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International Journal of Trend in Scientific Research and Development (IJTSRD)
Volume 4 Issue 2, February 2020 Available Online: www.ijtsrd.com e-ISSN: 2456 – 6470
@ IJTSRD | Unique Paper ID – IJTSRD30128 | Volume – 4 | Issue – 2 | January-February 2020 Page 688
Effect of Temperature and Humidity on
Indoor Radon Concentration
Jai-Won Chung1, Tae-In Hyon2, Gyu-Sik Kim1
1Department of Electrical and Computer Engineering, University of Seoul, Seoul, South Korea
2Linc+Industry-University Cooperation Group, Jeonju University, Jeonju, South Korea
ABSTRACT
Because radon gas is colorless and odorless, it is impossible for human's five
senses to know whether one is exposed to it and as it is an inert gas that is
nine times heavier than air it is prone to accumulationafterbeing broughtinto
the room through cracks in old buildings, connections and drains, thus
creating indoor radon exposure problem. Although indoor radon
concentration is related to indoor temperature and humidity, no researchhas
been conducted to actually control indoor temperature and humidity, and to
find out how changes in indoor temperature and relative humidity have
affected indoor radon concentration. In this paper, we experimented with
varying temperature and relative humidity respectively to certain conditions
in the laboratory where the thermo-hygrostat is installed, and using the
results of the measured experiment,therelation between indoortemperature,
and relative humidity and indoor radon concentration was explored.
KEYWORDS: radon concentration, temperature, relative humidity, correlation
coefficient
How to cite this paper: Jai-Won Chung |
Tae-In Hyon | Gyu-Sik Kim "Effect of
Temperature and Humidity on Indoor
Radon Concentration" Published in
International Journal
of Trend in Scientific
Research and
Development(ijtsrd),
ISSN: 2456-6470,
Volume-4 | Issue-2,
February 2020,
pp.688-693, URL:
www.ijtsrd.com/papers/ijtsrd30128.pdf
Copyright © 2019 by author(s) and
International Journal ofTrendinScientific
Research and Development Journal. This
is an Open Access article distributed
under the terms of
the Creative
CommonsAttribution
License (CC BY 4.0)
(http://creativecommons.org/licenses/by
/4.0)
I. INTRODUCTION
Radium is generated during the natural decay of uranium or
thorium into lead, and radon is produced when the radium
decays. Radon is colorless, odorless and tasteless and is an
inertgas ninetimesheavierthanair[1].Radon alsohasalong
half-life of 3.82 days, allowing it to stay long in the air. Due to
thesecharacteristics,radoncaneasilybeaccumulatedindoors
and one can be continuously exposed to radon unknowingly
[2]. 80 to 90 percent of radon is generated from the soil and
spreads between pores in the soil, or is emitted from building
grounds and ore, and the radon that has been discharged
enters the room through cracks in old buildings, connections
and drains [3]
If indoor radon concentrations increase and radon stays in
the body for a long time, radon will collapse in the body,
causing mutations in DNA that can cause lung cancer. The
domestic radon exposure limit is 148 Bqm-3 (= 4 pCi / L),
which is the same as the radon exposure limit in the US [4].
According to theUSEnvironmental ProtectionAgency(EPA),
more than 10% of Americans' annual lung cancer deaths,
about 20,000, are due to cumulative exposure of radon
progeny, more than 10 times higher than deaths from air
pollution [5]. The World Health Organization lists radon as
the second leading cause of lung cancer after smoking [6],
and the International Agency for Research on Cancer, a
subsidiary of WHO, has identified radon as a definite
carcinogen [7]. In Korea, the national radon survey
conducted by the National Institute of Environmental
Research shows that the national radon concentration is
50.5 ~ 98.6 Bqm-3, with33.0%ofsingle-familyhomes,14.4%
of townhouses and multi-family houses, and 5.9% of
apartments exposed to radon. It is problematic because it
evidently exceeds the recommended thresholdof148Bqm-3
[8].
Studies have shown that this indoor radon problem is
related to indoor temperatureandhumidity.Brunoreported
that as the indoor temperature increases, the indoor radon
concentration may increase due to thestackingeffectcaused
by the indoorandoutdoortemperaturedifferences,resulting
in an increase in the inflow of soil radon gas,a majorcauseof
the increase in indoor radon concentration [9]. Akbari et al.
