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Pressure Dependance of the Curie temperature of TbNi 2 Mn, Investigated Using Designer Diamond Anvils Damon D Jackson Scott K McCall Sam T Weir Lawrence Livermore Nat’l Lab Wei Qiu Yogesh K. Vohra Univ. Alabama, Birmingham Dave P Young Louisiana State University UCRL-PRES-228374 ; This work was performed under the auspices of the U.S. Department of Energy by University of California, Lawrence Livermore National Laboratory under Contract W-7405-Eng-48.
Pressure Dependance of the Curie temperature of TbNi 2 Mn, Investigated Using Designer Diamond Anvils Wei Qiu Yogesh K. Vohra Univ. Alabama, Birmingham Damon D Jackson Scott K McCall Sam T Weir Lawrence Livermore Nat’l Lab Dave P Young Louisiana State University UCRL-PRES-228374 ; This work was performed under the auspices of the U.S. Department of Energy by University of California, Lawrence Livermore National Laboratory under Contract W-7405-Eng-48.
3 d  - 4 f  magnetic interactions ,[object Object],[object Object],[object Object],[object Object],[object Object],Cubic Laves Structure MgCu 2 -type R  site - (green) diamond lattice T  site - (red) tetrahedra around  R
R Ni 2 Mn is Cubic Laves!  ,[object Object],[object Object],[object Object],[object Object]
Compounds for Comparison:  R Mn 2 ,[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],GdMn 2  Phase Diagram
Compounds for Comparison:  R Ni 2 ,[object Object],[object Object],[object Object],[object Object],[object Object],TbNi 2  Properties
Compounds for Comparison: TbMn 2
Motivation for TbNi 2 Mn ,[object Object],[object Object],[object Object],GdMn 2 TbNi 2 What are the anomalies in TbNi 2 Mn?
R Ni 2 Mn - Cubic Laves FM ,[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],T C  = 151 K Magnetization of TbNi 2 Mn T C  vs de Gennes
Feature at  T* ≈37 K ,[object Object],[object Object],[object Object],[object Object],ZFC Magnetization 50 G 100 G 200 G Magnetization, 400 G FC ZFC
Magnetic Field Dependancies ,[object Object],[object Object],Coercivity T*  Anomaly
Specific Heat of TbNi 2 Mn ,[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],Specific Heat
Investigate High Pressure Magnetic Phase Diagram ,[object Object],[object Object]
Designer Diamond Anvils ,[object Object],[object Object],[object Object],[object Object],60-250 µm 4-12 µm
[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],Designer Diamond Anvil Fabrication 300 µm
Representative Results ,[object Object],[object Object],[object Object],MEW AC Susceptibility no pressure medium
Magnetic Phase Diagram ,[object Object],[object Object],[object Object],[object Object],[object Object],P-medium No P-medium Download Magnetic Phase Diagram
Conclusions ,[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],Magnetic Phase Diagram Magnetization of TbNi 2 Mn T*  Anomaly Cubic Laves Crystal Structure ( R 1-2 x ◻ y Mn 2 x - y )(Ni 1- x Mn x ) 2
Questions Remain... ,[object Object],[object Object],[object Object],[object Object],[object Object],Magnetic Phase Diagram
[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],Designer Diamond Anvils for AC Magnetic Susceptibility
Magnetic Susceptibility Schematic ,[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object]
[object Object],[object Object],[object Object],Designer Diamond Anvils for AC Magnetic Susceptibility
Conventional Magnetic Susceptibility with a DAC T. Timofeev, et al., Fizika I Tekhnika Vysokikh Davlenii,  16 , 15 (1984) low sensitivity low signal to noise
Magnetic Susceptibility with Designer Diamond Anvils •  χ ac  experiments are difficult because magnetic field decreases as  1 /r 3 •  Using Designer Diamond Anvils, “filling factor” is drastically increased due to embedded microloops •  10-turn pick-up coil •  coil lines are 5 µm wide and 0.35 µm thick •  mechanically robust •  high signal-to-noise sensitivity (10 -2 emu/cm 3 ) •  no need for a compensation coil
Multiloop Designer Anvil Fabrication Lithographic Fabrication Diamond Encapsulation Diamond Polishing (reflected light) Completed Anvil (transmitted light)
[object Object],[object Object],[object Object],[object Object],Experimental Setup

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Pressure Dependance of Tc for TbNi2Mn

  • 1. Pressure Dependance of the Curie temperature of TbNi 2 Mn, Investigated Using Designer Diamond Anvils Damon D Jackson Scott K McCall Sam T Weir Lawrence Livermore Nat’l Lab Wei Qiu Yogesh K. Vohra Univ. Alabama, Birmingham Dave P Young Louisiana State University UCRL-PRES-228374 ; This work was performed under the auspices of the U.S. Department of Energy by University of California, Lawrence Livermore National Laboratory under Contract W-7405-Eng-48.
  • 2. Pressure Dependance of the Curie temperature of TbNi 2 Mn, Investigated Using Designer Diamond Anvils Wei Qiu Yogesh K. Vohra Univ. Alabama, Birmingham Damon D Jackson Scott K McCall Sam T Weir Lawrence Livermore Nat’l Lab Dave P Young Louisiana State University UCRL-PRES-228374 ; This work was performed under the auspices of the U.S. Department of Energy by University of California, Lawrence Livermore National Laboratory under Contract W-7405-Eng-48.
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  • 14.
  • 15.
  • 16.
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  • 19.
  • 20.
  • 21.
  • 22.
  • 23. Conventional Magnetic Susceptibility with a DAC T. Timofeev, et al., Fizika I Tekhnika Vysokikh Davlenii, 16 , 15 (1984) low sensitivity low signal to noise
  • 24. Magnetic Susceptibility with Designer Diamond Anvils • χ ac experiments are difficult because magnetic field decreases as 1 /r 3 • Using Designer Diamond Anvils, “filling factor” is drastically increased due to embedded microloops • 10-turn pick-up coil • coil lines are 5 µm wide and 0.35 µm thick • mechanically robust • high signal-to-noise sensitivity (10 -2 emu/cm 3 ) • no need for a compensation coil
  • 25. Multiloop Designer Anvil Fabrication Lithographic Fabrication Diamond Encapsulation Diamond Polishing (reflected light) Completed Anvil (transmitted light)
  • 26.