 103.60± 5.23 to 162.10± 7.11 .Kg-1
for 232
Th with
mean values of 246.40±11.32, 57.92±1.22 and 246.40±11.32 Bq.kg -1
respectively. The concentrations of these radionuclides are compared
with the world average. The radium equivalent activity calculated
from the analyzed soil samples ranges from 200.2536 to 291.9765
Bq.Kg-1
with the mean value of 261.0386 Bq.Kg-1
. The mean values
40
K and Radium Equivalent are low compare to the world average but
the mean values for, 226
Raand232
Th are above the permissible value,
therefore pose a significant threat to inhabitants or workers dealing
with transportation of soil and there is no good safety index for all
building made from these materials and the inhabitants due to high
activity concentration of 232
Th and 226
Ra.
KEYWORDS: Radionuclides, Radium Equivalent Dose, 40
K, 226
Ra
and 232
Th
How to cite this paper: Chenko G. Y. N
| Mangset W. E | Terve S. J
"Radioactivity of Some Soil Samples
from Kuba, Butura Ward, Bokkos Local
Government Area, Plateau State,
Nigeria" Published
in International
Journal of Trend in
Scientific Research
and Development
(ijtsrd), ISSN: 2456-
6470, Volume-6 |
Issue-6, October
2022, pp.2163-2166, URL:
www.ijtsrd.com/papers/ijtsrd52250.pdf
Copyright © 2022 by author(s) and
International Journal of Trend in
Scientific Research and Development
Journal. This is an
Open Access article
distributed under the
terms of the Creative Commons
Attribution License (CC BY 4.0)
(http://creativecommons.org/licenses/by/4.0)
INTRODUCTION
Natural background radioactivity and the associated
external exposure due to gamma radiation depend
primarily on the geological and geographical
conditions and appear at different levels in the soils of
each region in the world. The knowledge of this
natural radioactivity distribution in the environment is
essential in various fields of science. The high
geochemical mobility of radionuclides in the
environment allows them to move easily and to
contaminate much of the environment with which
humans come in contact therefore it is important to
know the distribution of source –rock materials
containing elevated levels of radionuclides processes
that concentrate the radionuclides.
The meaning of the word soil varies in different fields
depending upon its relevance. Farmers consider it as
the part of the earth’s surface containing decayed and
organic materials in sufficient quantity to grow plants
and crops. The Geologist see it as the left over from
underlying parent rock that support root growth. To
the engineer, soil include all earth materials overlying
the rock crust and contain particles of minerals, gases
and liquids. According to the soil science society of
America (SSSA) soil is a living system that represents
a finite resource vital to life on earth. It forms the thin
skin of unconsolidated mineral and organic matter on
the earth’s surface, and develops slowly from various
parent materials and is modified by time, climate,
macro-and microorganisms, vegetation and
topography.
Soil contain organic, inorganic compounds and also
radionuclides. The naturally occurring radionuclides
present in soil include 226
Ra,226
Ra 232
Th and 40
K. The
gamma radiation emitted from these naturally
occurring radioisotopes called terrestrials background
radiation, represents the main source of irradiation to
the populace and contribute to the total absorbed dose
via inhalation, ingestion and external irradiation
calculate by beck suggested that 50-80 percentage of
IJTSRD52250
International Journal of Trend in Scientific Research and Development @ www.ijtsrd.com eISSN: 2456-6470
@ IJTSRD | Unique Paper ID – IJTSRD52250 | Volume – 6 | Issue – 6 | September-October 2022 Page 2164
the total gamma flux at the earth surface arises from
40
K, 238
U and 232
Th series in topsoil.
Kuba Village, in Bokkos Local Government Area,
Plateau State, Nigeria is one of the oldest tin mining
area in Plateau State. Due to the mining activity over
acentury, the bricks laying and plastering soil samples
were measured to assess the magnitude of the
radionuclides content.
