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Generalized spin
fluctuation feedback effect
and the tale of two
transitionsAdil Amin
&
Daniel F. Agterberg
University of Wisconsin-Milwaukee
arXiv:1910.10780
arXiv:1910.10780
Accepted : Physics Review Research
Experimental Survey
UPt3 𝑈1−𝑥 𝑇ℎ 𝑥 𝐵𝑒13
𝑃𝑟𝑂𝑠4 𝑆𝑏12
Hasselbach et al. 1989 Kim et al. 1991 Vollmer et al. 2003
Specific HeatTime Reversal Symmetry Breaking
Schemm et al. 2014 Heffner et al 1990 Levenson-Falk et al. 2018
Low Energy Excitations
Spin fluctuations : (Inelastic) Neutron Scattering
Aeppli et al. 1988
Antiferromagnetic (AFM) fluctuations
Hiess et al. 2002
AFM fluctuations
Kaneko 2007 et al.
Antiferroquadrapolar (AFQ) fluctuations
Q= (1/2,0,0) Q= (1/2,1/2,0) Q= (1,0,0)
Neutron Scattering Inelastic Neutron Scattering Inelastic Neutron Scattering
UPt3 𝑈1−𝑥 𝑇ℎ 𝑥 𝐵𝑒13 𝑃𝑟𝑂𝑠4 𝑆𝑏12
Common Mechanism?
Multi dimensional irreps (order parameter)
UPt3 𝑈1−𝑥 𝑇ℎ 𝑥 𝐵𝑒13 𝑃𝑟𝑂𝑠4 𝑆𝑏12
3D (T irreps)
2D (E irreps)
2D (E irreps)
3D (T irreps)
2D (E irreps)
A : (1,0) Nematic TRS
B : (1,i) Broken TRS
A : Time Reversal Symmetry (TRS)
B: Time reversal Symmetry Breaking (TRSB)
Hexagonal : 𝐷6ℎ
Tetrahedral: 𝑇ℎOctarahedral: 𝑂ℎ
𝑇𝑐𝐴 = 550𝑚𝐾
𝑇𝑐𝐵 = 480𝑚𝐾
𝑈𝑃𝑡3
𝛽2> 0
(1,i)
𝛽2 < 0
(1,0)
Two transitions ??
AFM → Symmetry Breaking Field :
But AFM not long ranged
Kioke et. Al 1998
3He
Add coupling to paramagnetic fluctuations
Large fluctuations imply 𝐴1 → 0 and +ve
𝑑 𝑎 = 𝑘 𝑥 + 𝑖𝑘 𝑦 𝒛
𝑑 𝑏 = 𝑘
A phase puzzling : weak coupling → B stable always
We want phenomenogical model
Resolved by Anderson & Brinkman : Spin fluctuation feedback effect
Couple superfluidity + spin fluctuations : Microscopic
The SFEE cheat code
Integrate out the Gaussian spin fluctuations
𝑓𝐵 − 𝑓𝐴=
3𝐾2
2
𝐴1
2 , A : Stable with large fluctuations (𝐴1 → 0)
A—B transition : temperature dependence
𝛽 →
1
𝑇2 , 𝐾 →
1
𝑇
[ Brinkman et al. 1973, Kozii 2019]
Start in A state (SFFE) : T ↓ : → B state (weak coupling)
Back to 𝑈𝑃𝑡3
Add a coupling between superconductivity and AFM fluctuations
Q1 =
1
2
a*, Q2 =
1
2
(b*-a*), Q3 = −
1
2
b*𝑚1, 𝑚2 and 𝑚3 →
New effective free energy
𝛽2 > 0 but ( 𝛽2-
6
4
𝐾2
2
𝐴1
2 ) < 0 → (1,0) : nematic TRS A state
A → B TRSB (1,i) as T ↓
𝑈1−𝑥 𝑇ℎ 𝑥 𝐵𝑒13
𝑂ℎ: AFM fluctuations : TRSB ( 𝜇SR)
2D Case
* → Kerr Inactive : Ruled out by possible Kerr measurement
3D Case
Ruled out by coupling
See paper
A
B
A
B
𝑃𝑟𝑂𝑠4 𝑆𝑏12