analyzed computational fluiddynamicsineight-roomhomes
and found that in the absence of inflow of soil radon gas, the
radon diffusion coefficient and convectionaircirculation are
increased when temperature increases, whichlowersindoor
radon concentration [10]. Kojima et al. measured indoor
radon concentration and seven variables (outdoor radon
concentration, atmospheric pressure, change in pressure,
indoor temperature, indoor steam pressure, indoor and
outdoor temperature difference, wind speed) in a closed-
door environment, and investigated a correlation between
indoor radon concentration and each of the variables and
reported a high correlation between indoor steam pressure
and indoor radon concentration [11]. Janik et al. tested the
relationship between absolute humidity and radon
IJTSRD30128
International Journal of Trend in Scientific Research and Development (IJTSRD) @ www.ijtsrd.com eISSN: 2456-6470
@ IJTSRD | Unique Paper ID – IJTSRD30128 | Volume – 4 | Issue – 2 | January-February 2020 Page 689
exhalation rate of building materials by placing bricks and
granite in the chamber and changing the absolute humidity
and reported that the radon emission rate of materials
tended to increase as absolute humidity increased [12].
Although such changes in indoor temperature and humidity
can affect indoor radon concentration, no study was
conducted to determine the effect of room temperature and
relative humidity on indoor radon concentration by
measuring only temperature and relative humidity in actual
indoor environment.
In this paper, the effect of changes in room temperature and
relative humidity on indoor radon concentration was
investigated experimentally. A total of nine experiments
were conducted in the laboratory where the thermo-
hygrostat was installed, varying the temperature and
relative humidity respectively to certain conditions, and the
relationship between indoor temperature,relativehumidity
and indoor radon concentration was explored using the
statistical analysis.
II. Main Results
2.1. Experiment method
Figure 1 shows the temperature and humidity sensor
module used in the experiment. The temperature and
humidity sensor module was implemented using the
Arduino Mega 2560 and the DHT22 (Aosong ElectronicsCo.,
China) sensor that can measure temperature and relative
humidity. For DHT22 sensors, the measurement error is
±0.5°C at the temperature range of -40°C to 80°C, and the
measurement error is ±2% at the relative humidity range of
0% to 100%. Temperature and humidity sensorsweresetto
measure temperature and relative humidity every 1minute.
The high precision radon concentration measuring
equipment RAD7 (DURRIDGE Company Inc., USA) was used
to measure the concentration of radon during the
experiment, and a dehumidifying filter was used for the
measurement to remove the effects of humidity, and the
concentration of radon was set to be measured every hour.
(a) DHT22 (b) Arduino (c) Implemented
Temperature Mega 2560 temperature and
humidity sensor humidity sensor
Module
Fig.1. Temperature and humidity sensor module
The experiment was conducted in an electrical engineering
laboratory on the first floor of the Information Technology
Museum at University of Seoul, where thermo-hygrostat AP-
DPA-100UE (AR Co., Korea) is installed to maintainconstant
room temperature and relative humidity conditions. EPA
(Environmental Protection Agency) recommends that the
measurement equipment be spaced at least 90 cm away
from windows or exterior doors, at least 50 cm from the
ground, and at least 10 cm from other objects when
measuring indoor radon concentrations [5]. Therefore, the
measuring equipment was separated by 60cm from the
ground using an acrylic box in the center of the laboratory,
and the equipment was installed to maintain a distance of at
least 10cm from other objects.
To find out the effect of temperature and relative humidity
changes on indoor radon concentration, the thermo-
hygrostat was used to set the temperature at 10°C, 20°C,
30°C, and the relative humidity at 20%, 50%, and 80%,
respectively, and the temperature, relative humidity and
radon concentration were measured under each condition,
resulting in a total of nine experiments. EPA recommends
that indoor radon concentration measurements be done
under closed conditions 12 hours prior to measurementand
continuous-type radon measurement equipment should be
measured continuously for at least 48 hours [13].Therefore,
after measuring a total of 84 hours per experiment, data
from the beginning of the measurement to 12 hours were
not used, and 72 hours of subsequent data were used to
analyze the effects of relative humidity and temperature.
Figure 2 shows the temperature, relative humidity and
radon concentration values measured for a total of 84 hours
at a temperature of 20°C and a relative humidity of 50%.
Fig.2. Temperature, relative humidity, and radon
concentration values measured for a total of 84 hours
at a temperature of 20 ° C and a relative humidity of
50%
2.2. Analysis and Discussion
For each of the nine experiments, the results were analyzed
using measured temperature, relative humidity and radon
concentration measurements for 72 hours each. For
temperature and relative humidity, the temperature and
humidity sensor module averaged the measured values that
were taken at a minute interval over each hour. For radon
concentration, the values measured at intervals of one hour
in RAD7 were used. To evaluate the effect of temperature
and relative humidity on indoor radon concentration, the
Spearman correlationcoefficientoftemperatureand relative
humidity were obtained respectively.