THE STUDY AREA
This study was conducted in and around Kuba
community where local bricks are made for building
and Plastering sand are collected for finishing of most
of residential houses in of Butura Ward, in Bokkos
Local Government Area of Plateau State, Nigeria.
The samples were collected along Kuba-Bagodu road,
Kuba-Kafuta road and Kuba-Kafuta road
MATERIALS AND METHODS
In order to measure natural radioactivity in soil, ten
surface samples were collected from from three
different sites. After removing the stone and organic
materials, the sample were dried in an oven at about
1500C for 1-2h to remove the moisture content and
then crushed to pass through a 150 mesh sieve to
homogenize it. The representative powered samples
were filled in a polyethylene circular disc of 55-m
diameter and 13 mm height. finally, every sample was
stored for four weeks to reach the equilibrium state
between radon and its decay products, since radium
measurements are usually based on the activities of
radon daughters 214
Bi, 214
Pb and then the gamma ray
spectrum was accumulated for up to 900min. the
method is discuss in earlier publication. Each sample
was subjected to a gamma ray spectrometer with HP
Ge setup and multichannel analyzer. The applied low-
level gamma –ray spectrometer consists basically of
high purity germanium detector with its electronic
circuit. The detector is coaxial closed end closed
facing window geometry with vertical dipstick (500-
800microns) the HPGe GEM is P-Type with the
following specifications.
Resolution (FWHM) at 122keV,57Co
is 1100eV and at
1.33 MeV, 60
Co is 2.00 K e V peak-to Compton
Ratio, 60
Co is 46, relative’s efficiency at 1. 33 Me V,
60
Co is 20% operation bias voltage is +2000 V dc.
The detector is shielded in a chamber of four layers
starting with Plexiglas (10mm thick) copper (30mm
thick) lead (100mm thick) and finally cadmium (3mm
thick) this shield serves In reducing different
radiation hazards. The soft component of cosmic rays,
consisting of photons and electrons, is reduced to
avery low level by 100mm of the lead shielding. The
x-rays (73.9keV) emitted from lead by its interaction
with external radiation is suppressed by the cupper
layer.
The emitted x-rays from lead which contains
radioactive impurities due to antimonyimpurities due
to antimony impurities can be absorbed by lining the
inside of the shield with a graded layer of 0.05 inch
cadmium and 0.25 inch prespex. To minimize the
effect of the scattered radiation from the shield, the
detector is located in the chamber.
The spectra were evaluated with the computer
software program maestro (EG &GORTIC) or
manually with the use of a spread sheet (micro excel)
to calculate the natural radioactivity, 226 Ra activity
of the sample was determined through the intensity of
the 295.2 keV, 351.9keV and 609.3keV y-lines for
214
Pb and 214
Bi respectively. 232
Th activity was
determined through 238, 583.1 and 911.1 keV y-lines
for 212
Pb, 208TI and 228
Ac respectively 40
K measured
directly through the gamma line emission at
1460.8keV.
TABLE OF RESULTS: Activity Concentration of K,Ra and Th (B/Kg)
CK CTh CRa Raeq
Kuba-Bagodu road
1 397.20±13.32 146.7±5.33 44.19±1.22 289.79
2 211.70±9.13 118.3±6.44 35.93±1.11 214.97
3 129.80±11.51 162.1±7.11 37.88±1.33 278.73
Kuba-Kafuta road
1 116.70±9.24 103.6±5.23 43.87±1.02 200.35
2 182.10±10.31 140.1±7.61 52.58±1.42 265.77
3 321.00±14.41 133.5±6.48 78.65±1.22 292.08
Kuba-Butura road
1 347.30±13.23 142±6.37 49.09±1.03 276.58
2 215.80±10.61 110.4±6.51 60.81±1.41 233.83
3 263.30±11.42 119.9±7.34 93.16±1.30 283.02
4 275.10±10.22 117.8±5.54 88.09±1.14 275.95
AVERAGE 246.40±11.32 129.4±6.44 57.92±1.22 261.04
40
K, 232
Th and 226
Ra, activity concentrations measured in soil samples Kuba
International Journal of Trend in Scientific Research and Development @ www.ijtsrd.com eISSN: 2456-6470
@ IJTSRD | Unique Paper ID – IJTSRD52250 | Volume – 6 | Issue – 6 | September-October 2022 Page 2165
All the values of the activity per unit mass are in the
range of the corresponding typical world values
which 400Bq.kg-1 for 40
K while for 232
Th an 226
Ra
the values obtained are above the world permissible
limit of 30Bq/Kg. and 35Bq/Kg (UNSCEAR,2000)
respectively. The results of the present work indicate
that the area under investigation may has a high level
of natural background radiation, so these materials do
pose a significant radiological hazard when used for
construction of buildings and even the workers.
