This document summarizes research on a hematite photoanode coated with a nickel-iron hydroxide catalyst layer for water splitting. The coating was applied via a "zippering" method using sodium citrate to provide a conformal, void-free layer on hematite nanowire arrays. Characterization showed the coating achieved intimate contact between the hematite and catalyst. Photoelectrochemical tests demonstrated the coated electrode had a lower oxygen evolution reaction turn-on potential, higher charge transfer efficiency, and greater stability compared to uncoated hematite. The zippered interface improved the photoanode performance for water oxidation.