Table 1 shows the average and standard deviation values of
temperature, relative humidity, radon concentration,
measured at intervals of one hour for a total of 72 hours for
each experiment. In each experiment, the measured mean
and standard deviation values of the temperature and the
relative humidity, respectively, confirmed that the
temperature and relativehumidityadheredtotheconditions
set during the experiment. A maximum mean radon
concentration of 68.34 Bqm-3 was measured with a
minimum set temperature of 10°C and a maximum set
relative humidity of 80%, and a minimum mean radon
concentration of 45.07 Bqm-3 was measured with a
maximum set temperature of 30°C and a minimum set
relative humidity of 20%.
International Journal of Trend in Scientific Research and Development (IJTSRD) @ www.ijtsrd.com eISSN: 2456-6470
@ IJTSRD | Unique Paper ID – IJTSRD30128 | Volume – 4 | Issue – 2 | January-February 2020 Page 690
Table1. Average ± standard deviation value of the temperature, relative humidity and radon concentration
measured for a total of 72 hours for each experiment
Experiments Temperature (°C) Relative Humidity (%) Radon Concentration (Bqm-3)
Experiment (1) 9.99 ± 0.37 19.66 ± 0.90 59.37 ± 9.56
Experiment (2) 21.14 ±0.62 20.18 ± 1.18 51.84 ± 7.14
Experiment (3) 29.97± 0.69 21.54 ± 0.62 45.07 ± 9.69
Experiment (4) 9.59 ± 0.50 50.92 ± 1.03 63.14 ± 10.53
Experiment (5) 19.90 ± 0.49 50.28 ± 0.86 56.32 ± 9.85
Experiment (6) 31.12 ± 0.41 49.66 ± 1.05 46.73 ± 7.66
Experiment (7) 10.08 ± 0.39 79.58 ± 0.63 68.34 ± 10.74
Experiment (8) 20.56 ± 0.55 80.39 ± 1.12 59.31 ± 7.85
Experiment (9) 29.56 ± 0.72 81.10 ± 0.84 49.04 ± 9.26
To evaluate the effect of temperature and humidity on the change of indoor radon concentration, the Spearman correlation
coefficient of temperature and relative humidity for radon concentration was calculated and the scatter plot was plotted. For
the Spearman correlation coefficient of relative humidity and radon concentration, the r value was 0.12 when theP-valuewas
less than 0.05, indicating that there was a slight correlation between the two variables. The Spearman'scorrelation coefficient
of temperature and radon concentration showed an r value of -0.53 when theP-valuewaslessthan0.001,indicating a negative
correlation between the two variables. Figure 3 shows the scatter plot of temperature and relative humidity for radon
concentration. This shows that there is a negative correlation between temperature and radon concentration, and there is a
slight correlation between relative humidity and radon concentration.
(a) Temperature and radon concentration (n=648)
(b) Relative humidity and radon concentration (n=648)
Fig. 3. Scatter plot of temperature and relative humidity for radon concentration
Table2. Spearman correlation coefficient of temperature and radon concentration at each relative humidity
Spearman
correlation coefficient
Relative Humidity 20%
(n=216)
Relative Humidity 50%
(n=216)
Relative Humidity 80%
(n=216)
r -0.49 -0.54 -0.56
p-value ≤0.01 ≤0.01 ≤0.01
International Journal of Trend in Scientific Research and Development (IJTSRD) @ www.ijtsrd.com eISSN: 2456-6470
@ IJTSRD | Unique Paper ID – IJTSRD30128 | Volume – 4 | Issue – 2 | January-February 2020 Page 691
Table 2 shows the Spearman's correlation coefficient between temperatureand radonconcentrationateachrelative humidity.
The correlation coefficient between temperature and radon concentration was -0.49 for relative humidity of 20%, -0.54 for
relative humidity of 50%, and -0.56 for relative humidity of 80%, with p-value ≤ 0.01 in all cases. This indicates that under all
relative humidity conditions there is a negative correlation between thetwovariables, andthatradonconcentrationdecreases
as the room temperature increases. Figure 4 shows the scatter plot of temperature and radon concentration at each relative
humidity condition. This confirms that there is a negative correlation between temperature and radon concentration at all
relative humidity.
(a) 20% relative humidity (n=216)
(b) 50% relative humidity (n=216)
(c) 80% relative humidity (n=216)
Fig. 4. Scatter plot of temperature radon concentration
International Journal of Trend in Scientific Research and Development (IJTSRD) @ www.ijtsrd.com eISSN: 2456-6470
@ IJTSRD | Unique Paper ID – IJTSRD30128 | Volume – 4 | Issue – 2 | January-February 2020 Page 692
Table 3 shows the Spearman's correlation coefficients for relative humidity and radon concentration at each temperature.