RADIUM EQUIVALENT ACTIVITY (Raeq): The
associated radium equivalent activity was calculated
using the formula
Raeq = CRa+ 1.43CTh + 0.077C
k
Where :CRa and CK are the specific activities of 226
Ra
and 40
K in Bq.kg-1
respectively. The radium
equivalent activities of samples under investigation
were calculated on the basis of the above equation
and are shown in the table above. For all soil samples
under investigation, the radium equivalent value are
lower than the acceptable value of 370 Bq.Kg-1
,
ranging from 200.35 to 289.79 Bq.kg-1
CONCLUSIONS
The investigation carried out showed the the results of
measuring the activity concentrated of terrestrial
gamma emitters for soil samples from Kuba village,
Butura ward of Bokkos Local Government Area,
Plateau State, Nigeria. The results obtain indicate that
there could be high exposure for either inhabitants or
workers dealing with transportation of soil and there
is no good safety index for all building made from
these materials and the inhabitants due to high
activity concentration of 232
Th and 226
Ra.
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[3] Khan, K., H.M. Khan, M. Tufail and N.
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Environment Radioactivity, 38. 77-83.
[4] Beck, H.L., 1972. The physics of
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Proceeding of the Second International
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Radioactivity of Some Soil Samples from Kuba, Butura Ward, Bokkos Local Government Area, Plateau State, Nigeria

  • 1. International Journal of Trend in Scientific Research and Development (IJTSRD) Volume 6 Issue 6, September-October 2022 Available Online: www.ijtsrd.com e-ISSN: 2456 – 6470 @ IJTSRD | Unique Paper ID – IJTSRD52250 | Volume – 6 | Issue – 6 | September-October 2022 Page 2163 Radioactivity of Some Soil Samples from Kuba, Butura Ward, Bokkos Local Government Area, Plateau State, Nigeria Chenko G. Y. N1 , Mangset W. E2 , Terve S. J3 1 Department of Physics, Faculty of Natural Sciences, Plateau State University, Bokkos, Nigeria 2 Department of Physics, Faculty of Natural Sciences, University of Jos, Jos, Nigeria 3 Department of Chemistry Faculty of Natural Sciences, Plateau State University, Bokkos, Nigeria ABSTRACT The activity concentration of naturally occurring radionuclide 40 K, 226 Ra and 232 Th were measured in some soil samples from Kuba village, Bokkos Local Government Area, Plateau State, Nigeria using gamma ray spectroscopy. The soil activity ranges from 246.40± 11.32, 129.40± 6.44 and 57.92± 22 Bq.kg-1 respectively 116.70± 9.24 to 397.2± 13.32Bq.Kg -1 for 40 K, 35.87± 1.02 to 88.09±1.14 Bq.kg-1 for 226 Ra, and 103.60± 5.23 to 162.10± 7.11 .Kg-1 for 232 Th with mean values of 246.40±11.32, 57.92±1.22 and 246.40±11.32 Bq.kg -1 respectively. The concentrations of these radionuclides are compared with the world average. The radium equivalent activity calculated from the analyzed soil samples ranges from 200.2536 to 291.9765 Bq.Kg-1 with the mean value of 261.0386 Bq.Kg-1 . The mean values 40 K and Radium Equivalent are low compare to the world average but the mean values for, 226 Raand232 Th are above the permissible value, therefore pose a significant threat to inhabitants or workers dealing with transportation of soil and there is no good safety index for all building made from these materials and the inhabitants due to high activity concentration of 232 Th and 226 Ra. KEYWORDS: Radionuclides, Radium Equivalent Dose, 40 K, 226 Ra and 232 Th How to cite this paper: Chenko G. Y. N | Mangset W. E | Terve S. J "Radioactivity of Some Soil Samples from Kuba, Butura Ward, Bokkos Local Government Area, Plateau State, Nigeria" Published in International Journal of Trend in