Aoki et al 2003
𝑇ℎ: AFQ fluctuations : TRSB ( 𝜇SR + Polar Kerr)
2D Case
A—B Kerr Inactive
3D Case
A
B
Take away
• Developed a simple and quick phenomenological approach to generalized SFFE
• Provides a unifying description of two transitions in heavy fermion superconductors
• 2D 𝐸 𝑔/𝑢 for 𝑃𝑟𝑂𝑠4 𝑆𝑏12 ruled out by polar Kerr
• For 𝑈1−𝑥 𝑇ℎ 𝑥 𝐵𝑒13, form SFFE allows only one out of two possible A states
• Suggest polar Kerr measurements for 𝑈1−𝑥 𝑇ℎ 𝑥 𝐵𝑒13 → can rule out 2D 𝐸 𝑔/𝑢 rep scenario and constrain 3D (𝑇𝑔/𝑢) situation
https://arxiv.org/abs/1910.10780
Thank you and Questions
https://arxiv.org/abs/1910.10780
Effective theory for A—B transitions
• Start out in A state of UP𝑡3 stabilized by SFFE i.e. (1,0) with for and for
• Grow B phase continuously out of A , i.e. (1 + 𝜂1𝑅 + 𝜂1𝐼, 0 + 𝜂2𝑅+𝜂2𝐼)
• Use time reversal symmetry to classify these effective order parameter
Want to break time reversal
Character table for 𝐷2
→ 𝐴1 → 𝐵1
Now use polar Kerr effect
Signal trainable by field → order parameter TRSB & has same symmetry as magnetic field (𝑅 𝑥, 𝑅 𝑦, 𝑅 𝑧)
Schemm et . al 2014

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Generalized Spin Fluctuation Feedback in Heavy Fermion Superconductors

  • 1. Generalized spin fluctuation feedback effect and the tale of two transitionsAdil Amin & Daniel F. Agterberg University of Wisconsin-Milwaukee arXiv:1910.10780 arXiv:1910.10780 Accepted : Physics Review Research
  • 2. Experimental Survey UPt3 𝑈1−𝑥 𝑇ℎ 𝑥 𝐵𝑒13 𝑃𝑟𝑂𝑠4 𝑆𝑏12 Hasselbach et al. 1989 Kim et al. 1991 Vollmer et al. 2003 Specific HeatTime Reversal Symmetry Breaking Schemm et al. 2014 Heffner et al 1990 Levenson-Falk et al. 2018
  • 3. Low Energy Excitations Spin fluctuations : (Inelastic) Neutron Scattering Aeppli et al. 1988 Antiferromagnetic (AFM) fluctuations Hiess et al. 2002 AFM fluctuations Kaneko 2007 et al. Antiferroquadrapolar (AFQ) fluctuations Q= (1/2,0,0) Q= (1/2,1/2,0) Q= (1,0,0) Neutron Scattering Inelastic Neutron Scattering Inelastic Neutron Scattering UPt3 𝑈1−𝑥 𝑇ℎ 𝑥 𝐵𝑒13 𝑃𝑟𝑂𝑠4 𝑆𝑏12
  • 4. Common Mechanism? Multi dimensional irreps (order parameter) UPt3 𝑈1−𝑥 𝑇ℎ 𝑥 𝐵𝑒13 𝑃𝑟𝑂𝑠4 𝑆𝑏12 3D (T irreps) 2D (E irreps) 2D (E irreps) 3D (T irreps) 2D (E irreps) A : (1,0) Nematic TRS B : (1,i) Broken TRS A : Time Reversal Symmetry (TRS) B: Time reversal Symmetry Breaking (TRSB) Hexagonal : 𝐷6ℎ Tetrahedral: 𝑇ℎOctarahedral: 𝑂ℎ 𝑇𝑐𝐴 = 550𝑚𝐾 𝑇𝑐𝐵 = 480𝑚𝐾