Correlation coefficients betweenrelativehumidityandradonconcentrationsshowedthattherewasa weak positivecorrelation
between the two variables, with r values of 0.23 and 0.32, respectively, at 10 ° C and 20 ° C, all with p-value ≤ 0.01, but at
temperature of 30 ° C, the r-value was 0.09 at p-value = 0.172 and no statistically significantcorrelationwasobserved.Figure5
shows the scatter plots of relative humidity and radonconcentrationateachtemperaturecondition.Throughthisitcanbeseen
that when the temperature is 10 ° C or 20 ° C there is a weak positive correlation between the relative humidity and radon
concentration. When the temperature is 30 ° C, the correlation is not large, but as the relative humidity is increased, the radon
concentration is slightly increased.
Table3. Spearman correlation coefficient of relative humidity and radon concentration at each temperature
Spearman
correlation coefficient
Temperature 10°C
(n=216)
Temperature 20°C
(n=216)
Temperature 30°C
(n=216)
r 0.23 0.32 0.09
p-value ≤0.01 ≤0.01 0.17
(a) 10 ° C temperature (n=216)
(b) 20 ° C temperature (n=216)
(c) 30 ° C temperature (n=216)
Fig. 5. Scatter plot of relative humidity and radon concentration
International Journal of Trend in Scientific Research and Development (IJTSRD) @ www.ijtsrd.com eISSN: 2456-6470
@ IJTSRD | Unique Paper ID – IJTSRD30128 | Volume – 4 | Issue – 2 | January-February 2020 Page 693
III. Conclusion
In this study, the effects of room temperature and relative
humidity on the indoor radon concentration were
experimentally investigated. In the case of room
temperature and radon concentration, radon concentration
tended to decrease with increasing temperature regardless
of relative humidity. In the absence of soil radon gasinflows,
an increase in indoor temperature can reduce indoor radon
concentration by increasing convective air circulation and
radon diffusion coefficients, thereby reducing the indoor
radon concentration [10]. For this reason, the radon
concentration tends to decrease with increasing room
temperature. In the case of relative humidity, the radon
concentration tended to increase as the relative humidity
increased except in the case where the temperature was30°
C. Increased humidity may increase the amount ofradongas
emitted from building materials such as bricks and cements
[12]. For this reason, indoor radon concentrations tended to
increase with relative humidity. However, it was found that
temperature had a greater effect on indoor radon
concentration than relative humidity. For the effects of
temperature and relative humidity changes onindoorradon
concentrations, the propensity and degree of influence may
vary depending on the location or environment of
measurement. Therefore, further research in various places
and environments is deemed to be necessary.
Acknowledgment
This work was also supported by the National Research
Foundation of Korea (NRF) grant funded by the Korea
government (MSIP) (No. 2019R1H1A 2101157).
References
[1] NCRP (National Council on Radiation Protection and
Measurements), “Measurement of radon and radon
daughters in air”, Recommendations of the National
Council on Radiation Protection and Measurements.
Bethesda, No.97, 1988.
[2] International Commission on Radiological Protection
(ICRP), “Radiological protection against radón
exposure, ICRP Publication 126”, ICRP, Vol.43, No.3,
2014.
[3] R.C. Bruno, “Sources of indoor radon in houses: a
review”, Journal of the Air Pollution Control
Association, Vol.33, No.2, pp.105-109, 1983.
[4] Korea Environment Corporation, "Internal Radon
Management," Korea Environment Corporation, 2016.
[5] United States Environmental Protection Agency
(USEPA), “A Citizen’s Guide to Radon”, USEPA,
EPA/402/K-12/002, 2012.
[6] World Health Organization (WHO), “Handbook on
Indoor Radon”, WHO Press., Geneva, 2009.
[7] International Agency for Research on Cancer, “Man-
made mineral fibres and radon: summary of data
reported and evaluation”, IARC monographs, Vol.43,
1988.
[8] Ministry of Environment of Republic of Korea (MoE),
“Development of RadonMitigationStandardManual by
Building Types”, MoE, 2013.
[9] R.C. Bruno, "Sources of indoor radon in houses: a
review", Journal of the Air Pollution Control
Association, vol. 33, no. 2, pp. 105-109, 1983.
[10] Environmental K. Akbari, J. Mahmoudi, M. Ghanbari,
“Influence of indoor air conditions on radon
concentration in a detached house”, Journal of
environmental radioactivity”, vol. 116, pp. 166-173,
2013.
[11] H. Kojima, S. Abe, “Effect of HumiditytotheVariationof
Radon Daughter Concentrationina building”, Japanese
Journal of Health Physics, vol. 20, no. 4, pp. 379-383,
1985.