Scientific Research and Development (ijtsrd), ISSN: 2456- 6470, Volume-6 | Issue-6, October 2022, pp.2163-2166, URL: www.ijtsrd.com/papers/ijtsrd52250.pdf Copyright © 2022 by author(s) and International Journal of Trend in Scientific Research and Development Journal. This is an Open Access article distributed under the terms of the Creative Commons Attribution License (CC BY 4.0) (http://creativecommons.org/licenses/by/4.0) INTRODUCTION Natural background radioactivity and the associated external exposure due to gamma radiation depend primarily on the geological and geographical conditions and appear at different levels in the soils of each region in the world. The knowledge of this natural radioactivity distribution in the environment is essential in various fields of science. The high geochemical mobility of radionuclides in the environment allows them to move easily and to contaminate much of the environment with which humans come in contact therefore it is important to know the distribution of source –rock materials containing elevated levels of radionuclides processes that concentrate the radionuclides. The meaning of the word soil varies in different fields depending upon its relevance. Farmers consider it as the part of the earth’s surface containing decayed and organic materials in sufficient quantity to grow plants and crops. The Geologist see it as the left over from underlying parent rock that support root growth. To the engineer, soil include all earth materials overlying the rock crust and contain particles of minerals, gases and liquids. According to the soil science society of America (SSSA) soil is a living system that represents a finite resource vital to life on earth. It forms the thin skin of unconsolidated mineral and organic matter on the earth’s surface, and develops slowly from various parent materials and is modified by time, climate, macro-and microorganisms, vegetation and topography. Soil contain organic, inorganic compounds and also radionuclides. The naturally occurring radionuclides present in soil include 226 Ra,226 Ra 232 Th and 40 K. The gamma radiation emitted from these naturally occurring radioisotopes called terrestrials background radiation, represents the main source of irradiation to the populace and contribute to the total absorbed dose via inhalation, ingestion and external irradiation calculate by beck suggested that 50-80 percentage of IJTSRD52250
  • 2. International Journal of Trend in Scientific Research and Development @ www.ijtsrd.com eISSN: 2456-6470 @ IJTSRD | Unique Paper ID – IJTSRD52250 | Volume – 6 | Issue – 6 | September-October 2022 Page 2164 the total gamma flux at the earth surface arises from 40 K, 238 U and 232 Th series in topsoil. Kuba Village, in Bokkos Local Government Area, Plateau State, Nigeria is one of the oldest tin mining area in Plateau State. Due to the mining activity over acentury, the bricks laying and plastering soil samples were measured to assess the magnitude of the radionuclides content. THE STUDY AREA This study was conducted in and around Kuba community where local bricks are made for building and Plastering sand are collected for finishing of most of residential houses in of Butura Ward, in Bokkos Local Government Area of Plateau State, Nigeria. The samples were collected along Kuba-Bagodu road, Kuba-Kafuta road and Kuba-Kafuta road MATERIALS AND METHODS In order to measure natural radioactivity in soil, ten surface samples were collected from from three different sites. After removing the stone and organic materials, the sample were dried in an oven at about 1500C for 1-2h to remove the moisture content and then crushed to pass through a 150 mesh sieve to homogenize it. The representative powered samples were