  • 5. 𝑈𝑃𝑡3 𝛽2> 0 (1,i) 𝛽2 < 0 (1,0) Two transitions ?? AFM → Symmetry Breaking Field : But AFM not long ranged Kioke et. Al 1998
  • 6. 3He Add coupling to paramagnetic fluctuations Large fluctuations imply 𝐴1 → 0 and +ve 𝑑 𝑎 = 𝑘 𝑥 + 𝑖𝑘 𝑦 𝒛 𝑑 𝑏 = 𝑘 A phase puzzling : weak coupling → B stable always We want phenomenogical model Resolved by Anderson & Brinkman : Spin fluctuation feedback effect Couple superfluidity + spin fluctuations : Microscopic
  • 7. The SFEE cheat code Integrate out the Gaussian spin fluctuations 𝑓𝐵 − 𝑓𝐴= 3𝐾2 2 𝐴1 2 , A : Stable with large fluctuations (𝐴1 → 0) A—B transition : temperature dependence 𝛽 → 1 𝑇2 , 𝐾 → 1 𝑇 [ Brinkman et al. 1973, Kozii 2019] Start in A state (SFFE) : T ↓ : → B state (weak coupling)
  • 8. Back to 𝑈𝑃𝑡3 Add a coupling between superconductivity and AFM fluctuations Q1 = 1 2 a*, Q2 = 1 2 (b*-a*), Q3 = − 1 2 b*𝑚1, 𝑚2 and 𝑚3 → New effective free energy 𝛽2 > 0 but ( 𝛽2- 6 4 𝐾2 2 𝐴1 2 ) < 0 → (1,0) : nematic TRS A state A → B TRSB (1,i) as T ↓
  • 9. 𝑈1−𝑥 𝑇ℎ 𝑥 𝐵𝑒13 𝑂ℎ: AFM fluctuations : TRSB ( 𝜇SR) 2D Case * → Kerr Inactive : Ruled out by possible Kerr measurement 3D Case Ruled out by coupling See paper A B A B
  • 10. 𝑃𝑟𝑂𝑠4 𝑆𝑏12 Aoki et al 2003 𝑇ℎ: AFQ fluctuations : TRSB ( 𝜇SR + Polar Kerr) 2D Case A—B Kerr Inactive 3D Case A B
  • 11. Take away • Developed a simple and quick phenomenological approach to generalized SFFE • Provides a unifying description of two transitions in heavy fermion superconductors • 2D 𝐸 𝑔/𝑢 for 𝑃𝑟𝑂𝑠4 𝑆𝑏12 ruled out by polar Kerr • For 𝑈1−𝑥 𝑇ℎ 𝑥 𝐵𝑒13, form SFFE allows only one out of two possible A states • Suggest polar Kerr measurements for 𝑈1−𝑥 𝑇ℎ 𝑥 𝐵𝑒13 → can rule out 2D 𝐸 𝑔/𝑢 rep scenario and constrain 3D (𝑇𝑔/𝑢) situation https://arxiv.org/abs/1910.10780
  • 12. Thank you and Questions https://arxiv.org/abs/1910.10780
  • 13. Effective theory for A—B transitions • Start out in A state of UP𝑡3 stabilized by SFFE i.e. (1,0) with for and for • Grow B phase continuously out of A , i.e. (1 + 𝜂1𝑅 + 𝜂1𝐼, 0 + 𝜂2𝑅+𝜂2𝐼) • Use time reversal symmetry to classify these effective order parameter Want to break time reversal Character table for 𝐷2 → 𝐴1 → 𝐵1 Now use polar Kerr effect Signal trainable by field → order parameter TRSB & has same symmetry as magnetic field (𝑅 𝑥, 𝑅 𝑦, 𝑅 𝑧) Schemm et . al 2014