[12] M. Janik, Y. Omori, H. Yonehara, “Influence of humidity
on radon and thoron exhalation rates from building
materials”, applied radiation and Isotopes, vol. 95, pp.
102-107, 2015.
[13] Environmental Protection Agency (EPA), “Indoor
Radon and Radon Decay Product Measurement Device
Protocol“, EPA 402-R-92-004, 1992.

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Effect of Temperature and Humidity on Indoor Radon Concentration

  • 1. International Journal of Trend in Scientific Research and Development (IJTSRD) Volume 4 Issue 2, February 2020 Available Online: www.ijtsrd.com e-ISSN: 2456 – 6470 @ IJTSRD | Unique Paper ID – IJTSRD30128 | Volume – 4 | Issue – 2 | January-February 2020 Page 688 Effect of Temperature and Humidity on Indoor Radon Concentration Jai-Won Chung1, Tae-In Hyon2, Gyu-Sik Kim1 1Department of Electrical and Computer Engineering, University of Seoul, Seoul, South Korea 2Linc+Industry-University Cooperation Group, Jeonju University, Jeonju, South Korea ABSTRACT Because radon gas is colorless and odorless, it is impossible for human's five senses to know whether one is exposed to it and as it is an inert gas that is nine times heavier than air it is prone to accumulationafterbeing broughtinto the room through cracks in old buildings, connections and drains, thus creating indoor radon exposure problem. Although indoor radon concentration is related to indoor temperature and humidity, no researchhas been conducted to actually control indoor temperature and humidity, and to find out how changes in indoor temperature and relative humidity have affected indoor radon concentration. In this paper, we experimented with varying temperature and relative humidity respectively to certain conditions in the laboratory where the thermo-hygrostat is installed, and using the results of the measured experiment,therelation between indoortemperature, and relative humidity and indoor radon concentration was explored. KEYWORDS: radon concentration, temperature, relative humidity, correlation coefficient How to cite this paper: Jai-Won Chung | Tae-In Hyon | Gyu-Sik Kim "Effect of Temperature and Humidity on Indoor Radon Concentration" Published in International Journal of Trend in Scientific Research and Development(ijtsrd), ISSN: 2456-6470, Volume-4 | Issue-2, February 2020, pp.688-693, URL: www.ijtsrd.com/papers/ijtsrd30128.pdf Copyright © 2019 by author(s) and International Journal ofTrendinScientific Research and Development Journal. This is an Open Access article distributed under the terms of the Creative CommonsAttribution License (CC BY 4.0) (http://creativecommons.org/licenses/by /4.0) I. INTRODUCTION Radium is generated during the natural decay of uranium or thorium into lead, and radon is produced when the radium decays. Radon is colorless, odorless and tasteless and is an inertgas ninetimesheavierthanair[1].Radon alsohasalong half-life of 3.82 days, allowing it to stay long in the air. Due to thesecharacteristics,radoncaneasilybeaccumulatedindoors and one can be continuously exposed to radon unknowingly [2]. 80 to 90 percent of radon is generated from the soil and spreads between pores in the soil, or is emitted from building grounds and ore, and the radon that has been discharged enters the room through cracks in old buildings, connections and drains [3] If indoor radon concentrations increase and radon stays in the body for a long time, radon will collapse in the body, causing mutations in DNA that can cause lung cancer. The domestic radon exposure limit is 148 Bqm-3 (= 4 pCi / L), which is the same as the radon exposure limit in the US [4]. According to theUSEnvironmental ProtectionAgency(EPA), more than 10% of Americans' annual lung cancer deaths, about 20,000, are due to cumulative exposure of radon progeny, more than 10 times higher than deaths from air pollution [5]. The World Health Organization lists radon as the second leading cause of lung cancer after smoking [6], and the International Agency for Research on Cancer, a subsidiary of WHO, has identified radon as a definite carcinogen [7]. In Korea, the national radon survey conducted by the National Institute of Environmental Research shows that the national radon concentration is 50.5 ~ 98.6 Bqm-3, with33.0%ofsingle-familyhomes,14.4% of townhouses and multi-family houses, and 5.9% of apartments exposed to radon. It is problematic because it evidently exceeds the recommended thresholdof148Bqm-3 [8]. Studies have shown that this indoor radon problem is related to indoor temperatureandhumidity.Brunoreported that as the indoor temperature increases, the indoor radon concentration may increase due to thestackingeffectcaused by the indoorandoutdoortemperaturedifferences,resulting in an increase in the inflow of soil radon gas,a majorcauseof the increase in indoor radon concentration [9]. Akbari et al. analyzed computational fluiddynamicsineight-roomhomes and found that in the absence of inflow of soil radon gas, the radon diffusion coefficient and convectionaircirculation are increased when temperature increases, whichlowersindoor radon concentration [10]. Kojima et al. measured indoor radon concentration and seven variables (outdoor radon concentration, atmospheric pressure, change in pressure, indoor temperature, indoor steam pressure, indoor and outdoor temperature difference, wind speed) in a closed- door environment, and investigated a correlation between indoor radon concentration and each of the variables and reported a high correlation between indoor steam pressure and indoor radon concentration [11]. Janik et al. tested the relationship between absolute humidity and radon IJTSRD30128