filled in a polyethylene circular disc of 55-m diameter and 13 mm height. finally, every sample was stored for four weeks to reach the equilibrium state between radon and its decay products, since radium measurements are usually based on the activities of radon daughters 214 Bi, 214 Pb and then the gamma ray spectrum was accumulated for up to 900min. the method is discuss in earlier publication. Each sample was subjected to a gamma ray spectrometer with HP Ge setup and multichannel analyzer. The applied low- level gamma –ray spectrometer consists basically of high purity germanium detector with its electronic circuit. The detector is coaxial closed end closed facing window geometry with vertical dipstick (500- 800microns) the HPGe GEM is P-Type with the following specifications. Resolution (FWHM) at 122keV,57Co is 1100eV and at 1.33 MeV, 60 Co is 2.00 K e V peak-to Compton Ratio, 60 Co is 46, relative’s efficiency at 1. 33 Me V, 60 Co is 20% operation bias voltage is +2000 V dc. The detector is shielded in a chamber of four layers starting with Plexiglas (10mm thick) copper (30mm thick) lead (100mm thick) and finally cadmium (3mm thick) this shield serves In reducing different radiation hazards. The soft component of cosmic rays, consisting of photons and electrons, is reduced to avery low level by 100mm of the lead shielding. The x-rays (73.9keV) emitted from lead by its interaction with external radiation is suppressed by the cupper layer. The emitted x-rays from lead which contains radioactive impurities due to antimonyimpurities due to antimony impurities can be absorbed by lining the inside of the shield with a graded layer of 0.05 inch cadmium and 0.25 inch prespex. To minimize the effect of the scattered radiation from the shield, the detector is located in the chamber. The spectra were evaluated with the computer software program maestro (EG &GORTIC) or manually with the use of a spread sheet (micro excel) to calculate the natural radioactivity, 226 Ra activity of the sample was determined through the intensity of the 295.2 keV, 351.9keV and 609.3keV y-lines for 214 Pb and 214 Bi respectively. 232 Th activity was determined through 238, 583.1 and 911.1 keV y-lines for 212 Pb, 208TI and 228 Ac respectively 40 K measured directly through the gamma line emission at 1460.8keV. TABLE OF RESULTS: Activity Concentration of K,Ra and Th (B/Kg) CK CTh CRa Raeq Kuba-Bagodu road 1 397.20±13.32 146.7±5.33 44.19±1.22 289.79 2 211.70±9.13 118.3±6.44 35.93±1.11 214.97 3 129.80±11.51 162.1±7.11 37.88±1.33 278.73 Kuba-Kafuta road 1 116.70±9.24 103.6±5.23 43.87±1.02 200.35 2 182.10±10.31 140.1±7.61 52.58±1.42 265.77 3 321.00±14.41 133.5±6.48 78.65±1.22 292.08 Kuba-Butura road 1 347.30±13.23 142±6.37 49.09±1.03 276.58 2 215.80±10.61 110.4±6.51 60.81±1.41 233.83 3 263.30±11.42 119.9±7.34 93.16±1.30 283.02 4 275.10±10.22 117.8±5.54 88.09±1.14 275.95 AVERAGE 246.40±11.32 129.4±6.44 57.92±1.22 261.04 40 K, 232 Th and 226 Ra, activity concentrations measured in soil samples Kuba
  • 3. International Journal of Trend in Scientific Research and Development @ www.ijtsrd.com eISSN: 2456-6470 @ IJTSRD | Unique Paper ID – IJTSRD52250 | Volume – 6 | Issue – 6 | September-October 2022 Page 2165 All the values of the activity per unit mass are in the range of the corresponding typical world values which 400Bq.kg-1 for 40 K while for 232 Th an 226 Ra the values obtained are above the world permissible limit of 30Bq/Kg. and 35Bq/Kg (UNSCEAR,2000) respectively. The results of the present work indicate that the area under investigation may has a high level of natural background radiation, so these materials do pose a significant radiological hazard when used for construction of buildings and even the workers. RADIUM