  • 2. International Journal of Trend in Scientific Research and Development (IJTSRD) @ www.ijtsrd.com eISSN: 2456-6470 @ IJTSRD | Unique Paper ID – IJTSRD30128 | Volume – 4 | Issue – 2 | January-February 2020 Page 689 exhalation rate of building materials by placing bricks and granite in the chamber and changing the absolute humidity and reported that the radon emission rate of materials tended to increase as absolute humidity increased [12]. Although such changes in indoor temperature and humidity can affect indoor radon concentration, no study was conducted to determine the effect of room temperature and relative humidity on indoor radon concentration by measuring only temperature and relative humidity in actual indoor environment. In this paper, the effect of changes in room temperature and relative humidity on indoor radon concentration was investigated experimentally. A total of nine experiments were conducted in the laboratory where the thermo- hygrostat was installed, varying the temperature and relative humidity respectively to certain conditions, and the relationship between indoor temperature,relativehumidity and indoor radon concentration was explored using the statistical analysis. II. Main Results 2.1. Experiment method Figure 1 shows the temperature and humidity sensor module used in the experiment. The temperature and humidity sensor module was implemented using the Arduino Mega 2560 and the DHT22 (Aosong ElectronicsCo., China) sensor that can measure temperature and relative humidity. For DHT22 sensors, the measurement error is ±0.5°C at the temperature range of -40°C to 80°C, and the measurement error is ±2% at the relative humidity range of 0% to 100%. Temperature and humidity sensorsweresetto measure temperature and relative humidity every 1minute. The high precision radon concentration measuring equipment RAD7 (DURRIDGE Company Inc., USA) was used to measure the concentration of radon during the experiment, and a dehumidifying filter was used for the measurement to remove the effects of humidity, and the concentration of radon was set to be measured every hour. (a) DHT22 (b) Arduino (c) Implemented Temperature Mega 2560 temperature and humidity sensor humidity sensor Module Fig.1. Temperature and humidity sensor module The experiment was conducted in an electrical engineering laboratory on the first floor of the Information Technology Museum at University of Seoul, where thermo-hygrostat AP- DPA-100UE (AR Co., Korea) is installed to maintainconstant room temperature and relative humidity conditions. EPA (Environmental Protection Agency) recommends that the measurement equipment be spaced at least 90 cm away from windows or exterior doors, at least 50 cm from the ground, and at least 10 cm from other objects when measuring indoor radon concentrations [5]. Therefore, the measuring equipment was separated by 60cm from the ground using an acrylic box in the center of the laboratory, and the equipment was installed to maintain a distance of at least 10cm from other objects. To find out the effect of temperature and relative humidity changes on indoor radon concentration, the thermo- hygrostat was used to set the temperature at 10°C, 20°C, 30°C, and the relative humidity at 20%, 50%, and 80%, respectively, and the temperature, relative humidity and radon concentration were measured under each condition, resulting in a total of nine experiments. EPA recommends that indoor radon concentration measurements be done under closed conditions 12 hours prior to measurementand continuous-type radon measurement equipment should be measured continuously for at least 48 hours [13].Therefore, after measuring a total of 84 hours per experiment, data from the beginning of the measurement to 12 hours were not used, and 72 hours of subsequent data were used to analyze the effects of relative humidity and temperature. Figure 2 shows the temperature, relative humidity and radon concentration values measured for a total of 84 hours at a temperature of 20°C and a relative humidity of 50%. Fig.2. Temperature, relative humidity, and radon concentration values measured for a total of 84 hours at a temperature of 20 ° C and a relative humidity of 50% 2.2. Analysis and Discussion For each of the nine experiments, the results were analyzed using measured temperature, relative humidity and radon concentration measurements for 72 hours each. For temperature and relative humidity, the temperature and humidity sensor module averaged the measured values that were taken at a minute interval over each hour. For radon concentration, the values measured at intervals of one hour in RAD7 were used. To evaluate the effect of temperature and relative humidity on indoor radon concentration, the Spearman correlationcoefficientoftemperatureand relative humidity were obtained respectively. Table 1 shows the average and standard deviation values of temperature, relative humidity, radon concentration, measured at intervals of one hour for a total of 72 hours for each experiment. In each experiment, the measured mean and standard deviation values of the temperature and the relative humidity, respectively, confirmed that the temperature and relativehumidityadheredtotheconditions set during the experiment. A maximum mean radon concentration of 68.34 Bqm-3 was measured with a minimum set temperature of 10°C and a maximum set relative humidity of 80%, and a minimum mean radon concentration of 45.07 Bqm-3 was measured with a maximum set temperature of 30°C and a minimum set relative humidity of 20%.
  • 3. International Journal of Trend in Scientific Research and Development (IJTSRD) @ www.ijtsrd.com eISSN: 2456-6470 @ IJTSRD | Unique Paper ID – IJTSRD30128 | Volume – 4 | Issue – 2 | January-February 2020 Page 690 Table1. Average ± standard deviation value of the temperature, relative humidity and radon concentration measured for a total of 72 hours for each experiment Experiments Temperature (°C) Relative Humidity (%) Radon Concentration (Bqm-3) Experiment (1) 9.99 ± 0.37 19.66 ± 0.90 59.37 ± 9.56 Experiment (2) 21.14 ±0.62 20.18 ± 1.18 51.84 ± 7.14 Experiment (3) 29.97± 0.69 21.54 ± 0.62 45.07 ± 9.69 Experiment (4) 9.59 ± 0.50 50.92 ± 1.03 63.14 ± 10.53 Experiment (5) 19.90 ± 0.49 50.28 ± 0.86 56.32 ± 9.85 Experiment (6) 31.12 ± 0.41 49.66 ± 1.05 46.73 ± 7.66 Experiment (7) 10.08 ± 0.39 79.58 ± 0.63 68.34 ± 10.74 Experiment (8) 20.56 ± 0.55 80.39 ± 1.12 59.31 ± 7.85 Experiment (9) 29.56 ± 0.72 81.10 ± 0.84 49.04 ± 9.26 To evaluate the effect of temperature and humidity on the change of indoor radon concentration, the Spearman correlation coefficient of temperature and relative humidity for radon concentration was calculated and the scatter plot was plotted. For the Spearman correlation coefficient of relative humidity and radon concentration, the r value was 0.12 when theP-valuewas less than 0.05, indicating that there was a slight correlation between the two variables. The Spearman'scorrelation coefficient of temperature and radon concentration showed an r value of -0.53 when theP-valuewaslessthan0.001,indicating a negative correlation between the two variables. Figure 3 shows the scatter plot of temperature and relative humidity for radon concentration. This shows that there is a negative correlation between temperature and radon concentration, and there is a slight correlation between relative humidity and radon concentration. (a) Temperature and radon concentration (n=648) (b) Relative humidity and radon concentration (n=648) Fig. 3. Scatter plot of temperature and relative humidity for radon concentration Table2. Spearman correlation coefficient of temperature and radon concentration at each relative humidity Spearman correlation coefficient Relative Humidity 20% (n=216) Relative Humidity 50% (n=216) Relative Humidity 80% (n=216) r -0.49 -0.54 -0.56 p-value ≤0.01 ≤0.01 ≤0.01
  • 4. International Journal of Trend in Scientific Research and Development (IJTSRD) @ www.ijtsrd.com eISSN: 2456-6470 @ IJTSRD | Unique Paper ID – IJTSRD30128 | Volume – 4 | Issue – 2 | January-February 2020 Page 691 Table 2 shows the Spearman's correlation coefficient between temperatureand radonconcentrationateachrelative humidity. The correlation coefficient between temperature and radon concentration was -0.49 for relative humidity of 20%, -0.54 for relative humidity of 50%, and -0.56 for relative humidity of 80%, with p-value ≤ 0.01 in all cases. This indicates that under all relative humidity conditions there is a negative correlation between thetwovariables, andthatradonconcentrationdecreases as the room temperature increases. Figure 4 shows the scatter plot of temperature and radon concentration at each relative humidity condition. This confirms that there is a negative correlation between temperature and radon concentration at all relative humidity. (a) 20% relative humidity (n=216) (b) 50% relative humidity (n=216) (c) 80% relative humidity (n=216) Fig. 4. Scatter plot of temperature radon concentration
  • 5. International Journal of Trend in Scientific Research and Development (IJTSRD) @ www.ijtsrd.com eISSN: 2456-6470 @ IJTSRD | Unique Paper ID – IJTSRD30128 | Volume – 4 | Issue – 2 | January-February 2020 Page 692 Table 3 shows the Spearman's correlation coefficients for relative humidity and radon concentration at each temperature. Correlation coefficients betweenrelativehumidityandradonconcentrationsshowedthattherewasa weak positivecorrelation between the two variables, with r values of 0.23 and 0.32, respectively, at 10 ° C and 20 ° C, all with p-value ≤ 0.01, but at temperature of 30 ° C, the r-value was 0.09 at p-value = 0.172 and no statistically significantcorrelationwasobserved.Figure5 shows the scatter plots of relative humidity and radonconcentrationateachtemperaturecondition.Throughthisitcanbeseen that when the temperature is 10 ° C or 20 ° C there is a weak positive correlation between the relative humidity and radon concentration. When the temperature is 30 ° C, the correlation is not large, but as the relative humidity is increased, the radon concentration is slightly increased. Table3. Spearman correlation coefficient of relative humidity and radon concentration at each temperature Spearman correlation coefficient Temperature 10°C (n=216) Temperature 20°C (n=216) Temperature 30°C (n=216) r 0.23 0.32 0.09 p-value ≤0.01 ≤0.01 0.17 (a) 10 ° C temperature (n=216) (b) 20 ° C temperature (n=216) (c) 30 ° C temperature (n=216) Fig. 5. Scatter plot of relative humidity and radon concentration