EQUIVALENT ACTIVITY (Raeq): The associated radium equivalent activity was calculated using the formula Raeq = CRa+ 1.43CTh + 0.077C k Where :CRa and CK are the specific activities of 226 Ra and 40 K in Bq.kg-1 respectively. The radium equivalent activities of samples under investigation were calculated on the basis of the above equation and are shown in the table above. For all soil samples under investigation, the radium equivalent value are lower than the acceptable value of 370 Bq.Kg-1 , ranging from 200.35 to 289.79 Bq.kg-1 CONCLUSIONS The investigation carried out showed the the results of measuring the activity concentrated of terrestrial gamma emitters for soil samples from Kuba village, Butura ward of Bokkos Local Government Area, Plateau State, Nigeria. The results obtain indicate that there could be high exposure for either inhabitants or workers dealing with transportation of soil and there is no good safety index for all building made from these materials and the inhabitants due to high activity concentration of 232 Th and 226 Ra. RERENCES [1] Malanca, A, L. Gaidolif, V. Pessina and G. Dallara 1996. Distribution of 226Ra, 232Th and 40K in soils of rio Grande do Norte (Brazil). Journal of environmental radioactivity 30:55-67. [2] UNSCEAR, 200. United Nations Scientific Committee assembly. Annex B. exposure from natural radiation sources. New York. United Nations. [3] Khan, K., H.M. Khan, M. Tufail and N. Ahmed, 1998 Radiometric analysis of hazara phosphate rock and fertilizers kurnals of Environment Radioactivity, 38. 77-83. [4] Beck, H.L., 1972. The physics of environmental gamma radiation filed. Proceeding of the Second International Symposium on the natural radiation environment. Houston Texas, 101-131. [5] Khan. H.M K. Khan, M.A. Atta and F. Jan, 1994. Measurement of gamma activity of soil samples of charsadda district of Pakistan; Journal of chemical society of Pakistan, 16:183-188. [6] Sroor, A, S.M. El-Bahi, F Ahmed and A.S AbdelHaleem, 2001. Natural radioactivity and radon exhalaition rate of soil in southern in southern in Egypt. Applied Radiation and Isotopes, 55:873-879. [7] Chiozzi, P., V. Pasquale and M. Verdoya, 2002 Naturallyoccuring radioactivity at the Alps Apenines transition. Radiation Measurement, 35:147-154. [8] El-Arabi, A.M, 2005 Gamma activity in some Environmental samples in south Egypt. Indian Journal of pure and Applied Physics, 43:422- 426. [9] Aziz, A 1981, method of low-level counting and spectrometry symposium. Berlin, 221. [10] Beretka, J. and P.J. Mathew, 1985. Natural radioactivity of Austrialian building materals, industrial wates and by-products. Health Physics 48:87-95. [11] Veiga, R., N. Sanches, R.M, Anjos, K Macario. J. Bastos, M. Iguatemy, J.G. Aguiar, A.M.A Santos B. Mosquera, C. Carcalho, M Baptistafilho and N.K. Umisedo, 2006. Measurement of natural radioactivity in Brazilian beach sands. Radiation Measurement 41:189-196. [12] Al-Jundi, J., B.A. Al-Bataina, Y. bu-Rukan and H.H Shehadeh, 2003. Natural radioactivity concentrations in soil samples along the Amma Aqaba Highway, Jordan, Radiation Measurements, 36:555-560. [13] Steinhausler, F, 1992 The natural radiation environment future prospective Radiation protection Dosimetry, 45:1/4, 19-23. [14] Karahan, G and A Buyulken, 2000. Assessment of gamma dose rates around istanbul, Journal of Environmental Radioactivity 47:213-221. [15] Chowdhury, M.I., M. Kamal, M.N Alam, SalahaYeasmin and M.N. Mostafa, 2006. Distribution of naturally occurring radionuclide’s in soils of the southern Districts of Bangladesh. Radiation protection Dosimetry Journal, 118:126-130. [16] Ahmed, N.K., and A.M. Arabi 2005. Natural radioactivity in farm soil and phosphate
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