  • 6. International Journal of Trend in Scientific Research and Development (IJTSRD) @ www.ijtsrd.com eISSN: 2456-6470 @ IJTSRD | Unique Paper ID – IJTSRD30128 | Volume – 4 | Issue – 2 | January-February 2020 Page 693 III. Conclusion In this study, the effects of room temperature and relative humidity on the indoor radon concentration were experimentally investigated. In the case of room temperature and radon concentration, radon concentration tended to decrease with increasing temperature regardless of relative humidity. In the absence of soil radon gasinflows, an increase in indoor temperature can reduce indoor radon concentration by increasing convective air circulation and radon diffusion coefficients, thereby reducing the indoor radon concentration [10]. For this reason, the radon concentration tends to decrease with increasing room temperature. In the case of relative humidity, the radon concentration tended to increase as the relative humidity increased except in the case where the temperature was30° C. Increased humidity may increase the amount ofradongas emitted from building materials such as bricks and cements [12]. For this reason, indoor radon concentrations tended to increase with relative humidity. However, it was found that temperature had a greater effect on indoor radon concentration than relative humidity. For the effects of temperature and relative humidity changes onindoorradon concentrations, the propensity and degree of influence may vary depending on the location or environment of measurement. Therefore, further research in various places and environments is deemed to be necessary. Acknowledgment This work was also supported by the National Research Foundation of Korea (NRF) grant funded by the Korea government (MSIP) (No. 2019R1H1A 2101157). References [1] NCRP (National Council on Radiation Protection and Measurements), “Measurement of radon and radon daughters in air”, Recommendations of the National Council on Radiation Protection and Measurements. Bethesda, No.97, 1988. [2] International Commission on Radiological Protection (ICRP), “Radiological protection against radón exposure, ICRP Publication 126”, ICRP, Vol.43, No.3, 2014. [3] R.C. Bruno, “Sources of indoor radon in houses: a review”, Journal of the Air Pollution Control Association, Vol.33, No.2, pp.105-109, 1983. [4] Korea Environment Corporation, "Internal Radon Management," Korea Environment Corporation, 2016. [5] United States Environmental Protection Agency (USEPA), “A Citizen’s Guide to Radon”, USEPA, EPA/402/K-12/002, 2012. [6] World Health Organization (WHO), “Handbook on Indoor Radon”, WHO Press., Geneva, 2009. [7] International Agency for Research on Cancer, “Man- made mineral fibres and radon: summary of data reported and evaluation”, IARC monographs, Vol.43, 1988. [8] Ministry of Environment of Republic of Korea (MoE), “Development of RadonMitigationStandardManual by Building Types”, MoE, 2013. [9] R.C. Bruno, "Sources of indoor radon in houses: a review", Journal of the Air Pollution Control Association, vol. 33, no. 2, pp. 105-109, 1983. [10] Environmental K. Akbari, J. Mahmoudi, M. Ghanbari, “Influence of indoor air conditions on radon concentration in a detached house”, Journal of environmental radioactivity”, vol. 116, pp. 166-173, 2013. [11] H. Kojima, S. Abe, “Effect of HumiditytotheVariationof Radon Daughter Concentrationina building”, Japanese Journal of Health Physics, vol. 20, no. 4, pp. 379-383, 1985. [12] M. Janik, Y. Omori, H. Yonehara, “Influence of humidity on radon and thoron exhalation rates from building materials”, applied radiation and Isotopes, vol. 95, pp. 102-107, 2015. [13] Environmental Protection Agency (EPA), “Indoor Radon and Radon Decay Product Measurement Device Protocol“, EPA 402-R-92-004, 1992.